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arXiv:2606.00165

Chirality routing non-polaritonic vacuum correlations in Landau polaritons

Ayoub EL-Amrani, Zakaria Mzaouali, Houssam Sabri, Herschel Rabitz, Abdelouahed El Fatimy, Dukhyung Lee

cond-mat.mes-hallquant-phSubmitted May 29, 2026• Announced Jun 1, 2026• Revised Jun 2, 2026 (v2)
v1 · May 29, 2026v2 · Jun 2, 2026
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Abstract

Ultrastrong coupling between matter and cavity vacuum fields can turn the electromagnetic vacuum into a structured quantum environment, thereby opening passive routes for modifying and manipulating material properties. Recent work has identified light--matter entanglement as an important ingredient in these property changes, which raises the question of where the relevant vacuum correlations actually reside. Landau polaritons provide chiral ultrastrong coupling systems in which one circular cavity polarization forms the bright polariton branches. Here, using a quantum information approach, we show that an exact chiral charge in a multimode Hopfield model routes the dominant anomalous correlations, squeezing, and cavity--matter entanglement into the opposite polarization. We find that, using parameters extracted from a multimode Landau polariton system, this hidden sector correlates the cyclotron resonance with finite momentum magnetoplasmons through Gaussian discord, while pairwise matter--matter entanglement remains absent. We further predict a polarization anisotropy of dressed vacuum electric field fluctuations as a signature of this chiral routing. These results identify chirality as a symmetry principle for organizing ultrastrong coupling vacua and show that quantum information tools provide a powerful framework for revealing the salient properties of Landau polaritons.

