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arXiv:2511.19801

Exciton collective modes in a bilayer of axion insulator $\text{MnBi}_2 \text{Te}_4$

Olivia Liebman, Jonathan B. Curtis, Emily Been, Prineha Narang

cond-mat.mtrl-scicond-mat.otherquant-phSubmitted Nov 25, 2025• Announced Nov 26, 2025
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Abstract

We investigate the emergence of an exciton condensate and associated collective modes in a bilayer configuration of $\text{MnBi}_2\text{Te}_4$, an antiferromagnetic topological insulator and van der Waals material, recognized for hosting axion physics. Utilizing a minimal low-energy Hamiltonian for the two layer system which is gapped by the intrinsic Néel order, we first employ mean-field theory to establish the conditions for exciton condensation. Our analysis identifies a nonzero, spin-singlet exciton order parameter which is tuned by external displacement field, temperature, and Coulomb attraction. Beyond the mean-field, we explore collective mode fluctuations in the uncondensed phase via many-body perturbation theory and the random phase approximation. From this, we derive the exciton spectral function which allows for a direct comparison between theoretical prediction and experimental observation. We detail how the softening of the collective mode peak is a function of the competition between interlayer detuning and thermal fluctuations. This work elucidates how the unique topological and magnetic environment of $\text{MnBi}_2\text{Te}_4$ offers a tunable platform for the realization and manipulation of exciton condensates and the corresponding collective excitations. Our findings contribute to understanding the interplay of topology and bosonic condensates, which could inspire application in optically accessing topological properties, dissipationless transport, and gate-tunable optoelectronics.

