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arXiv:2604.25910 · Quantum Science and Technology

Heralding probability optimization for nonclassical light generated by photon counting measurements on multimode Gaussian states

Jaromír Fiurášek

quant-phSubmitted Apr 28, 2026• Announced Apr 29, 2026• 0 citations
v1 · Apr 28, 2026v2 · Aug 5, 2026
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Abstract

Generation of highly non-classical quantum states of light is essential for optical quantum information processing and quantum metrology. Given the lack of sufficiently strong nonlinear interactions between optical fields, the commonly employed optical quantum-state preparation schemes are conditional, based on nonlinearity induced by heralding photon number measurement on a part of a multimode squeezed Gaussian state. Development and optimization of such probabilistic quantum-state engineering schemes represents one of the central challenges in current quantum optics. As technology advances and experiments progress to detection of higher numbers of photons, the maximization of the heralding probability becomes essential to ensure sufficiently high state-preparation rates. Here, we show that for the conditional quantum state preparation schemes based on Gaussian states and photon number measurements the maximization of the heralding probability can be formulated as finding solution to a system of polynomial equations, which offers an efficient way to find the optimal configuration and allows us to apply techniques dedicated specifically to solving such systems of equations. Our approach can seamlessly incorporate bounds on the available single-mode quadrature squeezing, which is highly experimentally relevant. We mainly consider generation of finite superpositions of Fock states but show that the approach can be straightforwardly extended to generation of squeezed superpositions of Fock states. We focus on Gaussian states with vanishing coherent displacements, hence the conditionally generated states have well defined photon number parity. We illustrate our general methodology on examples of generation of single-mode and two-mode states with two heralding modes.

Journal reference
Quantum Sci. Technol. 11, 035074 (2026)
DOI
10.1088/2058-9565/ae9185
Comments
17 pages, 6 figures, REVTeX4

