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arXiv:2601.16747

Moderate-terahertz-induced plateau expansion of high-order harmonic generation to soft X-ray region

Doan-An Trieu, Duong D. Hoang-Trong, Cam-Tu Le, Sang Ha, Ngoc-Hung Phan, F. V. Potemkin, Van-Hoang Le, Ngoc-Loan Phan

physics.opticsquant-phSubmitted Jan 23, 2026• Announced Jan 26, 2026• Revised Feb 1, 2026 (v2)
v1 · Jan 23, 2026v2 · Feb 1, 2026
arXivHTMLPDF

Abstract

Extending the high-harmonic cutoff with experimentally accessible fields is essential for advancing tabletop coherent extreme ultraviolet (EUV) and soft X-ray sources. Although terahertz (THz) assistance offers a promising route, cutoff extension at weak, laboratory-accessible THz strengths remain poorly understood. In this report, we comprehensively investigate THz-assisted high-order harmonic generation (HHG) using time-dependent Schrödinger equation simulations supported by classical trajectory analysis and Bohmian-based quantum dynamics. By mapping the plateau evolution versus THz strength, we show that even weak THz fields can extend the cutoff, producing a pronounced ``fish-fin'' structure whose prominent rays saturate near $I_p + 8 U_p$. We trace this extension to long electron excursions spanning several optical cycles before recombination, and provide a fully consistent explanation using both classical analysis and Bohmian trajectories flow. Our findings reveal that this cutoff-extension mechanism is remarkably robust, persisting across different atomic species and remaining insensitive to variations in the driving parameters. These results demonstrate that cutoff control is achievable with laboratory-scale THz fields, offering practical guidelines for engineering coherent high-energy HHG, and providing a robust pathway for tracking ultrafast electron motion in real time.

