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arXiv:2511.22413

Entanglement gain in supercatalytic state transformations

Guillermo Díez-Pastor, Julio I. de Vicente

quant-phSubmitted Nov 27, 2025• Announced Nov 28, 2025• 0 citations
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Abstract

Catalysis refers to the possibility of performing an otherwise impossible local state transformation by sharing an additional state, i.e. a catalyst, which is returned at the end of the protocol. There is a stronger version, known as supercatalysis, in which the borrowed catalyst is returned in an enhanced form, i.e. more entangled. However, this phenomenon has remained little explored. In this work we introduce the supercatalytic entanglement gain as a figure of merit taking values in [0,1] that quantifies the performance of the protocol (with 0 corresponding to the standard case of catalysis and 1 representing the maximal possible gain) and we study in which cases it can be greater than zero and which strategies can maximize it. While it turns out that every catalytic transformation can be implemented in a supercatalytic fashion with entanglement gain equal to 1 if the state that is borrowed is chosen appropriately, other choices can make the gain strictly less than 1 and even 0. In fact, we prove that a large class of catalytic transformations are not fully supercatalyzable, i.e. there is at least one choice of catalyst for which the entanglement gain vanishes. On the other hand, the construction that shows that supercatalysis is always possible with maximal gain uses artificially highly entangled catalysts. For this reason, we also study minimal supercatalysis, where the entanglement content of the borrowed state is constrained in a precise and natural way. While we consider a scenario where we prove it is impossible to have entanglement gain equal to 1 in this case, we show that there exist minimal supercatalytic transformations with gain as close to 1 as desired. We also explore several examples and observe that, although choosing a catalyst with the least possible entanglement is often an optimal strategy for minimal supercatalysis, this is not necessarily always the case.

