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arXiv:2512.15051

Microscopic model for a spatial multimode generation based on Multi-pump Four Wave Mixing in hot vapours

H. M. Florez

quant-phSubmitted Dec 17, 2025• Announced Dec 18, 2025• 0 citations
arXivHTMLPDF

Abstract

Multipartite entanglement is an important resource for quantum information processing. It has been shown that it is possible to employ alkali atoms to implement single device multipartite entanglement by using nonlinear processes with spatial modes. This work presents the first microscopic description of such multi-mode generation with two-pump four wave mixing (4WM) in dense atomic media. We implement an extension of a double $Λ$ model for a single pump 4WM in order to describe the multi-mode generation with a two-pump configuration. We propose a Floquet expansion to solve the multimode gain amplification and noise properties. The model describes the angle and the two-photon dependency of the multimode generation and the quantum correlations among the modes. We investigate the entanglement properties of the system, describing the main properties of previous experimental observations. Such a microscopic description can be used to predict the gain distribution of modes and the quantum correlation within a typical range of experimental parameters.

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Multipartite entanglement is an important resource for quantum information processing. It has been shown that it is possible to employ alkali atoms to implement single device multipartite entanglement by using nonlinear processes with spatial modes. This work presents the first microscopic description of such multi-mode generation with two-pump four wave mixing (4WM) in dense atomic media. We implement an extension of a double ΛΛΛ model for a single pump 4WM in order to describe the multi-mode generation with a two-pump configuration. We propose a Floquet expansion to solve the multimode gain amplification and noise properties. The model describes the angle and the two-photon dependency of the multimode generation and the quantum correlations among the modes. We investigate the entanglement properties of the system, describing the main properties of previous experimental observations. Such a microscopic description can be used to predict the gain distribution of modes and the quantum correlation within a typical range of experimental parameters.
Multimode quantum states, such as multipartite quantum entanglement or quantum correlations, are important for both fundamental science and the future development of quantum technologies. Here we theoretically propose and experimentally realize a scheme that can fully exploit the multi-spatial-mode nature of the four-wave-mixing (FWM) process, i.e., spatial multiplexing, and thus integrates multiple FWM processes into a single cell at each stage of the cascaded process. The number of generated quantum-correlated beams 2n{2}^{n}2n is exponentially dependent on the number of vapor cells nnn. In addition, the quantum correlations between the multiple beams also increase as the number of vapor cell increases. For the case of n=2n=2n=2, we experimentally show that the degree of intensity-difference squeezing between the four quantum-correlated beams in our scheme is enhanced to $\ensuremath{-}8.2\ifmmode\pm\else\textpm\fi{}0.2$ dB from $\ensuremath{-}5.6\ifmmode\pm\else\textpm\fi{}0.3$ and $\ensuremath{-}6.5\ifmmode\pm\else\textpm\fi{}0.2$ dB of squeezing obtained with a single FWM process. Our system may find applications in quantum information and precision measurement.
Multimode quantum resources or states, in which quantum correlations are shared and distributed among multiple parties, are important not only for fundamental tests of quantum effects but also for their numerous possible applications in quantum technologies, such as quantum imaging and quantum metrology. Here we demonstrate the single-step fabrication of a multimode quantum resource from four-wave mixing (FWM) process in hot Rb vapor using a spatially structured pump, which consists of a coherent combination of two tilted pump beams. During this FWM process, one probe beam is amplified, three conjugate and two new probe beams are generated. The measured degrees of the intensity squeezing for the four-beam case and six-beam case are around $\ensuremath{-}4.1\ifmmode\pm\else\textpm\fi{}0.1$ dB and $\ensuremath{-}4.7\ifmmode\pm\else\textpm\fi{}0.1$ dB, respectively. The generated multiple quantum correlated beams are naturally separated with distinct directions, which is crucial for sending them out to quantum nodes at different locations in quantum communication. Our scheme is compact, simple, phase insensitive, and easily scalable to larger number of quantum-correlated modes.
