Wave--particle duality is a hallmark of quantum mechanics. For bosonic systems, there exists a continuum of intermediate states bridging wave-like Schrödinger cat states and particle-like Fock states. Such states have recently been recognized as valuable resources for enhancing fault-tolerant quantum computation (FTQC) with propagating light. Here we experimentally demonstrate tunable generation of these intermediate states by employing generalized photon subtraction (GPS). By detecting up to three photons from squeezed-light sources with a photon-number-resolving detector, we continuously control the balance between wave- and particle-like features. This approach allows us to construct a spectral family of quantum states with high generation rates, optimized according to the required fault-tolerance threshold. Our results establish GPS as a versatile toolbox for tailoring non-Gaussian resources, opening a pathway to efficient Gottesman--Kitaev--Preskill (GKP) qubit generation and addressing a central bottleneck in optical quantum computing.
Wave--particle duality is a hallmark of quantum mechanics. For bosonic systems, there exists a continuum of intermediate states bridging wave-like Schrödinger cat states and particle-like Fock states. Such states have recently been recognized as valuable resources for enhancing fault-tolerant quantum computation (FTQC) with propagating light. Here we experimentally demonstrate tunable generation of these intermediate states by employing generalized photon subtraction (GPS). By detecting up to three photons from squeezed-light sources with a photon-number-resolving detector, we continuously control the balance between wave- and particle-like features. This approach allows us to construct a spectral family of quantum states with high generation rates, optimized according to the required fault-tolerance threshold. Our results establish GPS as a versatile toolbox for tailoring non-Gaussian resources, opening a pathway to efficient Gottesman--Kitaev--Preskill (GKP) qubit generation and addressing a central bottleneck in optical quantum computing.
The generation of a logical qubit called the Gottesman-Kitaev-Preskill (GKP) qubit in an optical traveling wave is a major challenge for realizing large-scale universal fault-tolerant optical quantum computers. Recently, probabilistic generation of elementary GKP qubits has been demonstrated using photon number measurements and homodyne measurements. However, the generation rate is only a few Hz, and it will be difficult to generate fault-tolerant GKP qubits at a practical rate unless success probability is significantly improved. Here, we propose a method to efficiently synthesize GKP qubits from several quantum states by adaptive Gaussian operations. In the initial-state preparation that utilizes photon number measurements, an adaptive operation allows any measurement outcome above a certain threshold to be considered as a success. This threshold is lowered by utilizing the generalized photon subtraction method. The initial states are synthesized into a GKP qubit by homodyne measurements and a subsequent adaptive operation. As a result, the single-shot success probability of generating fault-tolerant GKP qubits in a realistic scale system exceeds 10, which is $1\ifmmode\times\else\texttimes\fi{}{10}^{6}$ times better than previous methods. This proposal will become a powerful tool for advancing optical quantum computers from the proof-of-principle stage to practical application.
Quantum technologies, encompassing communication, computation, and metrology, rely on the generation and control of non-Gaussian states of light. These states enable secure quantum communication, fault-tolerant quantum computation, and precision sensing beyond classical limits, yet their practical realisation remains a major challenge due to reliance on high-photon-number Fock states or strong non-linearities. Here we introduce a unified optical framework that removes this constraint, using only Gaussian inputs, optical parametric amplification, and heralded photon detection. Within a single architecture, we demonstrate the generation of photon-added squeezed states with near unit fidelity, cubic-phase-like states with strong non-linearities and fidelities above 98.5%, and squeezed-cat states exceeding 99% fidelity that can be iteratively bred into GKP grid states surpassing the 9.75 dB fault-tolerance threshold. Operating entirely below 3 dB of input squeezing, the approach provides a scalable, experimentally accessible platform that unites the state resources required for quantum communication, metrology, and computation within one coherent optical framework.
