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arXiv:2601.04811 · Zeitschrift für Naturforschung A

Switching magnetization of quantum antiferromagnets: Schwinger boson mean-field theory compared to exact diagonalization

Florian Johannesmann, Asliddin Khudoyberdiev, Götz Silvester Uhrig

Published Mar 17, 2026• 1 citation
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Abstract

Abstract Antiferromagnets have attracted significant attention because of their considerable potential in engineering high-density and ultrafast memory devices, a crucial and increasingly demanded component of contemporary high-performance information technology. Theoretical and experimental investigations are actively progressing to provide the capability of efficient switching and precise control of the Néel vector, which is crucial for the intended practical applications of antiferromagnets. Recently, a time-dependent Schwinger boson mean-field theory has been successfully developed to study the sublattice magnetization switching in anisotropic quantum antiferromagnets [K. Bolsmann et al ., PRX Quantum , vol. 4, 2023, Art. no. 030332]. Here we use a complementary exact diagonalization method to study such sublattice magnetization switching, but in small-cluster quantum antiferromagnets, by means of an external magnetic field. Furthermore, this article aims to support the findings of the Schwinger boson approach. We show that the results of both approaches are consistent at short time scales, with only about 12.5 % deviations. The consistency of the outcomes obtained through this alternative exact approach demonstrates that the time-dependent Schwinger boson mean-field theory is a versatile framework to capture the essentials of the switching process in quantum antiferromagnets. Thereby, the findings of current article pave the way for further theoretical and computational progress in the study of antiferromagnets for engineering spintronic devices with ultrahigh density and ultrafast speed.

