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arXiv:2606.22292

Probing Single-Particle Spatial Extent With Helical Neutron Wavefronts

D. Sarenac, O. Lailey, C. W. Clark, D. G. Cory, H. Ekinci, D. V. Garrad, M. G. Huber, L. Matthews, N. Shentevski, P. R. Vadnere, D. A. Pushin

quant-phSubmitted Jun 21, 2026• Announced Jun 23, 2026• 0 citations
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Abstract

Distinguishing transverse coherence length from single-particle wavepacket extent is fundamentally challenging, as both manifest through spatial broadening of observed intensity profiles in conventional experiments. Here we introduce a method based on helical neutron wavefronts that enables this separation. Helical neutron states produce annular intensity profiles whose peak radius depends on the transverse wavepacket extent, while coherence length only contributes to profile broadening. In our experimental geometry we measure a beam divergence of ~1.1 mrad, corresponding to a transverse coherence length of ~180 nm. In contrast, the same measurement places a lower bound of >= 2 um on the spatial extent of the individual neutron wavepackets, more than an order of magnitude larger than the coherence length. These results provide direct experimental evidence that transverse coherence length and single-particle wavepacket extent are distinct physical quantities, resolving a longstanding source of confusion in the neutron literature.

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Distinguishing transverse coherence length from single-particle wavepacket extent is fundamentally challenging, as both manifest through spatial broadening of observed intensity profiles in conventional experiments. Here we introduce a method based on helical neutron wavefronts that enables this separation. Helical neutron states produce annular intensity profiles whose peak radius depends on the transverse wavepacket extent, while coherence length only contributes to profile broadening. In our experimental geometry we measure a beam divergence of ~1.1 mrad, corresponding to a transverse coherence length of ~180 nm. In contrast, the same measurement places a lower bound of >= 2 um on the spatial extent of the individual neutron wavepackets, more than an order of magnitude larger than the coherence length. These results provide direct experimental evidence that transverse coherence length and single-particle wavepacket extent are distinct physical quantities, resolving a longstanding source of confusion in the neutron literature.
In the analysis of neutron scattering measurements of condensed matter structure, it normally suffices to treat the incident and scattered neutron beams as if composed of incoherent distributions of plane waves with wavevectors of different magnitudes and directions which are taken to define an instrumental resolution. However, despite the wide-ranging applicability of this conventional treatment, there are cases in which the wave function of an individual neutron in the beam must be described more accurately by a spatially localized packet, in particular with respect to its transverse extent normal to its mean direction of propagation. One such case involves the creation of orbital angular momentum (OAM) states in a neutron via interaction with a material device of a given size. It is shown in the work reported here that there exist two distinct measures of coherence of special significance and utility for describing neutron beams in scattering studies of materials in general. One measure corresponds to the coherent superposition of basis functions and their wavevectors which constitute each individual neutron packet state function whereas the other measure can be associated with an incoherent distribution of mean wavevectors of the individual neutron packets in a beam. Both the distribution of the mean wavevectors of individual packets in the beam as well as the wavevector components of the superposition of basis functions within an individual packet can contribute to the conventional notion of instrumental resolution. However, it is the transverse spatial extent of packet wavefronts alone that determines the area within which a coherent scattering process can occur in the first place. This picture is shown to be consistent with standard quantum theory. It is also demonstrated that these two measures of coherence can be distinguished from one another experimentally.
The development of direct probes of entanglement is integral to the rapidly expanding field of complex quantum materials.Here we test the robustness of entangled neutrons as a quantum probe by measuring the Clauser-Horne-Shimony-Holt contextuality witness while varying the beam properties.Specifically, we show that the mode entanglement of the spin and path subsystems of individual neutrons prepared in two different experiments using two different apparatuses persists even after varying the entanglement length, coherence length, and neutron energy difference of the paths.The two independent apparatuses acting as entangler-disentangler pairs are static-field magnetic Wollaston prisms and resonance-field radio-frequency flippers.Our results show that the spatial and energy properties of the neutron beam may be significantly altered without reducing the contextuality witness value below the Tsirelson bound, meaning that maximum entanglement is preserved.We also show that two paths may be considered distinguishable even when the path states significantly overlap.Therefore, we have shown that our experimental results are consistent with the distinguishable subsystem assumption down to a separation of less than 100 nm, proving entanglement and the contextual nature of reality on short length scales.This work is the key step in the realization of the modular, robust technique of entangled neutron scattering, which can extract entanglement information from a sample without the knowledge of the microscopic sample Hamiltonian: only semiquantitative knowledge of the correlation lengths of the relevant degrees of freedom and the timescales of the characteristic dynamics is required.
In the experiment described in this paper, a chopper serves as a source of neutron intensity pulses which pass through a perfect Si-crystal neutron interferometer (NI), where they are split coherently into two parts that recombine and interfere. As the occupation number of a single pulse is much smaller than unity, the results very clearly demonstrate the single-particle interference phenomena of neutron interferometry experiments. While traveling the pulses spread, with faster (slower) neutrons tending toward the leading (trailing) edge. The coherence length of the neutrons depends on the spectral width of their wavelength distribution. When a material with a neutron-nuclear optical potential is placed in one beam path in the NI, there is a loss of fringe visibility (contrast), which depends on the coherence length. By using time-of-flight techniques, we divide the pulse into time segments. Within a given time slice, the wavelength spectrum is narrower than in the pulse as a whole. As a result, contrast remains in the time slices even when it disappears in the overall pulse. We also observe an additional contrast modulation due to the overlap of neighboring pulses.
We point out that many wavepacket discussions for the coherence properties of particle beams are unnecessary since they deal with stationary sources; and when the problem is stationary, essentially all information is in the energy spectrum. This recognition allows a simple answer to a number of long-debated points, usually framed in terms of the``length of the wavepacket.'' In particular we discuss neutrino oscillations, and some issues in neutron physics. The question as to whether two simple beams with the same energy spectrum are distinguishable is answered negatively for stationary situations. The question as to whether neutrino oscillations should be thought of as taking place between states of the same energy or the same momentum is answered in favor of energy for stationary situations. The consequences for proposals involving the 7Be{}^{7}\mathrm{Be}7Be neutrino line of the Sun, the observation of oscillations in supernova neutrinos, and wavepacket studies with neutrons are briefly discussed, as well as the connection with the coherence notions of quantum optics.
Neutrons are important probes of mater and quantum physics. They are particularly powerful at characterizing magnetic structures. In order to extend the applications of neutron physics as a quantum probes/sensors we have developed methods based on Quantum Information Processing for preparing structured waves such as orbital and spin-orbit states of neutrons. Such states may be prepared for the beam as a whole, or with reference to the coherence length of the neutron wavepacket, which is much smaller than the width of useful beams. I will describe experiments to prepare and characterize neutron beams with specific orbital and spin-orbit structure based on neutron interferometry and will show how we can apply these methods to other type of probes such as light.