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arXiv:2601.16306

A modified Lindblad equation for a Rabi driven electron-spin qubit with tunneling to a Markovian lead

Emily Townsend, Joshua Pomeroy, Garnett W. Bryant

cond-mat.mes-hallquant-phSubmitted Jan 22, 2026• Announced Jan 26, 2026• 0 citations
v1 · Jan 22, 2026v2 · Jan 26, 2026v3 · Feb 6, 2026
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Abstract

We derive a modified Lindblad equation for the state of quantum dot tunnel coupled to a Markovian lead when the spin state of the dot is driven by an oscillating magnetic field. We show that the equation is a completely positive, trace-preserving map and find the jump operators. This is a driven-dissipative regime in which coherent driving is relevant to the tunneling and cannot be treated as simply a rotation modifying the system with a bath derived under a static magnetic field. This work was motivated by an experimental desire to determine the Zeeman splitting of an electron spin on a quantum dot (a spin qubit), and in a related work we show that this splitting energy can be found by measuring the charge occupancy of the dot while sweeping the frequency of the driving field \ arXiv:2503.17481. Here we cover the full derivation of the equation and give the jump operators. These jump operators are potentially useful for describing the stochastic behavior of more complex systems with coherent driving of a spin capable of tunneling on or off of a device, such as in electron spin resonance scanning tunneling microscopy. The jump operators have the interesting feature of combining jumps of electrons onto and off of the device.

Comments
Supplemental info includes the files: LindbladSubstitutionScriptForPub.m (matlab script), LindbladSubstitutions.tex (output of previous), ThereAndBackAgainForPub.m (matlab script), ThereAndBackWRabi.pdf (output of previous)