Comments
20 pages, 13 figures

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Ultrastrong coupling between matter and cavity vacuum fields can turn the electromagnetic vacuum into a structured quantum environment, thereby opening passive routes for modifying and manipulating material properties. Recent work has identified light--matter entanglement as an important ingredient in these property changes, which raises the question of where the relevant vacuum correlations actually reside. Landau polaritons provide chiral ultrastrong coupling systems in which one circular cavity polarization forms the bright polariton branches. Here, using a quantum information approach, we show that an exact chiral charge in a multimode Hopfield model routes the dominant anomalous correlations, squeezing, and cavity--matter entanglement into the opposite polarization. We find that, using parameters extracted from a multimode Landau polariton system, this hidden sector correlates the cyclotron resonance with finite momentum magnetoplasmons through Gaussian discord, while pairwise matter--matter entanglement remains absent. We further predict a polarization anisotropy of dressed vacuum electric field fluctuations as a signature of this chiral routing. These results identify chirality as a symmetry principle for organizing ultrastrong coupling vacua and show that quantum information tools provide a powerful framework for revealing the salient properties of Landau polaritons.
Polariton formation and quantum vacuum dressing are usually regarded as intertwined consequences of ultrastrong light--matter coupling. Here we show that they can be selectively controlled through the relative direction of rotation of the cavity field and the matter excitation. We consider cyclotron resonance coupled to a chiral cavity supporting a single circularly polarized mode. We quantize the electromagnetic field within the cavity, derive from first principles the Hamiltonian, and investigate how mode hybridization and vacuum dressing are rendered as we tune the magnetic field. When the cavity field co-rotates with the cyclotron motion, energy is exchanged resonantly between light and matter, producing a large Rabi splitting and conventional polaritons, while the ground state remains the bare vacuum. Reversing the magnetic field makes the cyclotron motion counter-rotating with the cavity field. The same cavity mode then couples through anomalous processes that create and annihilate light and matter excitations in pairs: the conventional polaritonic anticrossing disappears, while the ground state acquires squeezing and virtual excitations. Our results show that spectral hybridization and quantum vacuum dressing are distinct manifestations of ultrastrong coupling, offering an additional degree of freedom for engineering cavity quantum materials.
We reveal that a chiral cavity distinguishes the resonant and antiresonant interactions between a two-dimensional electron gas and the cavity vacuum. For co-rotating helicities, the modes anticross, exhibiting vacuum Rabi splitting, and retain a bare vacuum ground state. For counter-rotating helicities, the modes cross, acquiring vacuum-mediated energy shifts and a two-mode squeezed ground state. We trace the origin of these observations to the SU(2) and SU(1,1) symmetries of the respective Hamiltonians and present their spectroscopic signatures in chiral photonic crystal cavities. We further predict that cavity chirality produces a handedness-dependent correction to Hall resistivity at finite polariton broadening, while such a correction is not present in an achiral cavity. For the longitudinal resistivity, we find an asymmetric response of the Shubnikov--de Haas oscillations for the different helicities. Finally, we present an experimentally accessible route for detecting the squeezed ground state through current fluctuations. Parameters based on a recently demonstrated terahertz chiral cavity place these effects within experimental reach.
Dressing quantum states of matter with virtual photons can create exotic effects ranging from vacuum-field modified transport to polaritonic chemistry, and may drive strong squeezing or entanglement of light and matter modes. The established paradigm of cavity quantum electrodynamics focuses on resonant light-matter interaction to maximize the coupling strength ΩR/ωcΩ_\mathrm{R}/ω_\mathrm{c}ΩR​/ωc​, defined as the ratio of the vacuum Rabi frequency and the carrier frequency of light. Yet, the finite oscillator strength of a single electronic excitation sets a natural limit to ΩR/ωcΩ_\mathrm{R}/ω_\mathrm{c}ΩR​/ωc​. Here, we demonstrate a new regime of record-strong light-matter interaction which exploits the cooperative dipole moments of multiple, highly non-resonant magnetoplasmon modes specifically tailored by our metasurface. This multi-mode coupling creates an ultrabroadband spectrum of over 20 polaritons spanning 6 optical octaves, vacuum ground state populations exceeding 1 virtual excitation quantum for electronic and optical modes, and record coupling strengths equivalent to ΩR/ωc=3.19Ω_\mathrm{R}/ω_\mathrm{c}=3.19ΩR​/ωc​=3.19. The extreme interaction drives strongly subcycle exchange of vacuum energy between multiple bosonic modes akin to high-order nonlinearities otherwise reserved to strong-field physics, and entangles previously orthogonal electronic excitations solely via vacuum fluctuations of the common cavity mode. This offers avenues towards tailoring phase transitions by coupling otherwise non-interacting modes, merely by shaping the dielectric environment.
The quantum Hopfield model is widely used to describe ultrastrong light--matter coupling between cavity photons and collective bosonic excitations in solids, where the diamagnetic interaction is conventionally assumed to be a constant. We experimentally demonstrate that the diamagnetic response of Landau polaritons is reduced under strong terahertz field excitation. We show that this behavior originates from field-driven redistribution of electrons into the nonparabolic regime of the conduction band of GaAs, which reduces the plasma frequency and consequently the diamagnetic interaction strength. A microscopic hot-electron model reproduces the observed nonlinear response. Motivated by this microscopic picture, we propose a nonlinear extension of the Hopfield model with a Kerr-like interaction. Our results establish a route toward nonlinear cavity quantum electrodynamics and driven ultrastrong light--matter coupling beyond the conventional linear Hopfield description, which is capable of creating uniquely quantum optical effects such as squeezed light generation.
By forming hybrid light-matter states, optical cavities offer a route for engineering material properties, however, unambiguously probing the effects of light-matter coupling remains difficult. Here, we show that the polarization-resolved statistics of photons transmitted through a cavity, measurable via g(2)g^{(2)}g(2), provide one such diagnostic. By relating g(2)g^{(2)}g(2) to matter correlation functions such as the Raman structure factor, we link photon bunching and antibunching to material properties. By applying this method to the stripy-to-antiferromagnetic transition in the Kitaev-Heisenberg spin model, we find that polarization-dependent patterns of bunching and antibunching encode the magnetic point-group symmetries of each phase and characterize the behavior at the phase boundary. Finally, we predict measuring g(2)g^{(2)}g(2) for output photon pairs polarized orthogonal to the input field will isolate higher-order light-matter scattering processes that probe higher-order material correlations.
I introduce and analyze chiral light-matter interaction in the ultrastrong coupling limit where the rotating-wave approximation cannot be made. Within this limit, a two-level system with a circularly polarized transition dipole interacts with a copolarized mode through rotating-wave terms. However, the counterrotating terms allow the two-level system to couple to a counterpolarized mode with the same coupling strength, i.e., one that is completely decoupled within the rotating-wave approximation. Although such a Hamiltonian is not particle number conserving, the conservation of angular momentum generates a U(1) symmetry which allows constructing an ansatz. The eigenstates and dynamics of this novel model are computed for single-cavity interactions and for a many-mode system. The form of the ansatz provides significant analytic insight into the physics of the ground state and the dynamics; e.g., it indicates that the ground states are two-mode squeezed. This work has significant implications for engineering light-matter interaction and novel quantum many-body dynamics beyond the rotating-wave approximation.