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arXiv:2603.13754

A Highly Sensitive Diamond NV Magnetometer Using Ramsey Interferometry with a Short Sensor-to-Sample Distance

Yuta Araki, Takeharu Sekiguchi, Yuji Hatano, Naota Sekiguchi, Chikara Shinei, Masashi Miyakawa, Takashi Taniguchi, Tokuyuki Teraji, Hiroshi Abe, Shinobu Onoda, Takeshi Ohshima, Takayuki Shibata, Mutsuko Hatano, Takayuki Iwasaki

quant-phSubmitted Mar 14, 2026• Announced Mar 17, 2026
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Abstract

In this study, we developed a diamond quantum magnetometer based on Ramsey interferometry with a short sensor-to-sample distance. Conventional biomagnetic sensors with ensemble nitrogen-vacancy centers using continuous-wave optically detected magnetic resonance and Ramsey methods typically rely on watt-level lasers to achieve high sensitivity, resulting in thermal issues. In contrast, by employing the light-trapping diamond waveguide technique in a high-pressure and high-temperature diamond sample treated with electron beam irradiation, we obtained a high photon conversion efficiency of 9.5%, enabling us to simultaneously achieve a high sensitivity of 2.93(7) pT/Hz^1/2 in the 100-400 Hz frequency range and a minimal temperature increase of only approximately 13 K at a low laser power of 210 mW. Using a dry phantom designed to mimic magnetoencephalography signals, we measured a weak magnetic field of 77.7(2) pT without signal averaging at a sensor-to-sample distance of 2.5 mm. This short-distance measurement prevents severe spatial signal attenuation, yielding a high signal-to-noise ratio. The development here is crucial for practical biomagnetic applications based on Ramsey interferometry.

