Non-Gaussian quantum states of light are of paramount importance to quantum computing. Nevertheless, their deterministic generation is challenging problem due to the difficulty to control nonlinearities in physical systems. In this work, we characterize the light stemming from one of the most fundamental quantum optics configurations: the unidirectional scattering of multimode and multiphoton light by a two-level system. We provide an analytic and explicit description of the output light solely in terms of the corresponding input temporal modes which allows a straightforward physical interpretation and is computationally more effective compared to numerical methods. Then, we focus on the specific case of the scattering of two photons in a single mode. By numerically decomposing the output state in terms of its principal modes, we find that it is possible to map single-mode two-photon inputs to be into two-mode entangled output states, i.e., two-photon NOON states, to very good approximation. The latter states, in turn, are known to have more Wigner negativity compared to the associated input, which ultimately suggests a potential application of our considered setup in the deterministic generation of non-Gaussian states.
Non-Gaussian quantum states of light are of paramount importance to quantum computing. Nevertheless, their deterministic generation is challenging problem due to the difficulty to control nonlinearities in physical systems. In this work, we characterize the light stemming from one of the most fundamental quantum optics configurations: the unidirectional scattering of multimode and multiphoton light by a two-level system. We provide an analytic and explicit description of the output light solely in terms of the corresponding input temporal modes which allows a straightforward physical interpretation and is computationally more effective compared to numerical methods. Then, we focus on the specific case of the scattering of two photons in a single mode. By numerically decomposing the output state in terms of its principal modes, we find that it is possible to map single-mode two-photon inputs to be into two-mode entangled output states, i.e., two-photon NOON states, to very good approximation. The latter states, in turn, are known to have more Wigner negativity compared to the associated input, which ultimately suggests a potential application of our considered setup in the deterministic generation of non-Gaussian states.
Abstract We explore a recently demonstrated deterministic photon subtraction scheme, based on single-photon Raman interaction with a Λ-type three-level atom, as a tool for manipulating quantum state of few-photon light pulses. We establish a comprehensive theoretical framework using input–output formalism and quantum regression theorem, enabling calculation of the first order autocorrelation matrices of the output light and identification of the temporal modes present in the generated light via their eigendecomposition. By modeling the entire system as a quantum network consisting multiple virtual cavities and a lambda-type emitter cascaded in two parallel guided modes of opposite propagation directions, we extract the quantum state occupying the modes of interest. For both squeezed vacuum and coherent light input pulses, the Wigner function of the output light after photon subtraction clearly reveals its non-Gaussian character. Furthermore, we propose a measurement-based scheme on the subtracted photon which can lead to conditional generation of quantum states resembling Schrodinger’s kitten state directly from coherent input light with fidelities above 99%. This result is particularly nothworthy, as coherent pulses, unlike the squeezed vacuum inputs commonly used in previous studies, are readily available in most experimental setups.
The theoretical description of broadband, multimode quantum pulses undergoing a second-order χ(2)-nonlinear interaction can be quite intricate, due to the large dimensionality of the underlying phase space. However, in many cases only a few broadband (temporal) modes are relevant before and after the nonlinear interaction. Here we present an efficient framework to calculate the relation between the quantum states at the input and output of a nonlinear element in their respective relevant modes. Since the number of relevant input and output modes may differ, resulting in an open quantum system, we introduce the generalized Bloch-Messiah decomposition (GBMD), reducing the description to an equal number of input and output modes. The GBMD enables us to calculate the multimode Wigner function of the output state by convolving the rescaled Wigner function of the reduced input quantum pulse with a multivariate Gaussian phase-space function. We expand on this result by considering two examples input states: A Fock state in a single broadband mode and a two-mode squeezed vacuum, both in the THz-frequency regime, up-converted to a single output broadband mode of optical frequencies. We investigate the effect, the convolution and thermalization due to entanglement breakage have on the output Wigner function by calculating the von Neumann entropy of the output Wigner function. The methods presented here can be used to optimize the amplification or frequency conversion of broadband quantum states, opening an avenue to the generation and characterization of optical quantum states on ultrafast time scales.
We study theoretically how multiple scattering of light in a disordered medium can spontaneously generate quantum correlations. In particular we focus on the case where the input state is Gaussian and characterize the correlations between two arbitrary output modes. As there is not a single all-inclusive measure of correlation, we characterise the output correlations with three measures: intensity fluctuations, entanglement, and quantum discord. We find that, while a coherent input state can not produce quantum correlations, any other Gaussian input will produce them in one form or another. This includes input states that are usually regarded as more classical than coherent ones, such as thermal states, which will produce a non-zero quantum discord.
