We theoretically investigate the response of a coherently-driven nonlinear optical cavity to an additional incident single photon. Using a quantum description of the nonlinear dynamics that fully accounts for the quantum fluctuations of the cavity field and for the discrete nature of the incident photon, we characterize the quantum dynamics of single-photon-stimulated jumps from the low-photon-number to the high-photon-number state of the optical bistability loop. We find that the system can exhibit a giant response to this single quantum of excitation, rooted in the phase-transition picture of optical bistability. In addition to shedding light on the role of quantum fluctuations in the non-equilibrium dynamics of a nonlinear optical cavity, our results suggest a strategy for an all-optical single-photon avalanche detector.
We theoretically investigate the response of a coherently-driven nonlinear optical cavity to an additional incident single photon. Using a quantum description of the nonlinear dynamics that fully accounts for the quantum fluctuations of the cavity field and for the discrete nature of the incident photon, we characterize the quantum dynamics of single-photon-stimulated jumps from the low-photon-number to the high-photon-number state of the optical bistability loop. We find that the system can exhibit a giant response to this single quantum of excitation, rooted in the phase-transition picture of optical bistability. In addition to shedding light on the role of quantum fluctuations in the non-equilibrium dynamics of a nonlinear optical cavity, our results suggest a strategy for an all-optical single-photon avalanche detector.
Observing non-classical properties of light is a long-standing interest to advance a wide range of quantum applications. Optical cavities are essential to generate and manipulate non-classical light. However, detecting changes in cavity properties induced by the quantum state remains a critical challenge in the optical domain due to the weak material nonlinearity. Here, we propose a framework for observing the dynamics of quantum states generated inside nonlinear optical cavities. We leverage the symmetry-breaking process of a bistable system, which is highly sensitive to the initial state, enabling detection of quantum state displacement through an asymmetric equilibrium of a macroscopic observable. With a nonlinear response at the single photon level, our approach directly imprints the cavity field distribution onto the statistics of bistable cavity steady-states. We experimentally demonstrate our approach in a degenerate optical parametric oscillator, generating and reconstructing different quantum states. As a validation, we reconstruct the Husimi Q function of the cavity squeezed vacuum state. In addition, we observe the evolution of the quantum vacuum state inside the cavity as it undergoes phase-sensitive amplification. By enabling generation and measurement of quantum states in a single nonlinear optical cavity, our method paves a way for studying exotic dynamics of quantum optical states in nonlinear driven-dissipative systems. Characterising an optical quantum state confined in a cavity is not an easy task, as standard tomographic techniques works by interfering propagating fields and therefore encounters the problems relative to outcoupling the state. Here, the authors fill this gap for states generated within a nonlinear cavity featuring multiple steady states.
Abstract We study the nonequilibrium dynamic behaviors in a driven-dissipative single-atom cavity electromagnetically induced transparency. The optical bistability and multistability beyond a Kerr nonlinearity are observed utilizing the optical Stark shift induced strong nonlinearity. We show that the nonequilibrium dynamical phase transition between bistability and multistability is highly tunable by the system parameters in a large parameter region. The first-order dissipative optical bistability (multistability) always corresponds to the photon-bunching quantum statistics, which indicates that the quantum fluctuations and correlations play important roles in nonequilibrium dynamics. Interestingly, bistability and multistability with photon-bunching quantum statistics occurring at extremely low steady-state cavity photon number are observed, even under a very strong cavity driven field. Furthermore, we demonstrate that the unique cavity steady-state solution of the full quantum calculation is excellently consistent with the lowest solution based on the semiclassical mean-field approach in bistability and multistability regimes when the cavity photon number is much less than unity, albeit these nonclassical quantum states should possess strong quantum fluctuations in this parameter regime. Our results pave the way to exploring nonclassical correlated optical multistability in quantum regime, which may bring exciting opportunities for potential applications from quantum information processing to quantum metrology.
We give a microscopic description of the optical bistability, where the transmission coefficient has two different values as a function of input light intensity, and the system exhibits a discontinuous jump with a hysteresis loop. We developed an efficient numerical algorithm to treat the quantum master equation for hybridized systems of many photons and a large number of two-level atoms. By using this method, we characterize the bistability from the viewpoint of eigenmodes and eigenvalues of the time-evolution operator of the quantum master equation. We classify types of optical bistability according to the photon number density in the cavity. In contrast to previous studies of optical bistability in the high-photon-density regime where the photons can be treated as a classical electromagnetic field and the resonance spectrum has a single-peak structure, we study the nature of optical bistability in the low-photon-density regime where the hybridization of photon and atom degrees of freedom occurs and the resonance spectrum has a double-peak structure. Unraveling the nature of the optical bistability in the latter regime may be important for the manipulation of quantum systems. Concretely, we discuss the steady-state properties of the optical bistability: dependencies of the photon number density on the intensity and the double-peak structure of the photon number distribution inside the bistable region. As for the dynamical properties, we find that the relaxation timescale shows an exponential growth with the system size and reveal how the hysteresis loop of the optical bistability depends on the size of the system and the sweeping rate of the driving amplitude. Finally, by investigating the effects of detuning frequency of the input field, we clarify the characteristic properties of the present optical bistability within the low-photon-density regime, which are qualitatively different from the standard optical bistable phenomena.
Abstract Observing non-classical properties of light is a long-standing interest to advance a wide range of quantum application from computing to metrology. Optical cavities are essential to generate and manipulate non-classical light. However, detecting changes in cavity properties induced by the quantum state remains a critical challenge in the optical domain due to the weak material nonlinearity, limiting our ability to observe quantum states generated in optical cavities. Here, we propose a framework for observing the dynamics of quantum states generated inside nonlinear optical cavities. We utilize symmetry-breaking to obtain high sensitivity to small perturbations introduced to the quantum state, resulting in an asymmetric equilibrium of a macroscopic observable. With a nonlinear response at the single photon level, our approach directly imprints the field distribution of the cavity quantum state onto the statistics of bistable cavity steady-states. We experimentally demonstrate our approach in a degenerate optical parametric oscillator, generating and reconstructing the quasi-probability distribution of different quantum states. As a validation, we reconstruct the Husimi Q function of the cavity squeezed vacuum state. In addition, we observe the evolution of the quantum vacuum state inside the cavity as it undergoes phase-sensitive amplification. By enabling generation and measurement of quantum states in a single nonlinear optical cavity, our method paves a way for studying exotic dynamics of quantum optical states in nonlinear driven-dissipative systems such as soliton generation and Kerr frequency combs.
We theoretically investigated the bistability in a small Fabry-Perot interferometer (FPI) with the optical wavelength size cavity, the nonlinear Kerr medium, and only a few photons, on average, excited by the external quantum field. Analytical expressions for the stationary mean photon number, the bistability domain, the field, and the photon number fluctuation spectra are obtained. Multiple stationary states of the FPI cavity field with different spectra are possible at realistic conditions, for example, in the FPI with the photonic crystal cavity and the semiconductor-doped glass nonlinear medium.
A quantum treatment of a coherently driven dispersive cavity is given based on a cubic nonlinearity in the polarisability of the internal medium. This system displays bistability and hysteresis in the semiclassical solutions. Quantum fluctuations are included via a Fokker-Planck equation in a generalised P representation. The transmitted light shows a transition from a single-peaked spectrum to a double-peaked spectrum above the threshold of the lower branch. Fluctuations in the field are reduced on the upper branch and both photon bunching and photon antibunching are predicted, for different operating points. An exact solution obtained for the steady-state generalised P function shows decidedly non-equilibrium behaviour, e.g. the lack of a Maxwell construction.