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arXiv:2512.24053 · ACS Photonics

Entangled photon triplets using lithium niobate nanophotonics

Nathan A. Harper, Ayantika Sengupta, Emily Y. Hwang, Scott K. Cushing

quant-phSubmitted Dec 30, 2025• Announced Dec 31, 2025• 0 citations
v1 · Dec 30, 2025v2 · Jan 7, 2026
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Abstract

Multiphoton states are needed for quantum communication and computation. Multiphoton states are significantly more difficult to generate than one- and two-photon states because two individual down-conversion processes must be cascaded. Only efficiencies of $<100$ Hz/mW have been reported to date. We integrate two down-converters on the same thin-film lithium niobate waveguide, significantly enhancing the cascaded process efficiency to $237 \pm 36$ kHz/mW. The measured $4.4\times10^{-5}$ probability of the second down-converter, which sets the limit on detectable triplet rates, exceeds those of previous triplet sources by an order of magnitude and demonstrates a path towards MHz rates of triplets for quantum applications.

Comments
Main text: 11 pages, 3 figures; Supplementary Material: 11 pages, 8 figures

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Multiphoton states are needed for quantum communication and computation. Multiphoton states are significantly more difficult to generate than one- and two-photon states because two individual down-conversion processes must be cascaded. Only efficiencies of <100<100<100 Hz/mW have been reported to date. We integrate two down-converters on the same thin-film lithium niobate waveguide, significantly enhancing the cascaded process efficiency to 237±36237 \pm 36237±36 kHz/mW. The measured 4.4×10−54.4\times10^{-5}4.4×10−5 probability of the second down-converter, which sets the limit on detectable triplet rates, exceeds those of previous triplet sources by an order of magnitude and demonstrates a path towards MHz rates of triplets for quantum applications.
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Abstract Integrated photon-pair sources are crucial for scalable photonic quantum systems. Thin-film lithium niobate is a promising platform for on-chip photon-pair generation through spontaneous parametric down-conversion (SPDC). However, the device implementation faces practical challenges. Periodically poled lithium niobate (PPLN), despite enabling flexible quasi-phase matching, suffers from poor fabrication reliability and device repeatability, while conventional modal phase matching (MPM) methods yield limited efficiencies due to inadequate mode overlaps. Here, we introduce a layer-poled lithium niobate (LPLN) nanophotonic waveguide for efficient photon-pair generation. It leverages layer-wise polarity inversion through electrical poling to break spatial symmetry and significantly enhance nonlinear interactions for MPM, achieving a notable normalized second-harmonic generation (SHG) conversion efficiency of 4615% W-1 cm-2. Through a cascaded SHG and SPDC process, we demonstrate photon-pair generation with a normalized brightness of 3.1×106 Hz nm-1 mW-2 in a 3.3 mm long LPLN waveguide, surpassing existing on-chip sources under similar operating configurations. Crucially, our LPLN waveguides offer enhanced fabrication reliability and reduced sensitivity to geometric variations and temperature fluctuations compared to PPLN devices. We expect LPLN to become a promising solution for on-chip nonlinear wavelength conversion and non-classical light generation, with immediate applications in quantum communication, networking, and on-chip photonic quantum information processing.
We report on multiphoton statistics of correlated twin beams produced in a periodic poled microring resonator on thin-film lithium niobate. Owing to high-cavity confinement and near-perfect quasi-phase-matching, the photon pairs are produced efficiently in single modes at rates reaching 27 MHz per $\text{\ensuremath{\mu}}\mathrm{W}$ pump power. By using a pump laser whose pulse-width impedance matches with the cavity, those photons are further created in single longitudinal modes with purity reaching 99%, without relying on later-on filtering. With a dual-channel photon-number-resolving detection system, we obtain directly the joint detection probabilities of multiphoton states up to three photons, with high coincidence to accidental contrast for each. Used as a single-photon source, it gives heralded gH(2)(0){g}_{H}^{(2)}(0)gH(2)​(0) around 0.04 at a single-photon rate of 650 kHz on chip. The findings of our research highlight the potential of this nanophotonic platform as a promising platform for generating nonclassical, few-photon states with ideal indistinguishability, for fundamental quantum optics studies and information applications.
Entangled photon pairs generated by a low-power continuous-wave laser could replicate pulsed laser-based tabletop spectroscopy by taking advantage of the inherent quantum correlations between the photons. Much of the current work in the thin-film lithium niobate platform has focused on infrared wavelengths, leaving shorter wavelengths still a largely unexplored space, particularly for spectroscopy. In this work, we have fabricated periodically poled lithium niobate nanophotonic waveguides for entangled photon generation through spontaneous parametric downconversion with a visible pump (406 nm). Characterization of the waveguided pair source confirms the spectral and temporal correlations of energy-time entangled photons with an on-chip pair generation efficiency of (2.3 ± 0.5) × 1011 pairs/s/mW, brightness of (1.6 ± 0.3) × 109 pairs/s/mW/nm, and two-photon interference visibility greater than 99%. With the same material platform, we have also demonstrated second harmonic generation with on-chip powers up to 30 μW and wavelengths as low as 355 nm, demonstrating lithium niobate's potential for ultraviolet nonlinear photonics and frequency doubling in the UV-A spectral region. Through design of larger cross-section waveguides, we have also explored how variations in the lithium niobate thin film thickness can affect quasi-phase matching. To date, this is the first reported demonstration of periodically poled lithium niobate nanophotonic waveguides for spontaneous parametric downconversion at a fully visible pump wavelength (406 nm) as well as second harmonic generation in the UV (355 nm). Future work towards fully on-chip spectroscopy will explore integrating an on-chip Mach-Zehnder interferometer with the entangled photon source.