Microwave spectroscopy of few-carrier states in bilayer graphene quantum dots
Max J. Ruckriegel, Christoph Adam, Rebecca Bolt, Chuyao Tong, David Kealhofer, Artem O. Denisov, Mohsen Bahrami Panah, Kenji Watanabe, Takashi Taniguchi, Thomas Ihn, Klaus Ensslin
cond-mat.mes-hallquant-phSubmitted Nov 25, 2025• Announced Nov 26, 2025
Bilayer graphene is a maturing material platform for gate-defined quantum dots that hosts long-lived spin and valley states. Implementing solid-state qubits in bilayer graphene requires a fundamental understanding of such confined electronic systems. In particular, states of two and three carriers, for which the exchange interaction between particles plays a crucial role, are a cornerstone for qubit readout and manipulation. Here we report on the spectroscopy of few-carrier states in bilayer graphene quantum dots, using circuit quantum electrodynamics (cQED) techniques that offer substantially improved energy resolution compared to standard transport techniques. Measurements using a superconducting high-impedance resonator capacitively coupled to the double quantum dot reveal dispersive features of two and three electron states, enabling the detection of Pauli spin and valley blockade and the characterization of the spin-orbit gap at zero magnetic field. The results deepen our understanding of few-carrier spin and valley states in bilayer graphene quantum dots and demonstrate that cQED techniques are a powerful state-selective probe for semiconductor nanostructures.
Bilayer graphene is a maturing material platform for gate-defined quantum dots that hosts long-lived spin and valley states. Implementing solid-state qubits in bilayer graphene requires a fundamental understanding of such confined electronic systems. In particular, states of two and three carriers, for which the exchange interaction between particles plays a crucial role, are a cornerstone for qubit readout and manipulation. Here we report on the spectroscopy of few-carrier states in bilayer graphene quantum dots, using circuit quantum electrodynamics (cQED) techniques that offer substantially improved energy resolution compared to standard transport techniques. Measurements using a superconducting high-impedance resonator capacitively coupled to the double quantum dot reveal dispersive features of two and three electron states, enabling the detection of Pauli spin and valley blockade and the characterization of the spin-orbit gap at zero magnetic field. The results deepen our understanding of few-carrier spin and valley states in bilayer graphene quantum dots and demonstrate that cQED techniques are a powerful state-selective probe for semiconductor nanostructures.
High Resolution Image Download MS PowerPoint Slide We implement circuit quantum electrodynamics (cQED) with quantum dots in bilayer graphene, a maturing material platform that can host long-lived spin and valley states. Our device combines a high-impedance ( Z r ≈ 1 kΩ) superconducting microwave resonator with a double quantum dot electrostatically defined in a graphene-based van der Waals heterostructure. Electric dipole coupling between the subsystems allows the resonator to sense the electric susceptibility of the double quantum dot from which we reconstruct its charge stability diagram. We achieve sensitive and fast detection of the interdot transition with a signal-to-noise ratio of 3.5 within 1 μs integration time. The charge–photon interaction is quantified in the dispersive and resonant regimes by comparing the resonator response to input–output theory, yielding a coupling strength of g /2π = 49.7 MHz. Our results introduce cQED as a probe for quantum dots in van der Waals materials and indicate a path toward coherent charge–photon coupling with bilayer graphene quantum dots.
Charge noise is an important factor limiting qubit coherence and relaxation in solid-state devices. In bilayer graphene (BLG) quantum dots, recently established as a promising platform for spin- and valley-based qubits, both the origin and magnitude of charge noise remain largely unexplored. Here, we investigate high-frequency charge noise using Landau-Zener-Stückelberg-Majorana (LZSM) interference spectroscopy. We study a single-particle charge qubit formed in a BLG double quantum dot at frequencies between 5 and 10 GHz and extract a noise spectral density Sε on the order of 0.5-0.9 neV/Hz. This is comparable to values reported for III-V semiconductor platforms and silicon. From the temperature and frequency dependence of the charge qubit decoherence, we conclude that thermal (Johnson) noise or electron-phonon coupling dominates over two-level fluctuators.
Bilayer graphene (BLG) quantum dots (QDs) are a promising platform for semiconductor qubits. However, the low-frequency charge noise that may ultimately limit coherence has remained largely unexplored. Here, we systematically characterize charge noise in gate-defined BLG QDs using transport-based noise spectroscopy. We extract a median amplitude of $ S_μ^{1/2} (1~\text{Hz}) = 1.16~μ\text{eV}/\sqrt{\text{Hz}}$, placing BLG well within the range reported for established semiconductor quantum-dot platforms. Across variations in charge occupation, confinement, source-drain bias, and charge-sensor operating conditions, neither the noise amplitude nor the spectral dependence shows a reproducible trend in electrostatic tuning, indicating that we extracted the intrinsic semiconductor noise. Consistent noise levels are further observed in double QDs and confirmed using an independent superconducting resonator-based dispersive readout. Extending the study to BLG devices incorporating transition metal dichalcogenide layers reveals no measurable charge noise increase in weakly proximitized QDs. These results validate BLG as a viable platform for coherent quantum information processing.
