An experimental investigation of intracavity dispersion effects in a synchronously pumped optical parametric oscillator (SPOPO) is presented. A flexible setup combining spectral and phase shaping of both pump and local oscillator fields with frequency-resolved balanced homodyne detection is employed to examine how intracavity dispersion influences squeezing. Different cavity configurations with varying finesse and dispersion conditions are studied, and the squeezing is measured as a function of pump power and local oscillator bandwidth. Contrary to expectations based on existing theoretical models, the measured squeezing levels remain essentially unchanged as dispersion varies. To account for these observations, a modeling approach is introduced in which intracavity dispersion is described as an effective spectral filtering occurring at the stage of SPOPO supermode generation. Within this framework, the filtering is incorporated directly into the interaction Hamiltonian of the nonlinear process. This perspective establishes a consistent experimental benchmark for the study of dispersion in SPOPOs and underscores the importance of spectral filtering in the interpretation of multimode squeezing experiments.
An experimental investigation of intracavity dispersion effects in a synchronously pumped optical parametric oscillator (SPOPO) is presented. A flexible setup combining spectral and phase shaping of both pump and local oscillator fields with frequency-resolved balanced homodyne detection is employed to examine how intracavity dispersion influences squeezing. Different cavity configurations with varying finesse and dispersion conditions are studied, and the squeezing is measured as a function of pump power and local oscillator bandwidth. Contrary to expectations based on existing theoretical models, the measured squeezing levels remain essentially unchanged as dispersion varies. To account for these observations, a modeling approach is introduced in which intracavity dispersion is described as an effective spectral filtering occurring at the stage of SPOPO supermode generation. Within this framework, the filtering is incorporated directly into the interaction Hamiltonian of the nonlinear process. This perspective establishes a consistent experimental benchmark for the study of dispersion in SPOPOs and underscores the importance of spectral filtering in the interpretation of multimode squeezing experiments.
Multimode squeezed light is a key resource for quantum technologies, enabling applications in boson sampling, quantum networks, and optical quantum computation [1],[2]. Parametric down-conversion in synchronously pumped optical parametric oscillators (SPOPOs) offers a versatile platform for generating multimode squeezed states across the time-frequency domain. In these systems, supermodes manifest as independent quantum states in the temporal domain and as frequency combs in the spectral domain [3]. Precise control of these states is crucial for quantum applications and requires an experimental setup capable of fine-tuning multiple parameters to optimize squeezing properties. In this work, we present an experimental setup for generating and characterizing multimode vacuum squeezed states using a SPOPO and a balanced homodyne detection scheme. Two spatial light modulators (SLMs) placed on the pump and local oscillator (LO) beams provide full control over their spectral properties, including amplitude and phase shaping. This flexibility allows us to optimize the experimental conditions and investigate squeezing dependence on key parameters such as the LO spectral detuning and bandwidth. By introducing a programmableπ-phase shift to the LO via the SLM, we selectively probe the multimode structure, distinguishing between even and odd supermodes. Additionally, the SLM on the pump can introduce an arbitrary chirp, further enhancing control over the system. Our setup, schematized in Figure 1a, is based on a commercial mode-locked Yb-fiber laser operating at 93MHz, emitting pulses centered at 1035nm with a 10nm bandwidth. A portion of the radiation is frequency-doubled to 517.5nm via an LBO crystal to serve as the pump for the SPOPO, while the remaining part is used as the LO for homodyne detection after transmission through the SPOPO cavity, ensuring high beam quality. The SPOPO cavity is frequency-locked to the laser via a Pound-Drever-Hall technique, ensuring stable and optimized operation. Figure 1b presents representative measurements of squeezing levels as a function of the LO spectral bandwidth, showing how its symmetric or antisymmetric phase influences the detection of different supermodes and, consequently, the squeezing level depending on their structure. The measurements were performed using lithium niobate (LNB) nonlinear crystals of 3.0mm and 1.5mm lengths. Our setup allows for future investigations of dispersion effects on squeezing, thus far only theoretically predicted [4], by introducing chirped mirrors for dispersion compensation. Moreover, different nonlinear crystals, such as lithium niobate, beta barium borate (BBO), and lithium triborate (LBO) of various lengths, will be tested to explore the multimode properties of the squeezed states. These investigations will provide insights into the experimental conditions required to achieve single-mode squeezing, crucial for applications such as Gaussian Boson Sampling, with results to be presented at the conference.