DOI
10.1103/n2fj-tqfb
Comments
Version 2: 6 pages, 3 figures

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Extending the high-harmonic cutoff with experimentally accessible fields is essential for advancing tabletop coherent extreme ultraviolet (EUV) and soft X-ray sources. Although terahertz (THz) assistance offers a promising route, cutoff extension at weak, laboratory-accessible THz strengths remain poorly understood. In this report, we comprehensively investigate THz-assisted high-order harmonic generation (HHG) using time-dependent Schrödinger equation simulations supported by classical trajectory analysis and Bohmian-based quantum dynamics. By mapping the plateau evolution versus THz strength, we show that even weak THz fields can extend the cutoff, producing a pronounced ``fish-fin'' structure whose prominent rays saturate near Ip+8UpI_p + 8 U_pIp​+8Up​. We trace this extension to long electron excursions spanning several optical cycles before recombination, and provide a fully consistent explanation using both classical analysis and Bohmian trajectories flow. Our findings reveal that this cutoff-extension mechanism is remarkably robust, persisting across different atomic species and remaining insensitive to variations in the driving parameters. These results demonstrate that cutoff control is achievable with laboratory-scale THz fields, offering practical guidelines for engineering coherent high-energy HHG, and providing a robust pathway for tracking ultrafast electron motion in real time.
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High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically non-classical, requiring from quantum mechanics for a complete explanation as, under suitable conditions, involves phenomena such as particle tunneling through a potential barrier. When exposed to a high-intensity, low-frequency laser field, bound electrons ionize via tunneling, accelerate under the driving field, and recombine with the parent ion, emitting high-harmonic radiation. However, electrons can follow two distinct pathways -- short and long trajectories -- during these steps. In this work, we evaluate the signatures left by these trajectories on the quantum optical state after HHG, and observe that they lead to entanglement between the driving field and the generated harmonics. By leveraging these correlations, we use harmonic generation to herald the creation of optical Schrödinger cat-like states in the driving field. Additionally, using an ab-initio approach, we examine how propagation effects, which spatially separate the harmonic contributions from short and long trajectories, influence the non-classical characteristics of the emitted light.
High harmonic generation (HHG) has emerged as a powerful probe of ultrafast electron dynamics in solids. However, in strongly correlated materials, where electronic excitations arise from many-body interactions rather than single-particle band dispersion, the field remains in its infancy. Here, we report HHG up to the 23rd^{rd}rd order in the prototypical Mott insulator La2_22​CuO4_44​. We observe a robust 4 eV cutoff that is independent of driving field strength, revealing an intrinsic energy scale defined by the Hubbard bands. Using time-resolved high harmonic spectroscopy, we disentangle the distinct contributions of carrier creation, intraband acceleration, and interband recombination to the nonequilibrium radiation spectrum. We demonstrate that photo-doping triggers a fundamental reorganization of the many-body manifolds above a critical excitation density, a process that renormalizes the band curvature and suppresses nonlinear intraband currents, thereby directly imprinting the signature of many-body band reconstruction onto the harmonic emission. These results establish HHG as a sensitive probe of subtle correlation-driven electronic reconstructions and highlight that many-body interactions enable extreme nonlinear optical responses that are highly tunable in nonequilibrium states.
We extend our recently developed semiclassical strong-field Herman-Kluk propagator (SFHK) method to calculate high-order harmonic generation (HHG) for atoms in intense lasers. We show that our method, based on a combination of the Herman-Kluk propagator and the strong-field approximation, can provide highly accurate results for both HHG yield and phase, nearly identical to those from the exact numerical solutions of the time-dependent Schrödinger equation. We provide detailed analyses of our method and its applications to the HHG process, particularly the recombination time. The main computational task in this method is to solve the classical Newton equations for the active electron in the combined atomic potential and laser-electron interaction. The motion of the centers of the electron wave packets, modeled by coherent states, is governed by independent classical trajectories so that the computation can therefore be parallelized very efficiently.
High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically nonclassical, requiring from quantum mechanics for a complete explanation as, under suitable conditions, involves phenomena such as particle tunneling through a potential barrier. When exposed to a high-intensity, low-frequency laser field, bound electrons ionize via tunneling, accelerate under the driving field, and recombine with the parent ion, emitting high-harmonic radiation. However, electrons can follow two distinct pathways, short and long trajectories, during these steps. In this work, we evaluate the signatures left by these trajectories on the quantum-optical state after HHG, and observe that they lead to entanglement between the driving field and the generated harmonics. By leveraging these correlations, we use harmonic generation to herald the creation of optical Schr\"odinger-cat-like states in the driving field. Additionally, using an ab initio approach, we examine how propagation effects, which spatially separate the harmonic contributions from short and long trajectories, influence the nonclassical characteristics of the emitted light.
High-order harmonic generation (HHG) is one of the most commonly studied nonlinear optical phenomena, originating in the ultrafast dynamics of electrons in atomic gases and semiconductors. It has attracted much attention because of its nonperturbative nature and potential for future attosecond laser pulse sources. On the theory side, a semiclassical picture based on tunneling ionization of electrons is successfully used in explaining key characteristics of the HHG. This model assumes that electric fields nonperturbatively excite electrons beyond the ionization potential or the band gap. Thus, intuitively, a larger gap should lead to an exponentially smaller HHG emission. Despite this intuition, the HHG in the Mott insulator Ca2RuO4{\mathrm{Ca}}_{2}{\mathrm{RuO}}_{4}Ca2​RuO4​ has shown an unconventional exponential increase with respect to the gap width. This experiment implies effects beyond the semiclassical theory. However, most theoretical works have focused on the dependence of the HHG on external control parameters, and the gap dependence of the HHG is poorly understood even in noninteracting systems. Thus, it is essential to clarify the gap dependence of the HHG in a fully quantum mechanical approach. Here, we analyze numerically exactly the gap dependence of the HHG in two-level systems. We find an increase in the strength of the HHG when the Rabi frequency is large compared to the gap width. Furthermore, the relaxation and scattering of electrons increase the visibility of this gap dependence. Finally, we find that the enhancement rate follows a universal scaling law regardless of the driving frequency. The existence of this gap dependence in two-level systems suggests that this unconventional gap dependence is a universal behavior that can be found not only in Mott insulators but also in atomic gases and semiconductors.