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Generation of highly non-classical quantum states of light is essential for optical quantum information processing and quantum metrology. Given the lack of sufficiently strong nonlinear interactions between optical fields, the commonly employed optical quantum-state preparation schemes are conditional, based on nonlinearity induced by heralding photon number measurement on a part of a multimode squeezed Gaussian state. Development and optimization of such probabilistic quantum-state engineering schemes represents one of the central challenges in current quantum optics. As technology advances and experiments progress to detection of higher numbers of photons, the maximization of the heralding probability becomes essential to ensure sufficiently high state-preparation rates. Here, we show that for the conditional quantum state preparation schemes based on Gaussian states and photon number measurements the maximization of the heralding probability can be formulated as finding solution to a system of polynomial equations, which offers an efficient way to find the optimal configuration and allows us to apply techniques dedicated specifically to solving such systems of equations. Our approach can seamlessly incorporate bounds on the available single-mode quadrature squeezing, which is highly experimentally relevant. We mainly consider generation of finite superpositions of Fock states but show that the approach can be straightforwardly extended to generation of squeezed superpositions of Fock states. We focus on Gaussian states with vanishing coherent displacements, hence the conditionally generated states have well defined photon number parity. We illustrate our general methodology on examples of generation of single-mode and two-mode states with two heralding modes.
Highly nonclassical states of light - such as the approximate Gottesman-Kitaev-Preskill states, states exhibiting cubic nonlinear squeezing, or cat-like states - can be generated from experimentally accessible Gaussian states via photon counting measurements on selected modes, conditioned on specific outcomes of these heralding events. A simplest yet important example of this approach involves performing photon number measurements on one mode of a two-mode entangled Gaussian state. The heralding probability of this scheme is a key figure of merit, as it determines the generation rate of the target nonclassical state. In this work we show that the maximum heralding probability for the two-mode setting can be calculated analytically, and we investigate its dependence on the number of detected photons n. Our results show that the number of required experimental trials scales only polynomially with n. Generation of highly complex optical quantum states with high stellar rank is thus in principle possible in this setting, given access to sufficiently strong squeezing.
Schrödinger cat states are important non-Gaussian resources for quantum information processing and quantum-enhanced metrology. Although photon subtraction from squeezed vacuum states has proven useful for generating such states in the optical domain, scaling to large amplitudes while maintaining high fidelity and heralding probability remains challenging. To address these obstacles, we analyze alternating squeezing and photon-number-subtraction operations. Rather than optimizing for a single heralding outcome, we formulate cat-state generation as a fidelity-constrained multibranch problem, jointly optimizing the total probability of all photon-number outcomes satisfying a prescribed fidelity threshold at one common experimental setting. Already for plain photon subtraction, this provides a more operational measure of the usable generation probability and can favor parameter configurations that differ from single-branch optima. Considering experimental constraints on available squeezing and photon-number-resolving capability, we demonstrate improvements in fidelity and success probability compared with plain photon subtraction, without necessarily increasing the required squeezing resources. Without restrictions on photon-number resolution, we find that the optimal architecture of the alternating scheme reduces to one of two single-subtraction endpoint configurations, depending on the available squeezing resources. When photon-number resolution is additionally limited, genuinely alternating branches can become advantageous. We derive analytical expressions for the conditional states, cat-state fidelities, and heralding probabilities, enabling efficient multibranch optimization and a systematic analysis of resource trade-offs, sensitivity to experimental parameter deviations, and heralding loss. Together, these results identify the architecture best suited to a given resource budget.
Abstract Conditional measurement schemes, which employ linear optical elements and photon detectors, have recently become powerful tools for generating and enriching nonclassical states in single- and multi-mode scenarios. Here, the nonclassical resourcefulness of a simple single-mode conditional measurement (CM) setup, with a coherent state as one input state, is examined. Studying the output of this setup in the form of displaced qudits (DQ) simplifies the complete characterization of nonclassical resources. The figures of merit of the prepared states are evaluated through quadrature squeezing and some of the non-Gaussian measures such as the Hilbert–Schmidt distance, the quantum relative entropy and the Wigner negativity to identify the squeezing and non-Gaussianity of the states, respectively. The squeezing capacity of the DQ output is compared with the achievable squeezing in finite superposed Fock states, since DQ also constitute a finite-dimensional representation. This optimal squeezing is attained when the detector detects the single photons in the CM setup. All the studied non-Gaussian measures confirm the qualitative agreement that the non-Gaussianity of the setup is limited and does not exceed that of the input number state. The interplay of nonclassical resources between non-Gaussianity and squeezing is exemplified, showing that states exhibiting non-Gaussianity do not exhibit squeezing, and vice versa. In addition, experimental imperfections, such as photon-source impurities and detector inefficiencies, are accommodated to analyze the realistic preparation of DQ. The calculated success probabilities are around 15 % to create the maximally squeezed states under experimental conditions. It demonstrates the potential of nonclassical state generation with minimal nonclassical inputs through the CM scheme.
We propose a heralded entanglement generation scheme based on Gaussian sources enhanced by photon addition and subtraction operations. By combining single-mode squeezing, linear interferometers, and conditional photon-number measurements on ancillary modes, our model can probabilistically generate dual-rail encoded Bell, GHZ, and W states. We systematically optimize the squeezing parameters and interferometer settings to maximize both the heralding success probability and the fidelity with the target states. Our results show that photon addition and subtraction significantly enhance the non-classicality of the output states and improve generation performance, while maintaining computational efficiency comparable to single-photon source models. We further analyze the robustness of the scheme under parameter perturbations and find that its performance remains stable under realistic experimental imperfections. This work provides a versatile and experimentally feasible framework for scalable heralded entanglement generation using Gaussian resources with non-Gaussian operations.
Non-Gaussian operations can reshape the photon statistics of continuous-variable probes, but their metrological advantage is meaningful only when heralding probability and photon-number resources are counted consistently. We compare photon subtraction, photon addition, and photon catalysis as input-side heralding operations in a balanced SU(1,1) interferometer with parity detection. A unified finite-transmissivity map supplies closed conditional moments and the corresponding quantum Fisher information at arbitrary operation order; internal loss is absorbed into a single effective parity observable whose lossless limit recovers the ideal pulled-back measurement. At fixed preparation parameters, single-photon subtraction and addition improve the conditional phase information over the Gaussian reference across most of the high-transmissivity regime, while multi-photon catalysis opens useful low-transmissivity windows. However, when the coherent--squeezed allocation is independently optimized at fixed conditional-probe energy and fixed interferometer gain, the success-weighted Fisher information of all three non-Gaussian operations remains below the optimized Gaussian benchmark. This conclusion is subject to the tested constraints: single-photon operations, a coherent-plus-squeezed-vacuum Gaussian family, fixed gain, and parity readout. Photon catalysis separately generates a conditional branch with high local quantum Fisher information that dark-point parity extracts poorly, identifying a measurement mismatch rather than a state-preparation failure. The result draws a sharp boundary between conditional non-Gaussian enhancement and practically available precision under explicitly stated resource constraints.
Optical quantum information science plays a central role in the development of advanced photonic technologies, with applications ranging from quantum imaging and communication to continuous-variable (CV) quantum computing. The efficient realization of these technologies depends not only on the generation of nonclassical states of light but also on their proper detection. Optical parametric amplification (OPA) has long been known as both a fundamental nonlinear process for generating nonclassical light and as a method to boost detection efficiency through pre-amplification. Recently, OPA has been revisited as a tool for all-optical quadrature detection, offering a powerful alternative to conventional homodyne detection by enabling broadband, loss-tolerant squeezing measurements across various optical platforms. In this thesis, I establish optical parametric amplification as a versatile tool for the detection of CV quantum states through all-optical quadrature detection. I extend squeezing detection to high-dimensional scenarios by exploiting the intrinsic multimode nature of OPA, thereby enabling, for the first time to the best of my knowledge, the real-time monitoring of multimode squeezed light, a long-standing challenge in quantum optics. This approach further permits the simultaneous monitoring of multiple CV Einstein–Podolsky–Rosen (EPR) mode pairs, providing a framework for scalable detection of multimode entanglement, namely optical cluster states, which constitute essential resources for CV quantum computing. Furthermore, I demonstrate OPA as a platform for loss-tolerant and broadband quantum state tomography, applying it to both Gaussian and non-Gaussian states. This paves the way for the scalable tomography of multimode quantum states. Finally, I show that OPA enables the certification of the non-Gaussian and nonclassical character of quantum states without the need for photon-number-resolving detectors, relying instead on post-amplification intensity statistics. In particular, I amplify a single photon sufficiently strongly that its non-Gaussian character becomes accessible through conventional intensity detectors. Altogether, this work establishes optical parametric amplification as a powerful and scalable platform for high-dimensional continuous-variable optical quantum technologies.