DOI
10.1515/zna-2026-0010

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Abstract Antiferromagnets have attracted significant attention because of their considerable potential in engineering high-density and ultrafast memory devices, a crucial and increasingly demanded component of contemporary high-performance information technology. Theoretical and experimental investigations are actively progressing to provide the capability of efficient switching and precise control of the Néel vector, which is crucial for the intended practical applications of antiferromagnets. Recently, a time-dependent Schwinger boson mean-field theory has been successfully developed to study the sublattice magnetization switching in anisotropic quantum antiferromagnets [K. Bolsmann et al ., PRX Quantum , vol. 4, 2023, Art. no. 030332]. Here we use a complementary exact diagonalization method to study such sublattice magnetization switching, but in small-cluster quantum antiferromagnets, by means of an external magnetic field. Furthermore, this article aims to support the findings of the Schwinger boson approach. We show that the results of both approaches are consistent at short time scales, with only about 12.5 % deviations. The consistency of the outcomes obtained through this alternative exact approach demonstrates that the time-dependent Schwinger boson mean-field theory is a versatile framework to capture the essentials of the switching process in quantum antiferromagnets. Thereby, the findings of current article pave the way for further theoretical and computational progress in the study of antiferromagnets for engineering spintronic devices with ultrahigh density and ultrafast speed.
The orientation of the order parameter of quantum magnets can be used to store information in a dense and efficient way.Switching this order parameter corresponds to writing data.To understand how this can be done, we study a precessional reorientation of the sublattice magnetization in an (an)isotropic quantum antiferromagnet induced by an applied magnetic field.For this intriguing nonequilibrium issue, we introduce a description including the leading quantum and thermal fluctuations, namely time-dependent Schwinger boson mean-field theory, because this theory allows us to describe both ordered phases and the phases in between them, as is crucial for switching.An activation energy has to be overcome, requiring a minimum applied field h t that is given essentially by the spin gap.It can be reduced significantly for temperatures approaching the Néel temperature, facilitating switching.The time required for switching diverges when the field approaches h t , which is the signature of an inertia in the magnetization dynamics.The temporal evolution of the magnetization and of the energy reveals signs of dephasing.The switched state has lost a part of its coherence because the magnetic modes do not evolve in phase.
The control of antiferromagnetic order can pave the way to large storage capacity as well as fast manipulation of stored data. Here achieving a steady-state of sublattice magnetization after switching is crucial to prevent loss of stored data. The present theoretical approach aims to obtain instantaneous stable states of the order after reorienting the Néel vector in open quantum antiferromagnets using time-dependent Schwinger boson mean-field theory. The Lindblad formalism is employed to couple the system to the environment. The quantum theoretical approach comprises differences in the effects of dephasing, originating from destructive interference of different wave vectors, and spin-lattice relaxation. We show that the spin-lattice relaxation results in an exponentially fast convergence to the steady-state after full ultrafast switching.
We present the first exact results for the T=0 dynamical structure factor of finite-sized two-dimensional square-lattice spin-(1/2 antiferromagnetic Heisenberg systems with up to 16 spins. Our results are compared to a recently proposed Schwinger boson mean-field theory. We find that the mean-field theory represents an excellent approximation to the exact spin excitation spectra at all allowed wave vectors and for all system sizes studied. We also determine the mean-field value for the T=0 staggered magnetization, mMF=0.306{m}^{\mathrm{MF}=0.306}mMF=0.306, to be in excellent agreement with published Monte Carlo results.
A generalized Schwinger boson representation is proposed to describe the two-dimensional SU(4) symmetric spin-orbital quantum antiferromagnet. A uniform mean field solution gives rise to an antiferromagnetic long range ordered state with a small staggered magnetization ms=0.07566m_{s}=0.07566ms​=0.07566, and the recent quantum Monte Carlo simulations on rather large lattice sizes have provided strong evidence to support these mean field results.
The Kitaev model is an exactly solvable model that exhibits a quantum spin liquid as its ground state. While this model was originally proposed as an S = 1 / 2 spin model on a honeycomb lattice, extensions to higher-spin systems have recently attracted attention. In contrast to the S = 1 / 2 case, such higher- S models are not exactly solvable and remain poorly understood, particularly for spin excitations at finite temperatures. Here, we focus on the S = 1 Kitaev model, which has been proposed to host bosonic quasiparticles. We investigate this model using Schwinger boson mean-field theory, where bosonic spinons are introduced as fractional quasiparticles by extending bond operators to address anisotropic spin interactions. We determine the mean-field parameters that realize a quantum spin liquid in both ferromagnetic and antiferromagnetic Kitaev models. Based on this mean-field ansatz, we calculate the dynamical and equal-time spin structure factors. We find that, when one uses the conventional decoupling scheme based on Wick decoupling with respect to spinons to calculate spin correlations, the resultant spin structure factors exhibit a momentum dependence that is not consistent with the sign structure expected from the exchange interaction: They possess a strong spectral weight indicating ferromagnetic (antiferromagnetic) correlations in the antiferromagnetic (ferromagnetic) Kitaev model. To resolve this issue, we propose an alternative scheme for evaluating the spin correlations, which is based on decoupling with respect to the bond operators. We demonstrate that, in our scheme, this discrepancy is removed, and the momentum dependence of the spin structure factors is consistent with the sign of the exchange constant. We also calculate the temperature evolution of the dynamical spin structure factor and find that the continuum observed at zero temperature splits into two distinct structures as the temperature increases, which can be understood in terms of the bandwidth narrowing of spinons. Finally, we clarify the origin of why the two distinct decoupling schemes result in different momentum dependences of the spin structure factors and discuss their relationship to results obtained in previous studies.
Classical nonlinear theories are highly successful in describing far-from-equilibrium dynamics of magnets, encompassing phenomena such as parametric resonance, ultrafast switching, and even chaos. However, at ultrashort length and time scales, where quantum correlations become significant, these models inevitably break down. While numerous methods exist to simulate quantum many-body spin systems, they are often limited to near-equilibrium conditions, capture only short-time dynamics, or obscure the intuitive connection between nonlinear behavior and its geometric origin in the su(2) spin algebra. To advance nonlinear magnetism into the quantum regime, we develop a theory in which semiclassical spin correlations, rather than individual spins, serve as the fundamental dynamical variables. Defined on the bonds of a bipartite lattice, these correlations are inherently nonlocal, with dynamics following through a semiclassical mapping that preserves the original spin algebra. The resulting semiclassical theory captures nonlinear dynamics that are entirely nonclassical and naturally accommodates phenomenological damping at the level of correlations, which is typically challenging to include in quantum methods. As an application, we focus on Heisenberg antiferromagnets, which feature significant quantum effects. We predict nonlinear scaling of the mean frequency of quantum oscillations in the Néel state with the spin quantum number S. These have no classical analog and exhibit features reminiscent of nonlinear parametric resonance, fully confirmed by exact diagonalization. The predicted dynamical features are embedded in the geometric structure of the semiclassical phase space of spin correlations, making their physical origin much more transparent than in full quantum methods. With this, semiclassical spin-correlation dynamics provide a foundation for exploring nonlinear quantum magnetism.