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arXiv:2606.24002

Picosecond Schrödinger cat states for ultrafast optical quantum processing

Mamoru Endo, Kan Takase, Takefumi Nomura, Tatsuki Sonoyama, Kazuma Takahashi, Sachiko Takasu, Daiji Fukuda, Takahiro Kashiwazaki, Asuka Inoue, Takeshi Umeki, Peter van Loock, Petr Marek, Radim Filip, Warit Asavanant, Akira Furusawa

quant-phphysics.opticsSubmitted Jun 22, 2026• Announced Jun 24, 2026• 0 citations
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Abstract

Non-Gaussian states are essential resources for universal, fault-tolerant optical quantum computing, but their generation rate remains limited by low heralding probabilities and operation in nanosecond temporal modes. Here, we demonstrate multi-photon generalized photon subtraction in picosecond optical wave packets, establishing the state-generation capability required for high-rate operation by addressing the temporal-mode bottleneck that has constrained the achievable rate. Two interfering ultrashort squeezed vacua are heralded by photon-number-resolving detection with a high-speed transition-edge sensor and characterized by pulsed homodyne detection matched to 10-ps temporal modes at a 5-MHz pump repetition rate. We reconstruct Wigner functions without loss correction that exhibit up to four distinct negative regions for four-photon heralding, together with an effective cat-state amplitude of $α_{\mathrm{eff}} = 1.69$. This amplitude approaches the range of practical relevance for fault-tolerant cat-code architectures and for adaptive breeding toward logical-qubit generation, while the picosecond temporal mode establishes a platform compatible with high-rate, scalable time-multiplexed photonic architectures.