Spin qubits in semiconductor quantum dots constitute one of the leading platforms for quantum information processing, combining long coherence times, high-fidelity gate operations, and compatibility with semiconductor industry technologies. In particular, holes confined in planar Ge/SiGe heterostructures have recently emerged as promising qubit candidates owing to their low effective mass, high mobility, low percolation density, absence of valley states, and strong spin-orbit interaction, which enables fast all-electrical spin control. At the same time, spin-orbit interaction also gives rise to a highly anisotropic and electrically tunable gyromagnetic response. Understanding and controlling this response is therefore essential for high-fidelity single- and multi-qubit operations. The realization of scalable quantum processors also requires efficient qubit readout and long-range connectivity. Circuit quantum electrodynamics (cQED), based on the coupling between artificial atoms and microwave photons confined in superconducting resonators, provides a natural framework to address these challenges. However, the implementation of hybrid semiconductor-superconductor devices in planar Ge has so far been hindered by large microwave losses originating from the heterostructure. In this thesis, we demonstrate, for the first time in planar Ge, strong coupling between a hole charge qubit in a double quantum dot and a high-impedance microwave resonator, reaching a cooperativity of C â 100. In addition, we leverage the frequency tunability of the resonator to perform detailed spectroscopy of a multi-level energy spectrum of low-lying states arising from strong Coulomb-correlation effects. To further improve the quality of the hole-photon interface, we investigate the source of microwave losses in different Ge/SiGe heterostructures, identifying defects at the lattice-mismatched Si/Ge interface as the dominant source of resonator losses in reverse-graded heterostructures. To mitigate this limitation, a deep tapered-etching approach is introduced, enabling the fabrication of superconducting resonators directly on etched heterostructures. This method yields internal quality factors exceeding Qint > 10 000 for high-impedance Josephson junction array resonators and Qint > 100 000 for 50 â Nb resonators. Finally, this thesis explores the spin properties of multi-hole quantum dots beyond the conventional single-orbital picture. By reconstructing and electrically tuning the g tensors of holes confined in different orbital states, we show that confinement can substantially modify both their magnitude and orientation. These results open new opportunities for engineering qubit properties through orbital occupation. Furthermore, highly coherent singlet-triplet oscillations are demonstrated in the seven-hole regime, yielding a quality factor of approximately 330 at in-plane magnetic fields as low as 2.5 mT. Together, these results establish a foundation for high-fidelity hole-spin-qubit operation based on g-tensor engineering and for the integration of planar Ge quantum dots with superconducting quantum circuits.
Semiconductor qubits rely on the control of charge and spin degrees of freedom of electrons or holes confined in quantum dots (QDs). Typically, semiconductor qubit-qubit coupling is short range, effectively limiting qubit distance to the spatial extent of the wavefunction of the confined particle (a few hundred nanometers). This is a significant constraint towards scaling of QD-based architectures to realize dense 1D or 2D arrays of QDs. Inspired by techniques originally developed for circuit QED, we recently demonstrated the strong coupling of individual electrons confined in GaAs quantum dots to individual microwave photons, making use of the enhanced electric component of the vacuum fluctuations of a resonator with impedance beyond the typical 50 Ohm of standard coplanar waveguides. In this hybrid technology, we recently realized a proof of concept experiment, where the coupling between a transmon and a double QD (DQD) is mediated by virtual microwave photon excitations in a high impedance SQUID array resonator, which acts as a quantum bus enabling long-range coupling between dissimilar qubits. Similarly, we achieved coherent coupling between two DQD charge qubits separated by approximately 50 um. In the dispersive regime, we spectroscopically observed qubit-qubit coupling as an avoided-crossing in the energy spectrum of the DQD charge qubits. The methods and techniques developed in this work are transferable to QD devices based on other material systems and can be beneficial for spin based hybrid systems.
As an application in circuit quantum electrodynamics coupled systems, superconducting resonators play an important role in high-sensitivity measurements in a superconducting-semiconductor hybrid architecture. Taking advantage of a high-impedance $\mathrm{Nb}\text{\ensuremath{-}}\mathrm{Ti}\text{\ensuremath{-}}\mathrm{N}$ resonator, we perform excited-state spectroscopy on a GaAs double quantum dot (DQD) by applying voltage pulses to one gate electrode. The pulse train modulates the DQD energy detuning and gives rise to charge state transitions at zero detuning. Benefiting from the outstanding sensitivity of the resonator, we distinguish different spin-state transitions in the energy spectrum according to the Pauli exclusion principle. Furthermore, we experimentally study how the interdot tunneling rate modifies the resonator response. The experimental results are consistent with the simulated spectra based on our model.