A synchronously pumped optical parametric oscillator (SPOPO) operating at 93 MHz is used to generate squeezed states at 1035 nm. The system features a counter-propagating beam at the same wavelength as the quantum state, which simultaneously actively stabilizes the cavity and, after transmission, acts as the local oscillator for homodyne detection. By deriving the local oscillator directly from the SPOPO cavity, the setup establishes an intrinsically excellent spatial mode overlap and high interference visibility, forming a distinctive self-referenced architecture. Two spatial light modulators enable precise spectral shaping of both the pump and the local oscillator in amplitude and phase, allowing investigation of the spectral properties of the generated states. The versatility of the setup further allows exploration of different SPOPO configurations, including regimes with varied finesse and escape efficiency. Representative measurements, including homodyne traces and squeezing levels as functions of pump power and local oscillator bandwidth, demonstrate the performance of the system. Theoretical simulations based on a multimode singular-value-decomposition model reproduce well the measured dependence of squeezing on pump power and LO bandwidth, confirming the accuracy of the description and the robustness of the setup. Measured squeezing levels up to − 3.3 dB are achieved, corresponding to − 5.7 dB at SPOPO output, evidencing the robustness and versatility of this platform for stable pulsed squeezed-light generation and advanced quantum optical applications.
Abstract Parametric down-conversion in a nonlinear crystal is a widely employed technique for generating quadrature squeezed light with multiple modes, which finds applications in quantum metrology, quantum information and communication. Here we study the generation of temporally multimode femtosecond pulsed squeezed light in a synchronously pumped optical parametric oscillator (SPOPO) operating below the oscillation threshold, while considering the presence of non-compensated intracavity group-velocity dispersion. Based on the developed time-domain model of the system, we show that the dispersion results in mode-dependent detuning of the broadband supermodes of the pulsed parametric process from the cavity resonance due to temporal Gouy phase, as well as linear coupling between these supermodes. With perturbation theory up to the second order in the coupling coefficients between modes, we obtained a solution for the amplitudes of multiple supermodes given an arbitrary sub-threshold pump level. The dispersion affects the quantum state of the supermodes by influencing their squeezing level and the rotation of the squeezing ellipse. It also affects the entanglement among the supermodes, leading to reduced suppression of shot noise level as measured in the balanced homodyne detection scheme. Furthermore, our study highlights the potential of SPOPO with group-velocity dispersion as a testbench for experimental investigations of multimode effects in linearly evanescent coupled parametric oscillators.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables [1]. They can be generated either by mixing different squeezed light sources using linear optical operations [2], or directly in a multimode optical device [3, 4]. Synchronously Pumped Optical Parametric Oscillators (SPOPO) — which correspond to an OPO pumped by a train of ultrashort pulses that are synchronized with the cavity round-trip time — have been theoretically shown to be promising devices for the generation of multimode nonclassical frequency combs, since a SPOPO is a sole optical cavity acting as an assembly of independent squeezers in a particular basis called the supermodes basis [5]. The supermodes are optical frequency combs with specific spectrum and phase profiles that are determined by the length of the intracavity nonlinear crystal and the pulse shape of the pump.
We present in this paper a general model for determining the quantum properties of the light generated by a synchronously pumped optical parametric oscillator (SPOPO) operating below threshold. This model considers time and frequency on an equal footing, which allows us to find new quantum properties, related for example to the carrier envelope offset (CEO) phase, and to consider situations that are close to real experiments. We show that, in addition to multimode squeezing in the so-called ‘supermodes’, the system exhibits quadrature entanglement between frequency combs of opposite CEO phases. We have also determined the quantum properties of the individual pulses and their quantum correlations with the neighboring pulses. Finally, we determine the quantum Cramer–Rao limit for an ultra-short time delay measurement using a given number of pulses generated by the SPOPO.
Quantum optical frequency combs are of great significance in the fields of quantum computing, quantum information, and high precision quantum measurement, which can be produced by using a degenerate type-I synchronously pumped optical parametric oscillator (SPOPO). When anisotropic crystal is used as a nonlinear medium in the SPOPO, the spatial walk-off effect will occur due to the birefringence effect, which cannot be ignored and will adversely affect the generation of squeezed state. In this work, we investigate the influence of spatial walk-off effect on the squeezing level of quantum optical frequency combs both theoretically and experimentally. A Ti∶sapphire mode-locked femtosecond pulsed laser which produces 130 fs pulse trains at 815 nm with a repetition rate of 76 MHz is utilized as a fundamental source. Its second harmonic at 407.5 nm is used to pump the collinear BiB3O6 (BIBO) crystal for generating the squeezed vacuum frequency comb. It is indicated that as the crystal length increases, the area of interaction between pump light and signal light decreases gradually. Thus the enhancement of squeezing is eventually limited by the spatial walk-off effect. According to the simulations, the squeezing level reaches a maximum value when the crystal length is 1.49 mm. The quantum properties of squeezed vacuum optical frequency combs obtained for four crystal lengths (0.5, 1.0, 1.5 and 2.0 mm) are subsequently measured experimentally. When the length of BIBO is 1.5 mm, the maximum vacuum squeezing of (3.6±0.2) dB is obtained, which is (7.0±0.2) dB after being corrected for detection loss. The experimental results are consistent with the numerical simulations. This study demonstrates that the spatial walk-off effect in nonlinear crystal is a significant factor affecting the quantum optical frequency comb, and the theoretical model presented in this paper can be used to provide a guideline for optimizing the experimental implementation.