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arXiv:2603.21751 · Advanced Materials

Nonlinear Electro-Optic Visible Photonic Circuits for Solid-State Quantum Defects

Yongchan Park, Yong Soo Lee, Hansol Kim, Jaepil Park, Junhyung Lee, Hye-yoon Jeon, Jinil Lee, Yong-gwon Kim, Yeeun Choi, Min-Kyo Seo, Dae-Hwan Ahn, Hojoong Jung, Dongyeon Daniel Kang, Hyounghan Kwon

physics.opticsquant-phSubmitted Mar 23, 2026• Announced Mar 24, 2026• 0 citations
arXivHTMLPDF

Abstract

Integrated visible photonic engines for solid-state quantum defects provide a foundation for scalable quantum networks. While miniaturization is advancing, active manipulation remains limited by the difficulty of achieving simultaneous milliwatt-scale visible light generation and high-contrast modulation. Despite extensive efforts, the concurrent chip-scale realization of nonlinear frequency conversion and fast temporal gating for high-fidelity quantum control has remained elusive. Here, we demonstrate a monolithic thin-film lithium niobate (TFLN) platform integrating periodically poled frequency conversion with GHz-bandwidth electro-optic (EO) switching. The device delivers off-chip green-light power exceeding 1 mW with an extinction ratio (ER) of 42.2 dB, enabling coherent spin control and time-resolved lifetime measurements of individual nitrogen-vacancy (NV) centers in diamond through nanosecond gating. System performance is validated through pulsed optically detected magnetic resonance (ODMR), Rabi oscillations, and Ramsey interference, supported by time-tagged photon counting with nanosecond resolution. By unifying sufficient nonlinear light generation with high-speed active manipulation, this platform establishes a scalable framework for the realization of high-rate quantum communication nodes.