Quantum entanglement is a fascinating physical resource that is central to the field of quantum information processing with important applications in such areas as quantum computing, quantum communication, quantum metrology, and quantum imaging. \nIt describes the physical phenomenon in which the quantum state of a multipartite system cannot be written as consisting of constituents that are independent of each other. In this case, the state of the system is called an entangled state. In this \ndissertation, the entanglement of photons--the elementary excitations of the quantized electromagnetic field--is studied. A focus is made on a particular type of entangled states of light called the d-mode N-photon NOON state, which consists of N photons with the N photons as an ensemble appearing at d orthogonal modes simultaneously and are inseparable. \nIn quantum metrology, a field that investigates the ultimate precision of measurements of unknown physical parameters, the two-mode NOON state has been studied extensively with respect to its ability to achieve super-resolution and super-sensitivity in the estimation of a single parameter. A lot of theoretical research has been conducted on the generation of two-mode NOON states, and two-mode NOON states with up to 4 photons have been experimentally and efficiently produced. On the other hand, recently there has been increasing interest in the study of the simultaneous estimation of multiple parameters. Accordingly, the multi-mode NOON state has been attracting more and more attention in view of its potential for enhanced efficiency as compared to using multiple two-mode NOON states separately to estimate the parameters. Nevertheless, no known generation method of multi-mode NOON states with more than 2 photons or 2 modes exists so far. \nIn this dissertation, several scalable generation methods of multi-mode NOON states are proposed. These methods take advantage of multi-photon quantum interference and they can theoretically be applied to produce NOON states with an \narbitrary number of modes and an arbitrary number of photons. The intrinsic generation probability for each method is calculated, and the methods are compared in regards to their feasibility and efficiency. The advantages of using multi-mode NOON \nstates in quantum metrology are also analyzed and discussed in detail.
Harnessing entanglement and quantum coherence plays a central role in advancing quantum technologies. In quantum optical light-atom platforms, these two fundamental resources are often associated with a Jaynes-Cummings model description describing the coherent exchange of a photon between an optical resonator mode and a two-level spin. In a generic nonlinear spin-boson system, more photons and more modes will take part in the interactions. Here we consider such a generalization: the two-mode multiphoton Jaynes-Cummings (MPJC) model. We demonstrate how entanglement and quantum coherence can be optimally generated and subsequently manipulated in experimentally accessible parameter regimes. A detailed comparative analysis of this model reveals that nonlinearities within the MPJC interactions produce genuinely non-Gaussian entanglement, devoid of Gaussian contributions, from noisy resources. More specifically, strong coherent sources may be replaced by weaker, incoherent ones, significantly reducing the resource overhead, though at the expense of reduced efficiency. At the same time, increasing the multiphoton order of the MPJC interactions expedites the entanglement generation process, thus rendering the whole generation scheme again more efficient and robust. We further explore the use of additional dispersive spin-boson interactions and Kerr nonlinearities in order to create spin coherence solely from incoherent sources and to enhance the quantum correlations, respectively. As for the latter, somewhat unexpectedly, there is not necessarily an increase in quantum correlations due to the augmented nonlinearity. Towards possible applications of the MPJC model, we show how, with appropriately chosen experimental parameters, we can engineer arbitrary NOON states as well as the tripartite W state. Published by the American Physical Society 2024
We develop a new computational tool and framework for characterizing the scattering of photons by energy-nonconserving Hamiltonians into unidirectional (chiral) waveguides, for example, with coherent pulsed excitation. The temporal waveguide modes are a natural basis for characterizing scattering in quantum optics, and afford a powerful technique based on a coarse discretization of time. This overcomes limitations imposed by singularities in the waveguide-system coupling. Moreover, the integrated discretized equations can be faithfully converted to a continuous-time result by taking the appropriate limit. This approach provides a complete solution to the scattered photon field in the waveguide, and can also be used to track system-waveguide entanglement during evolution. We further develop a direct connection between quantum measurement theory and evolution of the scattered field, demonstrating the correspondence between quantum trajectories and the scattered photon state. Our method is most applicable when the number of photons scattered is known to be small, i.e. for a single-photon or photon-pair source. We illustrate two examples: analytical solutions for short laser pulses scattering off a two-level system and numerically exact solutions for short laser pulses scattering off a spontaneous parametric downconversion (SPDC) or spontaneous four-wave mixing (SFWM) source. Finally, we note that our technique can easily be extended to systems with multiple ground states and generalized scattering problems with both finite photon number input and coherent state drive, potentially enhancing the understanding of, e.g., light-matter entanglement and photon phase gates.