We study the scattering of light by a binary system of identical atoms in which one of them is incoherently pumped. This system belongs to the kind of non-parity symmetric optical systems in which gains and losses are partially compensated. We carry out a fully quantum analysis of the directionality of the radiation scattered from the atoms when the incident light strikes the system either perpendicular or alongside the interatomic axis. By resolving the emitted field in space, the microscopic mechanisms associated with photon exchange, interference, and reciprocity become directly identifiable. We find that, generally, while the degree of asymmetry depends on the pump rate, the preferred direction for emission depends on the interatomic distance and the detuning of the probe field with respect to the resonant frequency. On physical grounds, for the case of frontal illumination, the asymmetry is the result of the interference of the photons emitted from different atoms. On the contrary, for side lighting, the asymmetry with respect to the side of incidence is caused by both the phase difference between the probe field photons that strike each atom and the interference between the photons emitted from different atoms. Further, for side lighting too, our quantum approach demonstrates that the forward scattered power depends on the side of incidence, which reveals the lack of reciprocity in the quantum optical response of the system. This result conflicts with what is obtained within a classical approach.
We study the scattering of light by a binary system of identical atoms in which one of them is incoherently pumped. This system belongs to the kind of non-parity symmetric optical systems in which gains and losses are partially compensated. We carry out a fully quantum analysis of the directionality of the radiation scattered from the atoms when the incident light strikes the system either perpendicular or alongside the interatomic axis. By resolving the emitted field in space, the microscopic mechanisms associated with photon exchange, interference, and reciprocity become directly identifiable. We find that, generally, while the degree of asymmetry depends on the pump rate, the preferred direction for emission depends on the interatomic distance and the detuning of the probe field with respect to the resonant frequency. On physical grounds, for the case of frontal illumination, the asymmetry is the result of the interference of the photons emitted from different atoms. On the contrary, for side lighting, the asymmetry with respect to the side of incidence is caused by both the phase difference between the probe field photons that strike each atom and the interference between the photons emitted from different atoms. Further, for side lighting too, our quantum approach demonstrates that the forward scattered power depends on the side of incidence, which reveals the lack of reciprocity in the quantum optical response of the system. This result conflicts with what is obtained within a classical approach.
We study the optical response of a binary system of identical atoms in which one of them is excited by an incoherent pump. Applying the diagrammatic formalism developed by Donaire [Phys. Rev. A 104, 043704 (2021)], we show how scattering, absorption, stimulated emission, spontaneous emission, and resonant energy transfer can be tailored by varying (1) the interatomic distance, which governs the interference effects of the emitted radiation, and (2) the pump rate, which determines the population of the atomic levels. It is found that, for sufficiently strong pumping, the collective component of the extinction cross section becomes negligible, regardless of the interatomic distance, as optical gains compensate for losses, and the total extinction cross section is reduced to less than half of its value in the absence of pumping. In contrast, at weak pumping and short interatomic distances, interference effects lead to a significant suppression of the extinction cross section relative to that of two noninteracting atoms.
Light scattered by a regular structure of atoms exhibits spatial interference signatures, similar to Young's classical double-slit experiment. The first-order interferences, however, are known to vanish for strong light intensities, where the incoherently fluctuating part of the emitted light dominates. Here, we show how to overcome these limitations to quantum interference in stronger laser fields, and how to recover the first-order interference in strong fields by a tailored electromagnetic vacuum with a suitable frequency dependence. We also discuss higher-order correlation functions of the scattered light, with applications, e.g., to lithography. In the second part, we study light propagation of a probe field pulse in closed-loop atomic systems. The closed interaction loop induces a sensitivity to the relative driving field phase, but in general prohibits a stationary steady state. In particular, the finite frequency width of the short probe pulse requires a time-dependent analysis beyond the so-called multiphoton resonance assumption. Using a Floquet decomposition, we identify the different contributions to the medium response, and demonstrate sub- and superluminal light propagation with small absorption or even gain, where a coupling field Rabi frequency allows to switch between sub- and superluminal light propagation.
We characterize the optical response of a three-level atom subjected to an incoherent pump and continuously illuminated with a weak quasiresonant probe field. To this end, we apply a wave-function approach based on QED Hamiltonian perturbation theory which allows for a reduction of the atomic dynamics to that of an effective two-level atom and for an implementation of the incoherent effects that respects unitarity. Using a diagrammatic representation, we identify and classify all the radiative processes. This allows us to compute the scattered power, the spontaneous emission, and the stimulated emission, as well as the total cross sections of extinction, absorption, and scattering. We find that, besides a general enhancement of the linewidth and an attenuation of the spectral amplitudes, the pump reduces the nonradiative losses and provides gains in the form of stimulated emission and incoherent radiation. For sufficiently strong pump, gains and losses compensate, resulting in the vanishing of extinction. In particular, for negligible nonradiative losses, extinction vanishes for a pumping rate of (1+5)/2 times that of the natural decay.
