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arXiv:2606.26081

Folds of one curve: the superradiant phase diagram of Dicke modes with interacting matter

Max Hörmann

cond-mat.str-elcond-mat.stat-mechquant-phSubmitted Jun 24, 2026• Announced Jun 25, 2026• 0 citations
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Abstract

We give a thermodynamic-limit account of Dicke models with one cavity mode coupled collectively to interacting matter. Integrating out the cavity yields an exact self-consistent functional of the magnetisation $m$, $\tilde e(m) = λm^2/2 + e_{\rm mat}(λm)$: a classical penalty on the bare-matter energy $e_{\rm mat}$ in the self-consistent field $h = λm$, with $λ= g^2/(2ω_c)$ the collective coupling. Supplying only that scalar field, the photon creates no phase the matter does not already possess. States holding a minimum form one connected curve, $λ(m) = μ_{\rm mat}^{-1}(m)/m$, so superradiant first-order transitions are folds of one equation of state not crossings of disjoint sheets, and a fold can straighten into a continuous line. The remaining rules are local, each with a spectral counterpart: onset by the leading singularity of $e_{\rm mat}$ (a softening polariton), order by one bare response -- the Landau quartic, or a divergent susceptibility forcing a Larkin-Pikin (LP) fold. For the Dicke-Ising model the Landau coefficients are exact, giving in closed form the second-order boundary and both zero-quartic fields, one tricritical; a $1/d$ expansion maps all four phases, with the AS-PS transition first order for $d\le d_{uc}=3=4-z$ (LP) and tricritical points in the $(d,ε)$ plane above. At the degenerate quadruple point the matter is a Rydberg-blockade chain, solved by strict-blockade iDMRG: the antiferromagnetic superradiant (AS) phase persists as a finite 1D wedge, first order into the corner. Other magnets: the triangular antiferromagnet keeps a continuous superradiant-superradiant line (3D-XY, no fold forced); the compass chain a BKT-functional onset; the Heisenberg and XX chains, via a conserved operator, a spectrally silent first-order onset; and the Dicke-Heisenberg diagram an exact tricritical point at the saturation corner.