Comments
11 pages, 4 figures

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Exciton collective modes in a bilayer of axion insulator MnBi2Te4\text{MnBi}_2 \text{Te}_4MnBi2​Te4​
We investigate the emergence of an exciton condensate and associated collective modes in a bilayer configuration of MnBi2Te4\text{MnBi}_2\text{Te}_4MnBi2​Te4​, an antiferromagnetic topological insulator and van der Waals material, recognized for hosting axion physics. Utilizing a minimal low-energy Hamiltonian for the two layer system which is gapped by the intrinsic Néel order, we first employ mean-field theory to establish the conditions for exciton condensation. Our analysis identifies a nonzero, spin-singlet exciton order parameter which is tuned by external displacement field, temperature, and Coulomb attraction. Beyond the mean-field, we explore collective mode fluctuations in the uncondensed phase via many-body perturbation theory and the random phase approximation. From this, we derive the exciton spectral function which allows for a direct comparison between theoretical prediction and experimental observation. We detail how the softening of the collective mode peak is a function of the competition between interlayer detuning and thermal fluctuations. This work elucidates how the unique topological and magnetic environment of MnBi2Te4\text{MnBi}_2\text{Te}_4MnBi2​Te4​ offers a tunable platform for the realization and manipulation of exciton condensates and the corresponding collective excitations. Our findings contribute to understanding the interplay of topology and bosonic condensates, which could inspire application in optically accessing topological properties, dissipationless transport, and gate-tunable optoelectronics.
We investigate the nature of the magnetic excitations of a bilayer single-orbital Hubbard model in the intermediate-coupling regime.This model exhibits a quantum phase transition (QPT) between a paramagnetic (PM) and an insulating antiferromagnetic (AFM) phase at a critical value of the coupling strength.By using the random phase approximation, we show that the QPT is continuous when the PM state is a band insulator and that the corresponding quantum critical point (QCP) arises from the condensation of preformed excitons.These low-energy excitons re-emerge on the other side of the QCP as the transverse and longitudinal modes of the AFM state.In particular, the longitudinal mode remains sharp for the model parameters relevant to Sr 3 Ir 2 O 7 because of the strong easy-axis anisotropy of this material.
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We studied the possibility of exciton condensation in Mott insulating bilayers. In these strongly correlated systems, an exciton is the bound state of a double occupied and empty site. In the strong coupling limit, the exciton acts as a hard-core boson. Its physics is captured by the exciton ttt-JJJ model, containing an effective XXZXXZXXZ model describing the exciton dynamics only. Using numerical simulations and analytical mean-field theory, we constructed the ground-state phase diagram. Three homogeneous phases can be distinguished: the antiferromagnet, the exciton checkerboard crystal, and the exciton superfluid. For most model parameters, however, we predict macroscopic phase separation between these phases. The exciton superfluid exists only for large exciton hopping energy. Additionally, we studied the collective modes and susceptibilities of the three phases. In the superfluid phase, we find the striking feature that the bandwidth of the spin-triplet excitations, potentially detectable by resonant inelastic x-ray scattering (RIXS), is proportional to the superfluid density. The superfluid phase mode is visible in the charge susceptibility, measurable by RIXS or electron energy loss spectroscopy (EELS).
We formulated an effective theory for a single interlayer exciton in a bilayer quantum antiferromagnet, in the limit when the holon and doublon are strongly bound onto one interlayer rung by the Coulomb force. Upon using a rung linear spin-wave approximation of the bilayer Heisenberg model, we calculated the spectral function of the exciton for a wide range of the interlayer Heisenberg coupling α = J ⊥ / Jz . In the disordered phase at large α , a coherent quasi-particle peak appears, representing free motion of the exciton in a spin singlet background. In the Néel phase, which applies to more realistic model parameters, a ladder spectrum arises due to Ising confinement of the exciton. The exciton spectrum is visible in measurements of the dielectric function, such as c -axis optical conductivity measurements.
A topological Mott insulator (TMI) with spontaneous time-reversal symmetry breaking and nonzero Chern number has been discovered in a real-space effective model for twisted bilayer graphene (TBG) at 3/4 filling in the strong coupling limit [1]. However, the finite temperature properties of such a TMI state remain illusive. In this work, employing the state-of-the-art thermal tensor network and the perturbative field-theoretical approaches, we obtain the finite-T phase diagram and the dynamical properties of the TBG model. The phase diagram includes the quantum anomalous Hall and charge density wave phases at low T, and an Ising transition separating them from the high-T symmetric phases. Because of the proliferation of excitons-particle-hole bound states-the transitions take place at a significantly reduced temperature than the mean-field estimation. The exciton phase is accompanied with distinctive experimental signatures in such as in charge compressibilities and optical conductivities close to the transition. Our work explains the smearing of the many-electron state topology by proliferating excitons and opens an avenue for controlled many-body investigations on finite-temperature states in the TBG and other quantum moiré systems.
Topological phases of matter are purely quantum mechanical and have no classical analogue. Most phases in nature can be classified and studied classically through the concept of symmetry breaking and its theoretical description, Landau-Ginzburg field theory. In contrast to the general wisdom of Landau-Ginzburg field theory, the topological phases share the same symmetry as a trivial insulator and still are different phases. Having gapped spectrum in bulk, they support a metallic edge excition robust against symmetry-respecting perturbation or an emergent fractional excitation in bulk. Following after fractional quantum Hall fluids, many topologically orderd phases, such as spin liquids and topological insulators, have been found and studied. Spin liquids are disordered phases of frustrated antiferromagnets and do not freeze and order even at the lowest temperature. They support an electrically neutral spin-1/2 excitation, which does not exist in a microscopic scale, with emergent dynamical gauge field in bulk and do not have an adiabatic path to a trivial paramagnet phase. The topological insulators are time-reversal symmetric band insulators which cannot evolve smoothly into a trivial insulator with the symmetry, and they have been intensely studied theoretically and experimetally for the last decade. Though the topological insulators are inherently non-interacting systems, they have exotic gapless edge and surface states which demonstrate many interesting quantum phenomena such as fractionalization, axionic electromagnetism, and half quantum Hall effect. In this thesis, we study various quantum phenomena of the topological phases, mainly of the topological insulator and its close relatives in which the physics of spin liquids has been merged into. As they are intrinsically quantum many-body states, the quantum field theory is an invaluable tool to explore the venue of the phases and will be used thorougly in this work. First, we present a topological field theoretic description of the topological insulators and translational symmetric Z2 spin liquid. We demostrate that abelian BF theory is an effective field theory for the two and three dimensional topological insulators. We show that the phenomenologies of BF theory are consistent with those of the topological insulators such as gapless edge and surface excitations and response functions to external gauge field. The same form of the BF theory is also applicable to study the certain classes of Z2 spin liquids with the gapless edge states. We closely examine the possible gapless edge theory of the BF theory and the translational symmetric spin liquids, and we show that the effective BF theories capture the bulk properties as well as the gapless edge spectrum of the spin liquid. Also we discuss the zero-temperature phase diagram of a thin film three dimensional topological insulators with two competing mass terms: time-reversal symmetric exciton condensation and time-reversal symmetry breaking Zeeman effect. There are two phases, quantum spin Hall phase and quantum anomalous Hall phase, and both phases support fractional excitations. We derive an effective topological field theory for the fractional excitations and examine the origin of the fractional excitations. Next we consider the relatives of the topological insulators. First we discuss the proximate symmetry broken phases of topological Mott insulator, a U(1) spin liquid with fermionic spinons in the topological insulator state. The topologically non-trivial band structure of the spinon generates the axion term for the gauge field, and we show that the axion term changes the nature of the confined phase of the spin liquid. Contrast to the conventional confined phase which has only a bond order, the confined phase of the spin liquid is in general a coexisting phase of the two different orders : a current order and a bond order. We then consider another relative of the topological insulator: a bosonic symmetry protected topological phase in two dimensional space, with both PSU(N) and time reversal symmetry. We develop an effective field theory for the phase, which is a SU(N) principal chiral model with a theta-term, and reveal the physics of the topological phase in detail.Finally we consider a topological semimetal, namely a Weyl semimetal. We first demonstrate that the Weyl semimetal can be realized in the magnetically doped topological band insulators. We explicitly derive the low energy theory of Weyl points from the general continuum Hamiltonian and tight-binding model of the topological insulators. Then we study superconducting instabilities of doped Weyl semimetals. We consider a minimal model for a Weyl semimetal and study the superconducting instabilities induced by a short-ranged attractive interaction. With the interaction, we find two competing states: a fully gapped finite-momentum pairing state and a nodal even-parity pairing state. We show that, in a mean field approximateion, the finite-momentum pairing state wins energetically against the usual even-parity paired state. We also show that exotic modes are localized at the full and half quantum vortices of the finite-momentum pairing state.