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arXiv:2605.14100

Effective Hamiltonians in Cavity and Waveguide QED from Transition-Operator Diagrammatic Perturbation Theory

Mohamed Meguebel, Maxime Federico, Louis Garbe, Nadia Belabas, Nicolas Fabre

quant-phSubmitted May 13, 2026• Announced May 15, 2026• 0 citations• Revised Jul 10, 2026 (v2)
v1 · May 13, 2026v2 · Jul 10, 2026
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Abstract

We propose an adiabatic-elimination formalism in the dispersive regime based on a transition-centric perturbation theory. The perturbative expansion is recast into a diagrammatic framework, while adiabatic elimination is implemented through controlled projections onto transition subspaces. Our approach applies systematically at arbitrary perturbation order, and is suited to multilevel systems and multiple qubits in both cavity and waveguide quantum electrodynamics. It ultimately enables the explicit construction of effective higher-order Hamiltonians while bypassing important limitations of existing techniques, thereby providing a practical toolbox for multiphoton processes in the dispersive regime.

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We propose an adiabatic-elimination formalism in the dispersive regime based on a transition-centric perturbation theory. The perturbative expansion is recast into a diagrammatic framework, while adiabatic elimination is implemented through controlled projections onto transition subspaces. Our approach applies systematically at arbitrary perturbation order, and is suited to multilevel systems and multiple qubits in both cavity and waveguide quantum electrodynamics. It ultimately enables the explicit construction of effective higher-order Hamiltonians while bypassing important limitations of existing techniques, thereby providing a practical toolbox for multiphoton processes in the dispersive regime.
Various approaches have been used in the literature for eliminating nonresonant levels in atomic systems and deriving effective Hamiltonians. Important among these are elimination techniques at the level of probability amplitudes, operator techniques to project the dynamics on to the subspace of resonant levels, Green’s function techniques, the James’ effective Hamiltonian approach, etc. None of the previous approaches is suitable for deriving effective Hamiltonians in intracavity situations. However, the James’ approach does work in the case of only two-photon transitions in a cavity. A generalization of the James’ approach works in the case of three-photon transitions in a cavity, but only under Raman-like resonant conditions. Another important approach for adiabatic elimination is based on an adaptation of the Markov approximation well-known in the theory of system–bath interactions. However, this approach has not been shown to work in intracavity situations. In this paper, we present a method of adiabatic elimination for atoms inside cavities in the presence of multiphoton transitions. We work in the Heisenberg picture, and our approach has the advantage that it allows one to derive effective Hamiltonians even when Raman-like resonance conditions do not hold.
We introduce a framework where light-matter transitions, rather than states, are the primary dynamical objects. Successive compositions of elementary transitions yield multiphoton processes with compact diagrammatic bookkeeping of resonant and off-resonant pathways. This approach enables transparent derivations of effective high-order Hamiltonians in the dispersive regime, foundational to quantum-information applications. Applied to the paradigmatic Jaynes-Cummings model, our framework reveals a photon-number-independent intrinsic Rabi frequency and persistent polaritonic hybridization in the dispersive regime, unifying resonant and dispersive limits.
Most quantum theorists are familiar with different ways of describing the effective quantum dynamics of a system coupled to external degrees of freedom, such as the Born-Markov master equation or the adiabatic elimination. Understanding the deep connection between these -- sometimes apparently unrelated -- methods can be a powerful tool, allowing us to derive effective dynamics in unconventional systems or regimes. This tutorial aims at providing quantum theorists across multiple fields (e.g., quantum and atom optics, optomechanics, or hybrid quantum systems) with a self-contained practical toolbox to derive effective quantum dynamics, applicable to systems ranging from N -level emitters to mechanical resonators. First, we summarize the projector approach to open quantum systems and the derivation of the fundamental Nakajima-Zwanzig equation. Then, we show how three common effective equations, namely the Brownian master equation, the Born-Markov master equation, and the adiabatic elimination used in atom and molecular optics, can be derived from different perturbative expansions of the Nakajima-Zwanzig equation. We also solve in detail four specific examples using this formalism, namely a harmonic oscillator subject to displacement noise, the effective equations of a mechanical resonator cooled by an optical cavity, the Purcell effect for a qubit coupled to an optical cavity, and the adiabatic elimination in a Lambda system.
Essential-state models are central for quantum control and technology in broad regimes of light-matter interaction. The canonical effective Hamiltonian is obtained equivalently from adiabatic elimination, the Markov approximation, and the pole approximation. These approximations are known to break down at high intensities, significantly limiting their applicability to moderate light-matter interaction. We show how this limitation can be addressed by applying quasi-degenerate Rayleigh-Schrödinger perturbation theory (QD-RSPT). We reconcile QD-RSPT with adiabatic elimination and propose a quasi-degenerate extension of adiabatic elimination that is robust when the detuning of the essential states is non-negligible. The accuracy of QD-RSPT is demonstrated in both the low- and high-frequency regime, showing excellent agreement with Floquet calculations at high intensities. The crucial corrections to adiabatic elimination make the eigenvectors of the effective Hamiltonian non-orthogonal. Physically, this allows us to account for the asymmetric strength with which different essential states couple to the non-essential states. We expect that our systematic approach to effective Hamiltonians from QD-RSPT will constitute a new state of the art in intense light-matter interaction and quantum optics with novel forms of strong coupling and quantum control phenomena being conceivable.
A systematic perturbation scheme is developed for approximate solutions to the time-dependent Schrödinger equation with a space-adiabatic Hamiltonian. For a particular isolated energy band, the basic approach is to separate kinematics from dynamics. The kinematics is defined through a subspace of the full Hilbert space for which transitions to other band subspaces are suppressed to all orders, and the dynamics operates in that subspace in terms of an effective intraband Hamiltonian. As novel applications, we discuss the Born-Oppenheimer theory to second order and derive for the first time the nonperturbative definition of the g factor of the electron within nonrelativistic quantum electrodynamics.