Comments
111 pages, 20 figures

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We give a thermodynamic-limit account of Dicke models with one cavity mode coupled collectively to interacting matter. Integrating out the cavity yields an exact self-consistent functional of the magnetisation mmm, e~(m)=λm2/2+emat(λm)\tilde e(m) = λm^2/2 + e_{\rm mat}(λm)e~(m)=λm2/2+emat​(λm): a classical penalty on the bare-matter energy emate_{\rm mat}emat​ in the self-consistent field h=λmh = λmh=λm, with λ=g2/(2ωc)λ= g^2/(2ω_c)λ=g2/(2ωc​) the collective coupling. Supplying only that scalar field, the photon creates no phase the matter does not already possess. States holding a minimum form one connected curve, λ(m)=μmat−1(m)/mλ(m) = μ_{\rm mat}^{-1}(m)/mλ(m)=μmat−1​(m)/m, so superradiant first-order transitions are folds of one equation of state not crossings of disjoint sheets, and a fold can straighten into a continuous line. The remaining rules are local, each with a spectral counterpart: onset by the leading singularity of emate_{\rm mat}emat​ (a softening polariton), order by one bare response -- the Landau quartic, or a divergent susceptibility forcing a Larkin-Pikin (LP) fold. For the Dicke-Ising model the Landau coefficients are exact, giving in closed form the second-order boundary and both zero-quartic fields, one tricritical; a 1/d1/d1/d expansion maps all four phases, with the AS-PS transition first order for d≤duc=3=4−zd\le d_{uc}=3=4-zd≤duc​=3=4−z (LP) and tricritical points in the (d,ε)(d,ε)(d,ε) plane above. At the degenerate quadruple point the matter is a Rydberg-blockade chain, solved by strict-blockade iDMRG: the antiferromagnetic superradiant (AS) phase persists as a finite 1D wedge, first order into the corner. Other magnets: the triangular antiferromagnet keeps a continuous superradiant-superradiant line (3D-XY, no fold forced); the compass chain a BKT-functional onset; the Heisenberg and XX chains, via a conserved operator, a spectrally silent first-order onset; and the Dicke-Heisenberg diagram an exact tricritical point at the saturation corner.
In the thermodynamic limit, the Dicke-Ising chain maps exactly onto an effective self-consistent matter Hamiltonian with the photon field acting solely as a self-consistent effective field. As a consequence, no quantum correlations between photons and spins are needed to understand the quantum phase diagram. This enables us to determine the quantum phase diagram in the thermodynamic limit using numerical linked-cluster expansions combined with density matrix renormalization group calculations (NLCE+DMRG) to solve the resulting self-consistent matter Hamiltonian. This includes magnetically ordered phases with significantly improved accuracy compared to previous estimates. For ferromagnetic Ising couplings, we refine the location of the multicritical point governing the change in the order of the superradiant phase transition, reaching a relative accuracy of 10−410^{-4}10−4. For antiferromagnetic Ising couplings, we confirm the existence of the narrow antiferromagnetic superradiant phase in the thermodynamic limit. The effective matter Hamiltonian framework identifies the antiferromagnetic superradiant phase as the many-body ground state of an antiferromagnetic transverse-field Ising model with longitudinal field. This phase emerges through continuous Dicke-type polariton condensation from the antiferromagnetic normal phase, followed by a first-order transition to the paramagnetic superradiant phase. Thus, NLCE+DMRG provides a precise determination of the Dicke-Ising phase diagram in one dimension by solving the self-consistent effective matter Hamiltonian.
We gain quantitative insights on effects of light-matter interactions on correlated quantum matter by quantum Monte Carlo simulations. We introduce a wormhole algorithm for the paradigmatic Dicke-Ising model which combines the light-matter interaction of the Dicke model with Ising interactions. The quantum phase diagrams for ferro- and antiferromagnetic interactions on the chain and the square lattice are determined. The occurring superradiant phase transitions are in the same universality class as the Dicke model, leading to a well-known peculiar finite-size scaling that we elucidate in terms of scaling above the upper critical dimension. For the ferromagnetic case, the transition between the normal and the superradiant phase is of second order with Dicke criticality (first order) for large (small) longitudinal fields separated by a multicritical point. For antiferromagnetic interactions, we establish the light-matter analog of a lattice supersolid with off-diagonal superradiant and diagonal magnetic order and determine the nature of all transition lines. Our achievements allow to quantitatively enter the domain of mesoscopic light-matter systems, which is an increasingly prominent topic at the interface of quantum optics and condensed matter physics.
In this doctoral thesis, the thermodynamic phases und phase transitions of a generalised Dicke model are studied and characterised. Both, finite and vanishing temperatures are considered. The Dicke model of quantum optics describes collective phenomena which occur when light interacts with a many-atom system. In the thermodynamic limit, a so-called Hepp–Lieb superradiant phase transition sets in. A superradiant phase develops for low temperatures or strong coupling between light and atoms, which is characterised by a macroscopic excitation of the light field and a spontaneous, collective polarisation of the atoms. This thesis discusses a generalised version of the Dicke model, which is described by a quantum mechanical system consisting of three-level atoms in Lambda-configuration and two modes of a resonator. By means of the Holstein–Primakoff transformation, the Hamiltonian of this system is written in terms of four interacting, non-linear oscillators, which can be linearised in the thermodynamic limit, yielding the ground-state energy as well as the low-energy excitations. The phase diagram consisting of two superradiant phases separated by continuous and first-order phase transitions is derived. In order to clarify the question whether or not the superradiant phase transition of this generalised Dicke model can be observed experimentally for real atoms, the significance of the diamagnetic term is discussed. In contrast to the original Dicke model, superradiant phase transitions are possible in principle. This is due to the first-order phase transitions. In addition, a no-go theorem for continuous superradiant phase transitions is presented. The argument is based on the Thomas–Reiche–Kuhn sum rule. Last, we study the superradiant phase transition of the generalised Dicke model at finite temperatures. Therefore, the partition sum is computed and analysed in the thermodynamic limit using Laplace’s method. At finite temperatures, the properties of the phase diagram and phases remain. However, here all phase transitions are of first order.
We present quantum phase diagrams for the antiferromagnetic long-range Ising model with a linear coupling to a single bosonic mode on the square and triangular lattice. For zero coupling, the ground-state magnetization forms a devil's staircase structure of magnetization plateaux as a function of a longitudinal field. Apart from a paramagnetic superradiant phase with a finite photon density at strong light-matter couplings, the long-range interactions lead to a plethora of intermediate phases that break the translational symmetry and have a finite photon density at the same time. We apply an adaption of the unit-cell-based mean-field calculations, which captures all possible magnetic unit cells up to a chosen extent. Further, we exploit an exact mapping of the non-superradiant phases to an effective Dicke model to calculate upper bounds for phase transitions towards superradiant phases. Finally, to treat quantum fluctuations in a quantitative fashion, we employ a generalized wormhole quantum Monte Carlo algorithm. We discuss how these three methods are used in a cooperative fashion. In the calculated phase diagrams we see several features arising from the long-range interactions: The devil's staircases of distinct magnetically ordered normal phases and non-trivial magnetically ordered superradiant phases beyond the findings for nearest-neighbor interactions. Examples are a superradiant phase with a three-sublattice magnetic order on the square lattice and the superradiant Wigner crystal with four sites per unit cell on the triangular lattice. We find the transition between normal and superradiant phases with the same (different) magnetic order to be of second order with Dicke universality (first order). Further, between superradiant phases we find first-order phase transitions, besides specially highlighted regimes for which we find indications for second-order behavior.
Light-matter interacting systems involving multilevel atoms are appealing platforms for testing equilibrium and dynamical phenomena. Here we explore a tricritical Dicke model, where an ensemble of three-level systems interacts with a single light mode, through two different approaches: a generalized Holstein-Primakoff mapping and a treatment using the Gell-Mann matrices. Both methods are found to be equivalent in the thermodynamic limit. In equilibrium, the system exhibits a rich phase diagram where both continuous and discrete symmetries can be spontaneously broken. We characterize all the different types of symmetries according to their scaling behaviors. Far from the thermodynamic limit, considering just a few tens of atoms, the system already exhibits features that could help characterize both second- and first-order transitions in a potential experiment. Importantly, we show that the tricritical behavior is preserved when dissipation is taken into account. Moreover, the system develops a rich steady-state phase diagram with various regions of bistability, all of them converging at the tricritical point. Having multiple stable normal and superradiant phases opens prospective avenues for engineering interesting steady states by a proper choice of initial states and/or parameter quenching.
The superradiant phenomenon, usually described by the Dicke model, is a hallmark of strong light-matter interaction. We explore how matter-matter interactions influence this phenomenon by performing ground-state simulations of Dicke-like models with both isotropic and anisotropic interactions. We find that Ising-type interactions produce two qualitatively distinct phase boundaries, one of which gives rise to an antiferromagnetic-normal phase connected to the superradiant regime via a first-order phase transition. Under anisotropic couplings, we uncover a strongly correlated phase where in-plane spin order coexists with superradiance, exhibiting sublinear scaling of the photon occupation per site and power-law decay of spin correlations. Furthermore, superradiance is strengthened by tuning either isotropic or anisotropic interactions, highlighting the role of intrinsic many-body correlations in shaping light-matter quantum phases.