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physics.opticsCross-listedarXiv:2603.08609•Mar 10, 2026
Integrated visible photonic engines for solid-state quantum defects provide a foundation for scalable quantum networks. While miniaturization is advancing, active manipulation remains limited by the difficulty of achieving simultaneous milliwatt-scale visible light generation and high-contrast modulation. Despite extensive efforts, the concurrent chip-scale realization of nonlinear frequency conversion and fast temporal gating for high-fidelity quantum control has remained elusive. Here, we demonstrate a monolithic thin-film lithium niobate (TFLN) platform integrating periodically poled frequency conversion with GHz-bandwidth electro-optic (EO) switching. The device delivers off-chip green-light power exceeding 1 mW with an extinction ratio (ER) of 42.2 dB, enabling coherent spin control and time-resolved lifetime measurements of individual nitrogen-vacancy (NV) centers in diamond through nanosecond gating. System performance is validated through pulsed optically detected magnetic resonance (ODMR), Rabi oscillations, and Ramsey interference, supported by time-tagged photon counting with nanosecond resolution. By unifying sufficient nonlinear light generation with high-speed active manipulation, this platform establishes a scalable framework for the realization of high-rate quantum communication nodes.
Time-bin encoded quantum states of light are crucial for quantum technology applications. The integration of manipulation functionalities into chip-scale devices is essential for deploying scalable, high-performance, and cost-effective quantum networks. Here we develop a fully integrated, high-throughput quantum receiver based on the thin-film lithium niobate (TFLN) platform, capable of high-speed electro-optic manipulation of time-bin encoded quantum states. The device's novel architecture enables active switching of time-bin quantum states with an electro-optic bandwidth exceeding 30 Ghz, while supporting real-time arbitrary projective measurements with a bandwidth of over 1 GHz. We showcase its versatility and performance through several applications, including the certification of entanglement with Bell's inequality violation by 38 standard deviations and with >95% visibility. We then apply it to a fiber-based quantum communication scenario, where we experimentally demonstrate an entanglement-based quantum key distribution (QKD) protocol, achieving stable finite-size secure key rates exceeding 25 kbit/s over 12 hours of continuous operation. By leveraging a high-speed active switching scheme, the system overcomes the need for temporal post-selection, eliminating a fundamental loophole that compromises the security of time-bin entanglement-based QKD protocols and relaxes the temporal resolution requirements of single-photon detectors. Moreover, it enables active selection of the projection basis, increasing the flexibility for communication parties. This approach establishes a versatile and scalable architecture for time-bin encoded quantum communication, enabling practical protocols on industry-grade photonic technology.
The realization of quantum networks capable of distributing quantum information over kilometer scale distances is key to maximizing the potential of quantum information technology. Implementing this technology requires both the ability to generate remote entanglement between quantum memory nodes, requiring an efficient spin-photon interface, and the ability to efficiently scale the classical optical control and multiplexing optics within a given node. In this work, we develop integrated photonics platforms in diamond and thin film lithium niobate to address both of these issues. Together, these platforms provide the necessary ingredients to create large scale quantum networking technology. For the quantum network nodes, we extend previous results combining diamond nanophotonic resonators with the silicon-vacancy defect as a quantum networking platform. We demonstrate, for the first time, quantum entanglement between SiV quantum memories across 35km in a deployed fiber network. We also develop additional functionalities within the SiV platform including the incorporation of deterministic strain to increase defect yield and deterministic single photon generation with the SiV. In order to enable the scalable control and multiplexing of individual SiV centers necessary for realizing practical quantum network nodes, we develop a state-of-the-art electro-optics platform operating at visible wavelengths using thin film lithium niobate. We develop an understanding of fabrication induced losses at visible wavelengths in the platform and a variety of key devices in the platform including high-bandwidth, low-drive voltage amplitude and phase modulators, as well as high-efficiency off chip couplers. Utilizing this platform we perform ultra-high efficiency electro-optic frequency shifting, achieving a 15 GHz frequency shift with over 50% efficiency. Finally, using our measured device performance, we discuss and model how these devices can effectively multiplex SiV-based quantum nodes. Thus through these two platforms we have demonstrated the necessary ingredients to realize large-scale quantum network nodes.
Within the last decade, thin-film lithium niobate (TFLN) has emerged as a leading integrated photonics platform with immediate applications in classical communications. Concurrently, TFLN components tailored to the requirements of photonic quantum information processing have also garnered considerable interest. Chief among these is the quasi-phase matched (QPM) nonlinear frequency mixer—implemented via periodic domain inversion in ferroelectric lithium niobate—which can be used to generate photon pairs, squeezed states of light, and to perform single photon frequency conversion. Here, we demonstrate progress towards realizing a spectrally separable photon pair source in lithium niobate via waveguide dispersion engineering—a technique uniquely enabled by sub-wavelength optical mode confinement in the thin-film platform. Subsequently, we design optimize a scalable fabrication process to produce QPM TFLN devices for applications that require strict adherence to a specified operating wavelength, such as quantum frequency conversion in a quantum communications network. Finally, we explore how high-performance electro-optic devices can be combined with these nonlinear optical devices to realize a multi-functional platform in which quantum states of light can be generated and manipulated within a single, compact photonic integrated circuit.
Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (±641 GHz or ±5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.
Diamond photonics has enabled efficient interfaces for quantum memories and is predicted to be a critical component of quantum networks. However, scalable network architectures require spatial, temporal, and spectral control of photons, which relies on nonlinear and electro-optic functionalities that diamond alone cannot provide. Here, we demonstrate heterogeneous integration of a thin-film lithium niobate (TFLN) platform, which has strong chi-2 nonlinearity and electro-optic effects, with thin diamond films. We demonstrate high-Q diamond photonic crystal cavities (Q factors exceeding 5x10^4 at 735 nm) that are lithographically aligned with TFLN photonic backbone and critically coupled to it. This allows us to realize low-loss diamond-TFLN "escalators" (loss ~1 dB/coupler) that support efficient light transfer between them. At cryogenic temperatures (5K), we can collect photons emitted from silicon vacancies (SiVs) embedded within the diamond structure via the TFLN photonic circuit. This approach establishes a scalable route toward integrated photonic circuits for practical quantum networking and other technologies.