Comments
17 pages, 5 figures

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Catalysis refers to the possibility of performing an otherwise impossible local state transformation by sharing an additional state, i.e. a catalyst, which is returned at the end of the protocol. There is a stronger version, known as supercatalysis, in which the borrowed catalyst is returned in an enhanced form, i.e. more entangled. However, this phenomenon has remained little explored. In this work we introduce the supercatalytic entanglement gain as a figure of merit taking values in [0,1] that quantifies the performance of the protocol (with 0 corresponding to the standard case of catalysis and 1 representing the maximal possible gain) and we study in which cases it can be greater than zero and which strategies can maximize it. While it turns out that every catalytic transformation can be implemented in a supercatalytic fashion with entanglement gain equal to 1 if the state that is borrowed is chosen appropriately, other choices can make the gain strictly less than 1 and even 0. In fact, we prove that a large class of catalytic transformations are not fully supercatalyzable, i.e. there is at least one choice of catalyst for which the entanglement gain vanishes. On the other hand, the construction that shows that supercatalysis is always possible with maximal gain uses artificially highly entangled catalysts. For this reason, we also study minimal supercatalysis, where the entanglement content of the borrowed state is constrained in a precise and natural way. While we consider a scenario where we prove it is impossible to have entanglement gain equal to 1 in this case, we show that there exist minimal supercatalytic transformations with gain as close to 1 as desired. We also explore several examples and observe that, although choosing a catalyst with the least possible entanglement is often an optimal strategy for minimal supercatalysis, this is not necessarily always the case.
Entanglement is a key quantum resource in various quantum protocols, with a rich set of laws governing its manipulation. In this context, catalysis refers to the possibility of an auxiliary state that enables a previously forbidden manipulation, while being completely returned at the end. While the catalytic setting has been thoroughly examined in the single-copy regime, much less is known in the asymptotically many copy regime. In this work, we focus on the entanglement cost of preparing asymptotically many copies of a given state exactly. We show that catalysis can significantly lower the exact entanglement cost by constructing an explicit catalytic protocol. Additionally, these findings generalize readily to other resource theories, showing a general catalytic advantage in the resource dilution task.
Quantum catalysis, the ability to enable previously impossible transformations by using auxiliary systems without degrading them, has emerged as a powerful tool in various resource theories. Although catalytically enabled state transformations have been formally characterized by the monotonic behavior of entropic quantifiers (e.g., the von Neumann entropy or nonequilibrium free energy), such characterizations often rely on unphysical assumptions, namely, the ability of using catalysts of infinitely large dimension. This approach offers very limited insights into the practical significance of using catalysis for quantum information processing. Here, we address this problem across a broad class of quantum resource theories. Leveraging quantum information tools beyond the asymptotic regime, we establish sufficient conditions for the existence of catalytic transformations with finite-size catalysts. We further unveil connections between finite-size catalysis and multicopy transformations. Notably, we discover a phenomenon of catalytic resonance: by carefully tailoring the catalysts's state, one can drastically reduce the required dimension of the catalyst, thus enabling efficient catalytic transformations with minimal resources. Finally, we illustrate our findings with examples from the resource theories of entanglement and thermodynamics, as well in the context of catalytic unitary transformations.
Quantum catalysts can overcome otherwise impossible quantum state transformations without being consumed, and allowing them to become correlated with the output makes this assistance substantially more powerful. This raises a fundamental question for entanglement theory: which limitations on state manipulation remain when such correlated catalysts are freely available? We answer this question in the positive-partial-transpose (PPT) resource theory, which allows a substantially broader class of operations than local operations and classical communication (LOCC). We identify general conditions under which regularized relative-entropy measures become strongly superadditive, and use them to construct monotones that constrain correlated catalytic PPT transformations without any knowledge of the catalyst. In particular, we prove that the regularized PPT relative entropy is fully additive and strongly superadditive, resolving an open problem in entanglement theory. Most importantly, these constraints show that even arbitrary correlated catalysts cannot restore asymptotic reversibility: for an explicit state, the optimal entanglement distillation rate remains strictly smaller than the entanglement cost. Thus, substantial catalytic assistance does not remove some of the fundamental limitations of mixed-state entanglement manipulation.
Understanding the fundamental limits of state convertibility is crucial for establishing the boundaries of quantum information processing and thermodynamic efficiency. While auxiliary systems, catalysts, can facilitate otherwise impossible transformations, standard catalysis rigidly requires the auxiliary system to return to its exact initial state. In this work, we investigate the power of flexible catalysis, where the catalyst evolves through a cycle of states, restoring its initial configuration only after a finite number of steps. Focusing on the regime of fixed, finite dimensions, we analyze the capabilities of flexible catalysis within the resource theories of entanglement and quantum thermodynamics. In the context of entanglement, we derive conditions limiting flexible catalysts, yet show that flexible catalysis can be strictly more powerful than same-dimensional standard catalysis: it enables deterministic transformations achievable by no standard catalyst of the same dimension, and it strictly increases the success probability of stochastic local operations and classical communication. A similar deterministic advantage arises in quantum thermodynamics, where flexible catalysis enables state transformations that are impossible with any standard catalyst of fixed dimension and Hamiltonian but become achievable via flexible catalysis.
The correlations of certain entangled states can be perfectly simulated classically via a local model. Hence such states are termed Bell local, as they cannot lead to Bell inequality violation. Here, we show that Bell nonlocality can nevertheless be activated for certain Bell-local states via a catalytic process. Specifically, we present a protocol where a Bell-local state, combined with a catalyst, is transformed into a Bell-nonlocal state while the catalyst is returned exactly in its initial state. Importantly, this transformation is deterministic and based only on local operations. Moreover, this procedure is possible even when the state of the catalyst is itself Bell local, demonstrating a new form of superactivation of Bell nonlocality, as well as an interesting form of quantum catalysis. On the technical level, our main tool is a formal connection between catalytic activation and many-copy activation.
Abstract In chemistry, a catalyst is a substance which enables a chemical reaction or increases its rate, while remaining unchanged in the process. Instead of chemical reactions, quantum catalysis enhances our ability to convert quantum states into each other under physical constraints. The nature of the constraints depends on the problem under study and can arise, e.g. from energy preservation. This article reviews the most recent developments in quantum catalysis and gives a historical overview of this research direction. We focus on the catalysis of quantum entanglement and coherence, and also discuss this phenomenon in quantum thermodynamics and general quantum resource theories. We review applications of quantum catalysis and also discuss the recent efforts on universal catalysis, where the quantum state of the catalyst does not depend on the states to be transformed. Catalytic embezzling is also considered, a phenomenon that occurs if the catalyst’s state can change in the transition.