Extensive attention has been drawn in generating multimode quantum states in recent years. Many efforts have been made during the last decade to produce such states. In this paper, we have experimentally demonstrated a scheme for generating a multi-spatial-mode quantum light source by a non-degenerated four-wave mixing process with a conical pump and a conical probe in a hot atomic vapor cell. The degree of the intensity-difference squeezing between the generated twin beams is about −4.1 dB. Due to the similar conical shape of the concentric quantum correlated beams, both the amplified probe and the generated conjugate beams can be decomposed into many angular modes. We have also experimentally verified the multi-spatial-mode nature of the generated quantum correlation by comparing the noise levels' variation tendencies of global attenuation and local cutting attenuations. In addition, we have also found the optimal values of each parameter in this scheme for further applications. Due to our scheme's advantages such as compactness, phase-insensitivity, and easy scalability, we have already shown a promising candidate for generating multi-spatial-mode quantum states, which may find potential applications in quantum metrology and quantum imaging, such as quantum-enhanced superresolution and the generation of multiple quantum correlated images.
Abstract We report the quantum correlated triple beams via cascaded four-wave mixing (CFWM) amplified in single hot atomic vapor. Experimentally, we show that strong quantum correlation of three light beams, among them any two’s quantum correlation is characterized by the maximum value of intensity-difference squeezing (IDS) about −7.8 ± 0.3 dB. We found there is IDS between two idler beams, because two pairs of Einstein–Podolsky–Rosen injections potentially exist in our system. Besides, CFWM can emit three-mode beams at three different frequencies, in which these beams can be well separated in the spatial domain. Moreover, much difference with other methods, the injecting probe field can manipulate the gain and IDS of output three-mode light beams, which is resulting from competition relationship between cascaded two four-wave mixing processes. More interestingly, Autler–Townes splitting of gain peaks of output signals due to dressing effect of pumping fields, will lead to the evolution of measured two- and three-mode IDS from single-mode to multi-mode at frequency domain. This result will provide a multimode quantum resource which can potentially realize multimode entanglement and quantum networks.
The frequency and spatial multimode of correlated fields are seen as essential resources for future multimode entanglement and quantum networks. Here, we present multimode properties from the process of parametric amplified cascaded four-wave mixing through a rubidium atomic ensemble under dressing and Kerr nonlinear effects. The experimental results complement the theoretical simulations. Three frequency modes and 34 spatial spots were experimentally observed due to the double-dressing and Kerr effect of the two pump fields. Further, it is verified that changing the pump field frequency has a larger line shift over pump field power and the angle between the two pump fields, which can be realized as a multicontact switch. Through a dressing effect, interestingly the number of coherent channels also increases by the order of dressing, indicating a large possibility of frequency and spatial multimode. These results will have important applications in quantum communications.
The nonlinear parametric process is of great significance for achieving high-quality coherent optical signals and quantum correlated photons. With the development of classical and quantum information processing, the study of the properties of parametric processes is evolving in complex scenarios of multimode, which is limited in conventional nonlinear media due to strict phase matching, e.g. nonlinear crystals. Here we study the dressing-energy-level-cascaded four-wave mixing process to generate multimode optical parametric signals. Via cascading double-Λ type configuration of 85 Rb D 1 line, the non-degenerate energy-level-cascaded FWM is constructed to generate multimode self-parametric amplification. Moreover, with the dressing effects based on atomic coherence, the spatial and frequency multimode characteristics of energy-level-cascaded FWM parametric amplification, i.e., the modes number and pattern, are actively modulated by the pump fields detuning. Also, the spatial modes from the coupling of two coexisting spontaneous parametric FWMs can be controlled to reach tremendous scalability via the atomic coherence and Kerr non-linearity. The atomic coherence effects and unique phase-matching symmetry nature allow flexible modulation of the multimode property of the generated parametric signals within a nonlinear device, which paves a way for multimode classical and quantum information processing.