Comments
43 pages, 12 figures

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Non-Gaussian states are essential resources for universal, fault-tolerant optical quantum computing, but their generation rate remains limited by low heralding probabilities and operation in nanosecond temporal modes. Here, we demonstrate multi-photon generalized photon subtraction in picosecond optical wave packets, establishing the state-generation capability required for high-rate operation by addressing the temporal-mode bottleneck that has constrained the achievable rate. Two interfering ultrashort squeezed vacua are heralded by photon-number-resolving detection with a high-speed transition-edge sensor and characterized by pulsed homodyne detection matched to 10-ps temporal modes at a 5-MHz pump repetition rate. We reconstruct Wigner functions without loss correction that exhibit up to four distinct negative regions for four-photon heralding, together with an effective cat-state amplitude of αeff=1.69α_{\mathrm{eff}} = 1.69αeff​=1.69. This amplitude approaches the range of practical relevance for fault-tolerant cat-code architectures and for adaptive breeding toward logical-qubit generation, while the picosecond temporal mode establishes a platform compatible with high-rate, scalable time-multiplexed photonic architectures.
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The generation of non-Gaussian quantum states is a key requirement for universal continuous-variable quantum information processing. We report the experimental generation of large-amplitude squeezed coherent-state superpositions (squeezed cat states) on free-space optical pulses, reaching an amplitude of α=2.47α= 2.47α=2.47, which, to our knowledge, exceeds all previously reported values. Our protocol relies on the controlled mixing of the Fock states ∣1⟩|1\rangle∣1⟩ and ∣2⟩|2\rangle∣2⟩ through a tunable beam splitter, followed by heralding via homodyne detection. The resulting state displays three well-resolved negative regions in its Wigner function and achieves a fidelity of 0.530.530.53 with the target state ∝S^(z)(∣α⟩−∣−α⟩)\propto \hat{S}(z)(|α\rangle - |-α\rangle)∝S^(z)(∣α⟩−∣−α⟩), with α=2.47α= 2.47α=2.47 and squeezing parameter z=0.56z = 0.56z=0.56. These results constitute a significant milestone for temporal breeding protocols and for the iterative generation of optical GKP states, opening new perspectives for scalable and fault-tolerant photonic quantum architectures.
In the field of continuous-variable quantum information processing, non-Gaussian states with negative values of the Wigner function are crucial for the development of a fault-tolerant universal quantum computer. While several non-Gaussian states have been generated experimentally, none have been created using ultrashort optical wave packets, which are necessary for high-speed quantum computation, in the telecommunication wavelength band where mature optical communication technology is available. In this paper, we present the generation of non-Gaussian states on wave packets with a short 8-ps duration in the 1545.32 nm telecommunication wavelength band using photon subtraction up to three photons. We used a low-loss, quasi-single spatial mode waveguide optical parametric amplifier, a superconducting transition edge sensor, and a phase-locked pulsed homodyne measurement system to observe negative values of the Wigner function without loss correction up to three-photon subtraction. These results can be extended to the generation of more complicated non-Gaussian states and are a key technology in the pursuit of high-speed optical quantum computation.
Schrödinger cat states are important non-Gaussian resources for quantum information processing and quantum-enhanced metrology. Although photon subtraction from squeezed vacuum states has proven useful for generating such states in the optical domain, scaling to large amplitudes while maintaining high fidelity and heralding probability remains challenging. To address these obstacles, we analyze alternating squeezing and photon-number-subtraction operations. Rather than optimizing for a single heralding outcome, we formulate cat-state generation as a fidelity-constrained multibranch problem, jointly optimizing the total probability of all photon-number outcomes satisfying a prescribed fidelity threshold at one common experimental setting. Already for plain photon subtraction, this provides a more operational measure of the usable generation probability and can favor parameter configurations that differ from single-branch optima. Considering experimental constraints on available squeezing and photon-number-resolving capability, we demonstrate improvements in fidelity and success probability compared with plain photon subtraction, without necessarily increasing the required squeezing resources. Without restrictions on photon-number resolution, we find that the optimal architecture of the alternating scheme reduces to one of two single-subtraction endpoint configurations, depending on the available squeezing resources. When photon-number resolution is additionally limited, genuinely alternating branches can become advantageous. We derive analytical expressions for the conditional states, cat-state fidelities, and heralding probabilities, enabling efficient multibranch optimization and a systematic analysis of resource trade-offs, sensitivity to experimental parameter deviations, and heralding loss. Together, these results identify the architecture best suited to a given resource budget.
We propose a multiphoton heralding scheme using an optical parametric amplifier (OPA) that converts squeezed vacuum into two families of non-Gaussian states: large-amplitude squeezed Schrödinger cat states and low-order parity-selective Fock superpositions. By injecting m photons into the idler port and detecting n photons at the output, effective high-order photon subtraction is realized in a single OPA device. The heralded states exhibit strong Wigner negativity and high phase-space complexity. Remarkably, under photon loss, the complexity remains substantial even after negativity vanishes, indicating a loss-resilient quantum resource. These states also surpass the Heisenberg limit in phase estimation. Our protocol establishes the OPA as a versatile platform for generating non-Gaussian states, with promising applications in loss-resilient quantum metrology and fault-tolerant quantum information processing.
A near-deterministic source of non-Gaussianity is the missing piece to reach universal and fault-tolerant quantum computing with continuous-variable optics. Due to a lack of strong non-linearities, the probabilistic photon-subtracted Gaussian states remain the most promising contender. In combination with Gaussian measurements and single-mode feed-forward operations, they have been shown to provide sufficient non-Gaussianity at high rates. However, these existing breeding protocols lack the necessary loss tolerance to be experimentally feasible. In this work, we introduce a mathematical formalism based on the application of a Gaussian blur and filter on the measured Fock Wigner function to describe general photon-subtracted Gaussian states. Within our representation, the initial squeezing, Gaussian measurements, and photon loss can all be understood as contributions to the total blurring and interchanged accordingly. We find that this intuitive approach can be used to find improvements to cat, cubic phase, and GKP state generation by compromising between success rates, feed-forward compatibility, and loss tolerance. In the case of multiple photon subtractions, this is achieved by introducing a hybrid setup variant bridging the gap between protocols based on breeding and post-selection. Finally, we establish a general lower bound on the resources needed to generate a given target state near-deterministically by introducing the expected Wigner logarithmic negativity as an additive monotone of non-Gaussianity.