We study off-resonant collective light scattering from ultracold atoms trapped in an optical lattice. Scattering from different atomic quantum states creates different quantum states of the scattered light, which can be distinguished by measurements of the spatial intensity distribution, quadrature variances, photon statistics, or spectral measurements. In particular, angle-resolved intensity measurements reflect global statistics of atoms (total number of radiating atoms) as well as local statistical quantities (single-site statistics even without optical access to a single site) and pair correlations between different sites. As a striking example we consider scattering from transversally illuminated atoms into an optical cavity mode. For the Mott-insulator state, similar to classical diffraction, the number of photons scattered into a cavity is zero due to destructive interference, while for the superfluid state it is nonzero and proportional to the number of atoms. Moreover, we demonstrate that light scattering into a standing-wave cavity has a nontrivial angle dependence, including the appearance of narrow features at angles, where classical diffraction predicts zero. The measurement procedure corresponds to the quantum nondemolition measurement of various atomic variables by observing light.
In recent years, the radiative properties of atomic systems have been a hot topic in the research fields of quantum optics and quantum information. With the continuous development of nanophotonics, quantum antennas have become an important model for studying atomic radiation. In order to investigate these phenomena in depth, we investigate a system composed of two two-level atoms, and study the two-photon emission phenomenon of diatomic system under conditions of driving directional tunable laser field, interatomic dipole-dipole interaction, and spontaneous emission coherence. In this study, we diagonalize the atomic Hamiltonian to obtain the eigenvalues and entangled states of the system (symmetric and asymmetric states of two atoms), and use the rotating wave approximation to rotate the system into the laser frame. The evolution of the system is characterized mainly by the evolution of symmetric and asymmetric state, as well as the evolution of coherent terms. In our studies it is found that for identical atoms, certain laser directions and geometric configurations can exclusively drive the superradiant and subradiant states of atoms, which can enhance the first-order interference effect of the atoms and markedly increase the probability of two-photon emission in a specific detection direction. When the superradiant state of the atom is solely driven, there will be no coupling between the superradiant state and subradiant state, resulting in a correlation function angular distribution that is symmetric along the direction perpendicular to atomic axis. Further adjusting the laser direction causes the atomic interference patterns to shift, and the system will exhibit two-photon emission characteristics on one side or both sides. For nonidentical atomic systems, due to detuning between the two atoms, the laser cannot drive the superradiant state or subradiant state individually, and the influence of changing the laser direction on the coupling strength diminishes with the increase of detuning between the atoms. When the laser is in resonance with one of the atoms, due to the atomic interactions, the other atom can achieve the strongest coherent effect without resonating with the laser. This research reveals that atomic detuning is crucial for the correlation values and angular distribution of the correlation function. By adjusting the atomic detuning and laser direction, the system can display highly directed one-sided two-photon emission characteristics. However, different dissipation rates will lead the probability of two-photon emission to decrease. Our studies can achieve highly directional two-photon emission on one side or both sides, which provides a theoretical basis for studying the two-photon emission of nanoantennas.
Abstract The interaction of light with a single two-level emitter is the most fundamental process in quantum optics, and is key to many quantum applications. As a distinctive feature, two photons are never detected simultaneously in the light scattered by the emitter. This is commonly interpreted by saying that a single two-level quantum emitter can only absorb and emit single photons. However, it has been theoretically proposed that the photon anticorrelations can be thought of as arising from quantum interference between two possible two-photon scattering amplitudes, which one refers to as coherent and incoherent. This picture is in stark contrast to the aforementioned one, in that it assumes that the atom has two different mechanisms at its disposal to scatter two photons at the same time. Here we experimentally validate the interference picture by showing that, when spectrally rejecting only the coherent component of the fluorescence light of a single two-level atom, the remaining light consists of photon pairs that have been simultaneously scattered by the atom. Our results offer fundamental insights into the quantum-mechanical interaction between light and matter and open up novel approaches for the generation of highly non-classical light fields enabling, for example, Fourier-limited photon-pair sources that approach the theoretical limit in brightness.