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We derive a modified Lindblad equation for the state of quantum dot tunnel coupled to a Markovian lead when the spin state of the dot is driven by an oscillating magnetic field. We show that the equation is a completely positive, trace-preserving map and find the jump operators. This is a driven-dissipative regime in which coherent driving is relevant to the tunneling and cannot be treated as simply a rotation modifying the system with a bath derived under a static magnetic field. This work was motivated by an experimental desire to determine the Zeeman splitting of an electron spin on a quantum dot (a spin qubit), and in a related work we show that this splitting energy can be found by measuring the charge occupancy of the dot while sweeping the frequency of the driving field \ arXiv:2503.17481. Here we cover the full derivation of the equation and give the jump operators. These jump operators are potentially useful for describing the stochastic behavior of more complex systems with coherent driving of a spin capable of tunneling on or off of a device, such as in electron spin resonance scanning tunneling microscopy. The jump operators have the interesting feature of combining jumps of electrons onto and off of the device.
We present a unified study of charge and spin qubits encoded in a single interacting quantum dot tunnel-coupled to Rashba fermionic leads. The dot is described by an Anderson impurity Hamiltonian with either repulsive or attractive local interactions and a magnetic field of arbitrary orientation. In the repulsive regime, a spin qubit is encoded in the singly occupied spin sector, whereas in the attractive regime, close to the degeneracy between the empty and doubly occupied configurations, these two states define a charge-qubit subspace. We combine a weak-coupling Lindblad master equation in the Markovian secular limit with numerically controlled matrix-product-state simulations of the full dot-reservoir system. In equilibrium, we identify magnetic pair breaking in the attractive regime and a weak Rashba-induced magnetic anisotropy when the magnetic field is rotated relative to the spin-orbit axis. In the dynamical regime, relaxation and decoherence are controlled by the energetic gap between the logical manifold and nearby leakage states, and are further enhanced by Rashba-dependent tunneling. These findings show that even a minimal Anderson-impurity description captures key ingredients for coherent spin and charge qubits: the energetic structure of leakage states and spin-orbit-dependent dot-lead hybridization.
We analyze the charge and spin dynamics in a DC biased double quantum dot driven by crossed DC and AC magnetic fields. In this configuration, spatial delocalization due to inter-dot tunnel competes with intra-dot spin rotations induced by the time dependent magnetic field, giving rise to a complicated time dependent behavior of the tunnelling current. When the Zeeman splitting has the same value in both dots and spin flip is negligible, the electrons remain in the triplet subspace (dark subspace) performing coherent spin rotations and the current does not flow. This electronic trapping is removed either by finite spin relaxation or when the Zeeman splitting is different in each quantum dot. In the first case, our results show that measuring the current will allow to get information on the spin relaxation time. In the last case, we will show that applying a resonant bichromatic magnetic field, the electrons become trapped in a coherent superposition of states and electronic transport is blocked. Then, manipulating AC magnetic fields, electrons are driven to perform coherent spin rotations which can be unambiguously detected by direct measurement of the tunneling current.
We study the dynamics of open quantum systems driven by an external time-periodic force. Combining Floquet theory and the time-convolutionless projection operator technique we derive a time-local quantum master equation which exactly takes into account the periodic driving, while treating the system-environment interaction within second order in the coupling strength without performing the Markov approximation. The resulting equation of motion for the reduced density matrix is called Floquet time-convolutionless master equation. Employing the example of the driven spin-boson system, we demonstrate that this master equation is capable of describing strong non-Markovian effects, while yielding the Floquet-Lindblad master equation in the Markovian limit. A characteristic feature of memory effects in such driven dissipative systems is the emergence of sharp peaks of the trace-distance based non-Markovianity measure as a function of the driving amplitude, which can be traced back to quasienergy crossings leading to almost decoherence-protected subspaces through a quasienergy-induced dissipative decoupling mechanism.
We analyze coherent spin rotations in a dc biased double quantum dot driven by crossed dc and ac magnetic fields. In this configuration, spatial delocalization due to interdot tunneling competes with intradot spin rotations induced by the time dependent magnetic field, giving rise to a complicated time dependent behavior of the tunneling current. When the Zeeman splitting has the same value in both dots and spin flip is negligible, the electrons remain in the triplet subspace performing coherent spin rotations and current does not flow. This electronic trapping is removed either by finite spin relaxation or when the Zeeman splitting is different in each quantum dot. In the last case, we will show that by applying a resonant bichromatic magnetic field, the electrons become trapped in a coherent superposition of states and electronic transport is blocked. Then, manipulating ac magnetic fields allows one to drive electrons to perform coherent spin rotations which can be unambiguously detected by direct measurement of the tunneling current.
Abstract The standard weak-coupling approximations associated to open quantum systems have been extensively used in the description of a two-level quantum system, qubit, subjected to relatively weak dissipation compared with the qubit frequency. However, recent progress in the experimental implementations of controlled quantum systems with increased levels of on-demand engineered dissipation has motivated precision studies in parameter regimes that question the validity of the approximations, especially in the presence of time-dependent drive fields. In this paper, we address the precision of weak-coupling approximations by studying a driven qubit through the numerically exact and non-perturbative method known as the stochastic Liouville–von Neumann equation with dissipation. By considering weak drive fields and a cold Ohmic environment with a high cutoff frequency, we use the Markovian Lindblad master equation as a point of comparison for the SLED method and study the influence of the bath-induced energy shift on the qubit dynamics. We also propose a metric that may be used in experiments to map the regime of validity of the Lindblad equation in predicting the steady state of the driven qubit. In addition, we study signatures of the well-known Mollow triplet and observe its meltdown owing to dissipation in an experimentally feasible parameter regime of circuit electrodynamics. Besides shedding light on the practical limitations of the Lindblad equation, we expect our results to inspire future experimental research on engineered open quantum systems, the accurate modeling of which may benefit from non-perturbative methods.
We propose a quantum trajectory analysis of a scheme to measure the states of a coupled-dot device (qubit) where there is a fluctuating energy gap Δ between the two states. The system consists of the qubit and a readout dot coupled to source and drain leads. The tunnel rate through the detector is conditioned by the occupation number of the nearer quantum dot (target) of the qubit and therefore probes the states of the qubit. We derive a Lindblad-form master equation to calculate the unconditional evolution of the qubit and a conditional stochastic master equation calculating the conditional evolution for different tunneling rates. The results show the effects of various device parameters and provide the optimum selection and combination of the system structure.