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In this study, we developed a diamond quantum magnetometer based on Ramsey interferometry with a short sensor-to-sample distance. Conventional biomagnetic sensors with ensemble nitrogen-vacancy centers using continuous-wave optically detected magnetic resonance and Ramsey methods typically rely on watt-level lasers to achieve high sensitivity, resulting in thermal issues. In contrast, by employing the light-trapping diamond waveguide technique in a high-pressure and high-temperature diamond sample treated with electron beam irradiation, we obtained a high photon conversion efficiency of 9.5%, enabling us to simultaneously achieve a high sensitivity of 2.93(7) pT/Hz^1/2 in the 100-400 Hz frequency range and a minimal temperature increase of only approximately 13 K at a low laser power of 210 mW. Using a dry phantom designed to mimic magnetoencephalography signals, we measured a weak magnetic field of 77.7(2) pT without signal averaging at a sensor-to-sample distance of 2.5 mm. This short-distance measurement prevents severe spatial signal attenuation, yielding a high signal-to-noise ratio. The development here is crucial for practical biomagnetic applications based on Ramsey interferometry.
Diamond quantum sensors utilizing nitrogen-vacancy (NV) centers in diamond can measure a tiny magnetic-field variation at room temperature with a high linearity and high spatial resolution. Because of these advantages, they have been actively studied for application to measure a biomagnetic field. In biomagnetic sensing applications, it is effective to measure at multiple points simultaneously with high sensitivity. In this study, we developed a highly sensitive diamond quantum sensor that can simultaneously measure the magnetic field at two points at the millimeter interval. We used two diamonds that were split from one HPHT-grown diamond and placed them at the 3-mm interval. A laser-induced fluorescence from the two diamonds were detected by a single photodiode. We applied different bias magnetic fields to each diamond, and thus the magnetic resonances at these diamonds had different resonance frequencies. By applying microwave fields whose frequencies were modulated at different modulation frequencies, the magnetic fields at the two diamonds can be obtained independently after demodulation. The noise spectral densities in the magnetic field measurement at the two diamonds’ locations. Since the measurement was performed outside a magnetic shield, a severe low-frequency environmental noise from railways and power line (50 Hz) noise peaks were observed. We evaluated the field sensitivities at the two diamonds to be 22 pT/√Hz in 25-300 Hz range with neglecting the power-line noise peaks and the environment noise peaks. The capability of simultaneously measuring a magnetic field at two points with the such high sensitivities will facilitate the biomagnetic sensing applications.
We developed a highly sensitive and long-term stable diamond quantum magnetometer by integrating a dual-feedback system that compensates for common- and differential-mode frequency shifts in double-quantum (DQ) 4-Ramsey interferometry. Detecting extremely weak magnetic-field signals requires extensive signal accumulation to enhance the signal-to-noise ratio. However, deviations from the optimal operating frequencies caused by thermal drift or environmental magnetic noise severely hinder the long-term stability of such a sensing system. To overcome the limitation, we first derived analytical solutions for the signal response to common- and differential-mode detunings based on a detuning-inclusive Hamiltonian to theoretically clarify the robustness limit in DQ 4-Ramsey sensing. Guided by this theoretical model, we introduced synchronized frequency modulation and a dual-feedback scheme to independently track and compensate for these frequency shifts while maintaining an optimal magnetic-field response. The proposed method enabled stable continuous operation against temperature variations of 2.8 K. By maintaining a magnetic field sensitivity of 7.0 pT/Hz^1/2 in the frequency range of 5-100 Hz for a prolonged duration of 4 hours, we achieved an extremely low noise floor of 64 fT/Hz^1/2. During prolonged continuous sensing, the system exhibited the expected 1/T^1/2 scaling with integration time T, and prevented both the underestimation of amplitude and waveform distortion. These results establish a robust approach for long-term DQ 4-Ramsey diamond magnetometry and demonstrate its potential for detecting weak biomagnetic signals.
Nitrogen-vacancy (NV) color centers in diamond are promising solid-state quantum sensors working at room temperature. The number of NV centers limits the magnetic sensitivity of the quantum magnetometer. Increasing the number of NV centers is a challenging task due to technical issues such as microwave power density, detection noise.Here, we developed the sensor system with a large detection volume which contains a lot of NV centers. The microwave circuit enhances microwave power density. Digital filter with frequency modulation of microwave allows us to detect the magnetic field with low noise. Consequently, we obtained a DC magnetic field sensitivity of 980 pT/√Hz.This work was supported by MEXT Quantum Leap Flagship Program (MEXT Q-LEAP) Grant Number JPMXS0118067395.
The nitrogen–vacancy center in diamond enables highly sensitive magnetic-field measurements. In this work, we demonstrate an excellent sensitivity of 7.9 pT·Hz –1/2 in the near-DC range of 1 to 1000 Hz. This performance is achieved using a 35 mW laser power and 1 mW microwave power enabled by 561 nm laser excitation and the resonant-antenna design. By leveraging dual resonance with intrinsic π shift for real-time common-mode rejection, this technique effectively suppresses low-frequency noise and pushes the 1/ f corner frequency down to 1 Hz, with a measured sensitivity at 1 Hz of 10.6 pT·Hz –1/2 . The magnetometer also exhibits excellent capability in detecting magnetic anomalies, promoting the practical use of diamond quantum sensors in biomedical, geophysical, and other real-world applications.
Nitrogen-vacancy (NV) centers in diamond have emerged as a robust room-temperature solid-state platform for weak magnetic field detection. Several NV-based magnetometers have been proposed in the past decades, but they still suffer from either low sensitivity or high power consumption. This is a challenge for sensors deployed in remote locations on Earth or in space that are not connected to the power grid. Although sunlight-driven quantum magnetometry, which does not rely on conventional energy sources, has been proposed as a possible solution, its sensitivity remains a limitation. Here, we present an impressive improvement in the sensitivity of the sunlight-driven NV-diamond quantum magnetometer. A crucial aspect of our approach involves leveraging the ground-state level anti-crossing properties of the NV centers, coupled with magnetic flux concentrators. This integration enables us to achieve a magnetic-field sensitivity of 26 pT/Hz in a laboratory environment and 49 pT/Hz when the magnetometer operates outdoors under sunlight. We also illustrate the promising potential of further improving the sensitivity to the subpicotesla level by using cutting-edge technologies. Furthermore, we reveal the capability of this quantum magnetometer as a receiver of extremely low-frequency magnetic signals and pave the way for communication applications. These advancements represent a significant leap toward attaining high-sensitivity and energy-efficient magnetic field sensing and expanding the range of possible applications for these environmentally sustainable quantum technologies.
Wide-field imaging of magnetic signals using ensembles of nitrogen-vacancy (NV) centers in diamond has garnered increasing interest due to its combination of micron-scale resolution, millimeter-scale field of view, and compatibility with diverse samples from across the physical and life sciences. Recently, wide-field NV magnetic imaging based on the Ramsey protocol has achieved uniform and enhanced sensitivity compared to conventional measurements. Here, we integrate the Ramsey-based protocol with spin-bath driving to extend the NV spin dephasing time and improve magnetic sensitivity. We also employ a high-speed camera to enable dynamic wide-field magnetic imaging. We benchmark the utility of this quantum diamond microscope (QDM) by imaging magnetic fields produced from a fabricated wire phantom. Over a 270 × 270 μm2 field of view, a median per-pixel magnetic sensitivity of 4.1(1) nT /Hz is realized with a spatial resolution ≲ 10 μm and sub-millisecond temporal resolution. Importantly, the spatial magnetic noise floor can be reduced to the picotesla scale by time-averaging and signal modulation, which enables imaging of a magnetic-field pattern with a peak-to-peak amplitude difference of about 300 pT. Finally, we discuss potential new applications of this dynamic QDM in studying biomineralization and electrically active cells.