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arXiv:2605.13694

Floquet engineering of nonreciprocal light-induced dipolar interactions

Livia Egyed, Murad Abuzarli, Manuel Reisenbauer, Iurie Coroli, Benjamin A. Stickler, Uroš Delić

quant-phphysics.atom-phphysics.opticsSubmitted May 13, 2026• Announced May 14, 2026
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Abstract

Tweezer arrays of polarizable objects are a promising platform for assembling quantum matter and building next-generation quantum sensors. Light-induced dipolar interactions have emerged as a method to couple their motion, thereby establishing a new paradigm for controlling collective mechanical degrees of freedom. Here, we extend these into the regime of Floquet-driven interactions, combined with the intrinsic nonreciprocity of optical forces. We demonstrate beamsplitter, single-, and two-mode squeezing operations, as well as signatures of a negative-mass-like oscillator arising from the nonreciprocity. Moreover, we show that a programmable combination of these operations enables continuous tuning of complex eigenfrequencies. These results establish a toolbox of quantum operations of nonreciprocal interactions that are essential for investigating non-Hermitian many-body physics and collective quantum optomechanics.

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Tweezer arrays of polarizable objects are a promising platform for assembling quantum matter and building next-generation quantum sensors. Light-induced dipolar interactions have emerged as a method to couple their motion, thereby establishing a new paradigm for controlling collective mechanical degrees of freedom. Here, we extend these into the regime of Floquet-driven interactions, combined with the intrinsic nonreciprocity of optical forces. We demonstrate beamsplitter, single-, and two-mode squeezing operations, as well as signatures of a negative-mass-like oscillator arising from the nonreciprocity. Moreover, we show that a programmable combination of these operations enables continuous tuning of complex eigenfrequencies. These results establish a toolbox of quantum operations of nonreciprocal interactions that are essential for investigating non-Hermitian many-body physics and collective quantum optomechanics.
We propose and analyze a general scheme to engineer programmable and nonreciprocal interactions in an array of atoms coupled to a photonic waveguide. By subjecting each atom to a local harmonic frequency modulation with a defined phase ${\ensuremath{\theta}}_{i}$, we demonstrate the emergence of effective long-range couplings whose parameters are dynamically controllable. For atoms coupled to a conventional waveguide, the modulation dresses the atomic operators, leading to effective interactions governed by the Bessel function J0{\mathcal{J}}_{0}J0​ whose argument depends on the phase differences $\mathrm{\ensuremath{\Delta}}{\ensuremath{\theta}}_{ij}$. For atoms coupled to a photonic crystal waveguide near its band edge, where the density of states is sharply varying, the modulation can be tuned to selectively activate the J12{\mathcal{J}}_{1}^{2}J12​ term, which simultaneously scales both the coherent and dissipative components of the complex coupling strength ${\mathrm{\ensuremath{\Gamma}}}_{ij}$. Crucially, the spatial profile of the local modulation phases imprints a factor $exp(\mathrm{i}\mathrm{\ensuremath{\Delta}}{\ensuremath{\theta}}_{ij})$ onto the waveguide-mediated coupling strength ${\mathrm{\ensuremath{\Gamma}}}_{ij}$, enabling the synthesis of nonreciprocal quantum interactions. Our approach thus provides a flexible toolbox for simulating a wide range of non-Hermitian Hamiltonians on waveguide-QED platforms.
Polar molecules are a promising platform for quantum-enhanced sensing and precision tests of fundamental physics, owing to their strong long-range dipolar interactions, broad sensitivity to electromagnetic fields, and sensitivity to potential physics beyond the Standard Model. However, the creation of metrologically useful entangled states in molecular systems has remained elusive. Here, we report the first observation of a class of metrologically useful entangled states - spin-squeezed states - in polar CaF molecules trapped in an optical tweezer array. The spin degree of freedom is encoded in rotational levels which are directly coupled by dipolar exchange interactions. By harnessing appropriate dynamical decoupling schemes we observe up to 3.0(3)dB of metrological gain, (2.2(3)dB without measurement correction) from direct exchange interactions. Using Floquet engineering, we further realize richer Hamiltonians that preserve spin squeezing while enabling the development of longer-range quantum correlations. Using site- and spin-resolved measurements we demonstrate that these entangled states enhance sensitivity to both homogeneous and spatially varying fields, and reveal strong non-classical correlations, including bipartite entanglement and Einstein-Podolsky-Rosen steering. Finally, we transfer the spin-squeezed states into long-lived and non-interacting hyperfine states, where the metrological enhancement persists for up to 100ms. Our results establish molecular optical tweezer arrays as a scalable platform for generating, controlling, characterizing, and storing entangled states of molecules, opening new opportunities for quantum-enhanced sensing and precision tests of fundamental physics.
Models of interacting quantum spins are used in many areas of physics ranging from the study of magnetism and strongly correlated materials to quantum sensing. In this work, we study coherent many-body dynamics of interacting spin models realized using polar molecules trapped in rearrangeable optical tweezer arrays. Specifically, we encode quantum spins in long-lived rotational states and use the electric dipolar interaction between molecules, together with Floquet Hamiltonian engineering, to realize 1/r31/r^31/r3 XXZ and XYZ models. We microscopically probe several types of coherent dynamics in these models, including quantum walks of single spin excitations, the emergence of magnon bound states, and coherent creation and annihilation of magnon pairs. Our results establish molecular tweezer arrays as a new quantum simulation platform for interacting quantum spin models.
Arrays of optically trapped nanoparticles have emerged as a platform for the study of complex nonequilibrium phenomena. Analogous to atomic many-body systems, one of the crucial ingredients is the ability to precisely control the interactions between particles. However, the optical interactions studied thus far only provide conservative optical binding forces of limited tunability. In this work, we exploit the phase coherence between the optical fields that drive the light-induced dipole-dipole interaction to couple two nanoparticles. In addition, we effectively switch off the optical interaction and observe electrostatic coupling between charged particles. Our results provide a route to developing fully programmable many-body systems of interacting nanoparticles with tunable nonreciprocal interactions, which are instrumental for exploring entanglement and topological phases in arrays of levitated nanoparticles.
We propose a Floquet-engineered framework for the coherent control of the light-matter interaction in a two-level system (TLS) located in a time-modulated cavity. Strictly phase-preserving operation of the TLS-cavity interaction is demonstrated, allowing the interrupt and retrieval of coherent Rabi oscillations without the loss of quantum information. By introducing a phonon reservoir, it is proved that the frequency instability induced from non-Markovian processes does not produce significant phase decoherence during Floquet modulation. Our results provide new insights into the fundamental physics of a driven quantum system and establish Floquet engineering as a powerful tool for coherent quantum information processing.
Neutral atom arrays driven into Rydberg states constitute a promising approach for realizing programmable quantum systems. Enabled by strong interactions associated with Rydberg blockade, they allow for simulation of complex spin models and quantum dynamics. We introduce a new Floquet engineering technique for systems in the blockade regime that provides control over novel forms of interactions and entanglement dynamics in such systems. Our approach is based on time-dependent control of Rydberg laser detuning and leverages perturbations around periodic many-body trajectories as resources for operator spreading. These time-evolved operators are utilized as a basis for engineering interactions in the effective Hamiltonian describing the stroboscopic evolution. As an example, we show how our method can be used to engineer strong spin exchange, consistent with the blockade, in a one-dimensional chain, enabling the exploration of gapless Luttinger liquid phases. In addition, we demonstrate that combining gapless excitations with Rydberg blockade can lead to dynamic generation of large-scale multipartite entanglement. Experimental feasibility and possible generalizations are discussed.