A near-deterministic source of non-Gaussianity is the missing piece to reach universal and fault-tolerant quantum computing with continuous-variable optics. Due to a lack of strong non-linearities, the probabilistic photon-subtracted Gaussian states remain the most promising contender. In combination with Gaussian measurements and single-mode feed-forward operations, they have been shown to provide sufficient non-Gaussianity at high rates. However, these existing breeding protocols lack the necessary loss tolerance to be experimentally feasible. In this work, we introduce a mathematical formalism based on the application of a Gaussian blur and filter on the measured Fock Wigner function to describe general photon-subtracted Gaussian states. Within our representation, the initial squeezing, Gaussian measurements, and photon loss can all be understood as contributions to the total blurring and interchanged accordingly. We find that this intuitive approach can be used to find improvements to cat, cubic phase, and GKP state generation by compromising between success rates, feed-forward compatibility, and loss tolerance. In the case of multiple photon subtractions, this is achieved by introducing a hybrid setup variant bridging the gap between protocols based on breeding and post-selection. Finally, we establish a general lower bound on the resources needed to generate a given target state near-deterministically by introducing the expected Wigner logarithmic negativity as an additive monotone of non-Gaussianity.
Abstract Quantum technologies, encompassing communication, computation, and metrology, rely on the generation and control of non-Gaussian states of light. These states enable secure quantum communication, fault-tolerant quantum computation, and precision sensing beyond classical limits, yet their practical realisation remains a major challenge due to reliance on high-photon-number Fock states or strong non-linearities. Here we introduce a unified optical framework that removes this constraint, using only Gaussian inputs, optical parametric amplification, and heralded photon detection. Within a single architecture, we demonstrate the generation of photon-added squeezed states with near unit fidelity, cubic-phase-like states with strong non-linearities and fidelities above 98.5%, and squeezed-cat states exceeding 99% fidelity that can be iteratively bred into GKP grid states surpassing the 9.75 dB fault-tolerance threshold. Operating entirely below 3 dB of input squeezing, the approach provides a scalable, experimentally accessible platform that unites the state resources required for quantum communication, metrology, and computation within one coherent optical framework.
Non-Gaussian states are essential resources for universal, fault-tolerant optical quantum computing, but their generation rate remains limited by low heralding probabilities and operation in nanosecond temporal modes. Here, we demonstrate multi-photon generalized photon subtraction in picosecond optical wave packets, establishing the state-generation capability required for high-rate operation by addressing the temporal-mode bottleneck that has constrained the achievable rate. Two interfering ultrashort squeezed vacua are heralded by photon-number-resolving detection with a high-speed transition-edge sensor and characterized by pulsed homodyne detection matched to 10-ps temporal modes at a 5-MHz pump repetition rate. We reconstruct Wigner functions without loss correction that exhibit up to four distinct negative regions for four-photon heralding, together with an effective cat-state amplitude of αeff=1.69. This amplitude approaches the range of practical relevance for fault-tolerant cat-code architectures and for adaptive breeding toward logical-qubit generation, while the picosecond temporal mode establishes a platform compatible with high-rate, scalable time-multiplexed photonic architectures.
Gottesman-Kitaev-Preskill (GKP) qubits, known for their exceptional error-correction capabilities, are highly coveted in quantum computing. However, generating optical GKP qubits has been a significant challenge. Measurement-based methods, where a portion of entangled squeezed vacuum modes are measured with photon number resolving detectors heralding a desired state in the undetected modes, have emerged as leading candidates for optical GKP qubit generation due their minimal resource requirements. While the current measurement-based methods can produce high-quality GKP qubits, they suffer from low success probabilities limiting experimental realization. The heart of the problem lies in the duality of photon number resolving measurements, being both the source of nonlinearity needed to generate quality GKP qubits and the component driving down their probability of successful production. Our method, breeding approximate squeezed coherent state superpositions created by generalized photon subtraction, overcomes this problem by supplementing two photon number resolving measurements with a single high success probability homodyne measurement. This scheme achieves success probabilities $\ensuremath{\ge}{10}^{\ensuremath{-}5}$, two orders of magnitude higher than strictly photon number resolving measurement based methods, while still producing states with high fidelity, possessing error-correction capabilities equivalent to up to a 10 dB squeezed GKP qubit. This breakthrough significantly advances the practical use of the optical GKP qubit encoding.