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arXiv:2604.09915

Phase-enhanced excitations in pumped collective nuclear systems

Mihai A. Macovei, Fabian Richter, Adriana Pálffy

quant-phSubmitted Apr 10, 2026• Announced Apr 14, 2026• 0 citations
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Abstract

The quantum dynamics of an externally driven ensemble of nuclear two-level systems embedded in a leaky broadband cavity is investigated theoretically. In the considered scenario both the nuclear ensemble and the cavity mode are coherently pumped by two externally applied x-ray electromagnetic fields. When the frequencies of the applied coherent fields are identical, cross-correlations among the existing decay channels increase the nuclear excitation probabilities depending on the phase difference of the applied fields. Our results show that the excited state of the nuclear ensemble may exhibit sub- to super-Poissonian nuclear statistics, demonstrating induced correlations during photon absorption or emission processes. The role of cross-correlations for the superradiant decay and the collective Lamb shift of the ensemble is also investigated.

Comments
9 pages, 5 figures

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The quantum dynamics of an externally driven ensemble of nuclear two-level systems embedded in a leaky broadband cavity is investigated theoretically. In the considered scenario both the nuclear ensemble and the cavity mode are coherently pumped by two externally applied x-ray electromagnetic fields. When the frequencies of the applied coherent fields are identical, cross-correlations among the existing decay channels increase the nuclear excitation probabilities depending on the phase difference of the applied fields. Our results show that the excited state of the nuclear ensemble may exhibit sub- to super-Poissonian nuclear statistics, demonstrating induced correlations during photon absorption or emission processes. The role of cross-correlations for the superradiant decay and the collective Lamb shift of the ensemble is also investigated.
Coherent control of nuclear pumping in a three-level system driven by x-ray light is investigated. In single nuclei the pumping performance is determined by the branching ratio of the excited state populated by the x-ray pulse. Our results are based on the observation that in ensembles of nuclei, cooperative excitation and decay leads to a greatly modified nuclear dynamics which we characterize by a time-dependent cooperative branching ratio. We discuss prospects of steering the x-ray pumping by coherently controlling the cooperative decay. First, we study an ideal case with purely superradiant decay and perfect control of the cooperative emission. A numerical analysis of x-ray pumping in nuclear forward scattering with coherent control of the cooperative decay via externally applied magnetic fields is presented. Next, we provide an extended survey of nuclei suitable for our scheme, and propose proof-of-principle implementations already possible with typical M\"ossbauer nuclei such as 57Fe^{57}\mathrm{Fe}57Fe. Finally, we discuss the application of such control techniques to the population or depletion of long-lived nuclear states.
Abstract The narrow nuclear resonances of Mössbauer isotopes constitute almost ideal two‐level systems to study cooperative effects in the interaction of x‐rays with matter. Embedding an ensemble of resonant Mössbauer nuclei into a planar cavity facilitates the excitation of superradiant oscillatory eigenmodes via pulses of synchrotron radiation. These modes exhibit a large collective Lamb shift that can be controlled via the excitation conditions and the cavity geometry. Cooperative emission in connection with the radiative coupling of two resonant ensembles in a cavity leads to electromagnetically induced transparency (EIT). This contribution gives a review on cooperative effects in nuclear resonant scattering of synchrotron radiation. Special emphasis is given to the basic principles of recent experiments that led to the observation of the collective Lamb shift and EIT with nuclear resonances in the regime of hard x‐rays.
The electromagnetic transitions of Mössbauer nuclei provide ideal two-level systems to study the cooperative effects of X-rays with matter. Recently, we have observed the collective Lamb shift (CLS) in nuclear γ-ray superradiance [Röhlsberger, R.; Schlage, K.; Sahoo, B.; Couet, S.; Rüffer, R. Science 2010, 328, 1248–1251]. An ensemble of resonant 57Fe nuclei was embedded in the center of a planar cavity and was collectively excited by synchrotron radiation into a purely superradiant state. The decay of the superradiant state can be almost two orders of magnitude faster than the single-atom nuclear decay and can be accompanied by a CLS of more than 10 times the natural linewidth. Here we review the basic features of cooperative effects that occur in nuclear γ-ray superradiance in comparison with similar effects observed in the optical regime of the electromagnetic spectrum. We show that nuclear resonant scattering of synchrotron radiation opens new ways for systematic studies of cooperative effects in the interaction of X-rays with matter.
Abstract We investigate a hybrid quantum system consisting of two coupled optical cavities, each containing an ensemble of coherently pumped artificial or real two-level atoms. The system is modelled within the dressed-state formalism, accounting for coherent driving and dissipative interactions with independent electromagnetic reservoirs. Focusing on the regime where the Rabi frequency greatly exceeds the collective spontaneous emission and cavity decay rates, respectively, we derive the equations of motion characterizing the system and analyse its steady-state behaviours. Special attention is given to the scenario in which only one cavity contains a pumped multi-atom ensemble, and as a consequence, coherent excitation transfer to the second cavity occurs via cavity–cavity coupling. In this case, the mean photon number in the second cavity mode scales proportional to the squared number of atoms, i.e., N2 from the first cavity. The proposed model offers insight into light–matter interaction in composite systems and suggests viable mechanisms for engineering collective interactions and non-local excitation transport in quantum optical platforms.
This thesis is dedicated to the study of collective effects of nuclei in single xray photon superradiance. To this end we investigate aspects of superradiance in both nuclear forward scattering and in thin-film cavities with an embedded 57Fe nuclear layer. A general theoretical framework is developed to investigate a single-photon cooperative emission from a cloud of resonant systems, atoms or nuclei, in the presence of magnetic hyperfine splitting. In the limit of a thick sample, we present our results for two means to coherently control the collective single x-ray photon emission in nuclear forward scattering. In the limit of a thin sample in a thin-film cavity with embedded resonant nuclei, we find out that unlike the magnetic hyperfine splitting of a single atom or nucleus, interesting collective effects may occur which modify the hyperfine level structure. In addition, for a certain parameter regime a spectrum reminiscent of electromagnetically induced transparency (EIT) can be achieved. Based on this EIT-like effect, a theoretical control mechanism for stopping x-ray pulses in the thin-film x-ray cavity is put forward. Finally, we show theoretically that for the case of two nuclear ensembles in the thin-film cavity, pseudo-Rabi splitting due to the strong coupling between the two layers should occur. The latter findings are confirmed by preliminary experimental data.
Superradiant burst often arises from photon-mediated interactions within an excited ensemble of emitters, where collective emission leads to a sharp increase in photon intensity. Here, we focus on a nuclear ensemble with cooperative excitations and propose, for the first time, the generation of superradiant burst of x-ray photons. We establish the required excitation conditions to observe x-ray superradiant bursts, offering guidance for the experiments utilizing state-of-the-art x-ray sources. Building on this, we investigate the dynamics of the x-ray superradiant burst and reveal novel nonlinear relationships between the time required to reach the peak intensity and the excitation number, as well as between the peak intensity and the excitation number. Additionally, we introduce a dimensionless parameter that serves as an indicator of the system, reflecting how strongly the burst can occur in a given configuration. Our work provides fresh insights into the understanding of collective emission in many-body x-ray-nuclei systems within the nonlinear regime, opening new avenues for x-ray quantum optics.