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arXiv:2601.00966 · Physical Review Applied

Four-Photon Interference with a High-Efficiency Quantum Dot Source

Alistair J. Brash, Luke Brunswick, Mark R. Hogg, Catherine L. Phillips, Malwina A. Marczak, Timon L. Baltisberger, Sascha R. Valentin, Arne Ludwig, Richard J. Warburton

quant-phSubmitted Jan 2, 2026• Announced Jan 6, 2026• 0 citations
v1 · Jan 2, 2026v2 · Jan 7, 2026
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Abstract

While two-photon Hong-Ou-Mandel interference visibility has become a standard metric for single-photon sources, many optical quantum technologies require the generation and manipulation of larger photonic states. To date, efficiency limitations have prevented scaling quantum dot-based interference to the coalescence of more than two photons at a single beamsplitter. We overcome this limitation by combining a state-of-the-art quantum dot source with deterministic demultiplexing, enabling the direct observation of quantum interference fringes arising from up to four photons. We measure high mean interference contrasts of $93.0 \pm 0.1~\%$ for two photons, and $84.1 \pm 1.0~\%$ for four photons, with the complex fringe structure fully reproduced by a theoretical model. These results reveal the existence of "deep fringes" whose minima are unaffected by distinguishable photons, rendering the maximum contrast of four-photon interference highly sensitive to multi-photon emission but robust against photon distinguishability. We predict that these phenomena will extend to interference of larger numbers of photons, with relevance across a range of potential optical quantum technologies. A Fisher information analysis demonstrates that interference fringes from our source can exhibit phase sensitivity beyond the standard quantum limit, illustrating potential applications in quantum metrology.

Comments
Main manuscript (25 pages, 4 figures), followed by supplementary material (17 pages, 5 figures)

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While two-photon Hong-Ou-Mandel interference visibility has become a standard metric for single-photon sources, many optical quantum technologies require the generation and manipulation of larger photonic states. To date, efficiency limitations have prevented scaling quantum dot-based interference to the coalescence of more than two photons at a single beamsplitter. We overcome this limitation by combining a state-of-the-art quantum dot source with deterministic demultiplexing, enabling the direct observation of quantum interference fringes arising from up to four photons. We measure high mean interference contrasts of 93.0±0.1 %93.0 \pm 0.1~\%93.0±0.1 % for two photons, and 84.1±1.0 %84.1 \pm 1.0~\%84.1±1.0 % for four photons, with the complex fringe structure fully reproduced by a theoretical model. These results reveal the existence of "deep fringes" whose minima are unaffected by distinguishable photons, rendering the maximum contrast of four-photon interference highly sensitive to multi-photon emission but robust against photon distinguishability. We predict that these phenomena will extend to interference of larger numbers of photons, with relevance across a range of potential optical quantum technologies. A Fisher information analysis demonstrates that interference fringes from our source can exhibit phase sensitivity beyond the standard quantum limit, illustrating potential applications in quantum metrology.
Abstract Quantum interference is known to become extinct with distinguishing information, as illustrated by the ubiquitous double-slit experiment or the two-photon Hong–Ou–Mandel effect. In the former case single particle interference is destroyed with which-path information while in the latter bunching interference tails-off as photons become distinguishable. It has been observed that when more than two particles are involved, these interference patterns are in general a non-monotonic function of the distinguishability. Here we perform a comprehensive characterization, both theoretically and experimentally, of four-photon interference by analyzing the corresponding correlation functions, contemplating several degrees of distinguishability across different parameters. This study provides all the necessary tools to quantify the impact of multi-photon interference on precision measurements of parameters such as phase, frequency, and time difference. We apply these insights to quantify the precision in the estimation of an interferometric phase in a two-port interferometer using a four-photon state. Our results reveal that, for certain phase values, partially distinguishable multi-photon states can achieve higher Fisher information values compared to the two-photon experiment. These findings highlight the potential of distinguishable multi-photon states for enhanced precision in quantum metrology and related applications.
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Quantum metrology promises greater sensitivity for optical phase measurements than could ever be achieved classically. Here, we present a theory of the phase sensitivity for the general case where the detection probability is given by an N photon interference fringe. We find that the phase sensitivity has a complicated dependence on both the intrinsic efficiency of detection η and the interference fringe visibility V . Most importantly, the phase that gives maximum phase sensitivity is in general not the same as the phase at which the slope of the interference fringe is a maximum, as has previously been assumed. We determine the parameter range where quantum enhanced sensitivity can be achieved. In order to illustrate these theoretical results, we perform a four-photon experiment with η=3/4 and V =82±6% (an extension of our previous work (Nagata et al 2007 Science 316 726)) and find a phase sensitivity 1.3 times greater than the standard quantum limit at a phase different to that which gives maximum slope of the interference fringe.
Quantum entanglement can help to increase the precision of optical phase measurements beyond the standard quantum limit (SQL) to the ultimate Heisenberg limit [1, 2]. However, the N-photon parity measurements required to achieve this optimal sensitivity are extremely difficult to realize with current photon detection technologies, requiring high-fidelity resolution of N + 1 different photon distributions between the output ports. Recent experimental demonstrations of precision beyond the SQL for two[3–5] and four[6–9] photons have therefore used only one or two photon-number detection patterns instead of parity measurements. Here we investigate the achievable phase sensitivity of the simple and efficient single interference fringe detection technique. We show that the maximally-entangled NOON[10] state does not achieve optimal phase sensitivity when N > 4, rather, the Holland-Burnett state[11] is optimal. We experimentally demonstrate this enhanced sensitivity using a single photon-counted fringe of the six-photon Holland-Burnett state. Specifically, our single-fringe six-photon measurement achieves a phase variance three times below the SQL.
We demonstrate optical interferometry beyond the limits imposed by the photon wavelength using 'triggered' entangled photon pairs from a semiconductor quantum dot. Interference fringes of the entangled biphoton state reveals a periodicity half of that obtained with the single photon, and much less than that of the pump laser. High fringe visibility indicates that biphoton interference is less sensitive to decoherence than interference of two sequential single photons. The results suggest that quantum interferometry may be possible using a semiconductor LED-like device. (C) 2007 Optical Society of America
We demonstrate optical interferometry beyond the limits imposed by the photon wavelength using 'triggered' entangled photon pairs from a semiconductor quantum dot. Interference fringes of the entangled biphoton state reveals a periodicity half of that obtained with the single photon, and much less than that of the pump laser. High fringe visibility indicates that biphoton interference is less sensitive to decoherence than interference of two sequential single photons. The results suggest that quantum interferometry may be possible using a semiconductor LED-like device.