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arXiv:2511.17749 · Physical Review Research

Entanglement Witnesses of Condensation for Enhanced Quantum Sensing

Lillian I. Payne Torres, Irma Avdic, Anna O. Schouten, Olivia C. Wedig, Gregory S. Engel, David A. Mazziotti

quant-phphysics.chem-phphysics.comp-phSubmitted Nov 21, 2025• Announced Nov 25, 2025• 1 citation• Revised Nov 25, 2025 (v2)
v1 · Nov 21, 2025v2 · Nov 25, 2025
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Abstract

Quantum phenomena such as entanglement provide powerful resources for enhancing classical sensing. Here, we theoretically show that collective entanglement of spin qubits, arising from a condensation of particle-hole pairs, can strongly amplify transitions between ground and excited spin states, potentially improving signal contrast in optically detected magnetic resonance. This collective state exhibits an $\mathcal{O}(\sqrt{N})$ enhancement of the transition amplitude with respect to an applied microwave field, where $N$ is the number of entangled spin qubits. We computationally realize this amplification using an ensemble of $N$ triplet spins with magnetic dipole interactions, where the largest transition amplitudes occur at geometries for which the condensation of particle-hole pairs is strongest. This effect, robust to noise, originates from the concentration of entanglement into a single collective mode, reflected in a large eigenvalue of the particle-hole reduced density matrix -- an entanglement witness of condensation analogous to off-diagonal long-range order, though realized here in a finite system. These results offer a design principle for quantum sensors that exploit condensation-inspired entanglement to boost sensitivity in spin-based platforms.

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Molecular quantum sensors represent a promising frontier for the detection of nuclear magnetic resonance signals and alternating current magnetic fields at the nanoscale, potentially reaching single-proton sensitivity. Although the triplet states T̂ of molecular pentacene provide a viable sensing architecture, the triplet pair states T̂T̂ produced by singlet fission of pentacene dimers could enable more flexible quantum manipulations through entanglement. In this work, we model the quantum sensing efficacy of a spin-polarized quintet manifold 5T̂T̂0,±1 in a photoexcited pentacene dimer generated via intramolecular singlet fission. Using a Lindblad master equation approach, we simulate the evolution of the triplet-pair state under standard dynamical decoupling sequences-including spin echo, XY4, and XY8-and provide a direct performance comparison to the traditional pentacene monomer benchmark. While both architectures exhibit comparable sensitivity for isolated single-spin detection, our findings indicate that the dimer architecture provides a superior interaction cross section for detecting small ensembles of nuclear spins. Analytical expressions derived for fluorescence modulation demonstrate that sensitivity is optimized in the low-magnetic field regime (≤0.01 T) and scales with the number of pulses in the sensing protocol. This study establishes a theoretical baseline for utilizing high-spin multi-excitonic states as chemically tunable, high-sensitivity quantum probes.
Abstract Quantum sensors that harness quantum coherence and entanglement are emerging as powerful tools in many fields, including particle physics, promising unprecedented sensitivity beyond classical detection methods. At the same time, electrons trapped on the surface of liquid helium have emerged as a promising quantum computing, and possibly sensing, platform owing to a nearly impurity-free environment and large predicted coherence times. In this context, single-electron confinement and control using microfabricated traps on helium has been experimentally demonstrated, highlighting the feasibility of scalable qubit architectures on this platform. Leveraging these features, and in line with CERN’s Detector R\&D Initiative 5 (DRD5) 1 on Quantum Sensors, we propose here a sensor concept that uses an entangled pair of electron qubits on superfluid helium for particle physics experiments. We outline the motivation for such spatially and spin-entangled sensors, develop the theoretical formalism for two electrons and their spins and spatial degrees of freedom in a helium-based double-well trap (analogous to a double quantum dot in semiconductor systems), and discuss the potential advantages for detecting rare high-energy events with quantum-enhanced sensitivity. By exploiting quantum entanglement between the two trapped electrons, this sensor concept can surpass classical sensitivity limits.
Ordered magnets harbor intrinsically squeezed ground states and magnonic excitations characterized by entanglement between spins and nonclassical magnon number composition. A pathway to detecting the superpositions of noneigenmode magnon number states underlying these nonclassical magnetic ground states has recently been demonstrated by utilizing a qubit coupled to the magnon mode via a direct dispersive interaction. Here, we theoretically develop this qubit spectroscopy further delineating the capabilities and limitations of this qubit spectroscopy for sensing the quantum superpositions that underlie the excited states. We demonstrate that the spectroscopy lends itself naturally to unraveling the superpositions that underlie the various quantized squeezed-magnon number states. However, excited states comprising superpositions of multiple squeezed Fock states become increasingly hard due to the large number of possible transitions, and resulting peaks, in the qubit spectroscopy thereby requiring qubits with narrower linewidths. Along the same lines, we theoretically demonstrate the qubit spectroscopy of a low amplitude coherent squeezed-magnon state analyzing the tradeoff between frequency crowding due to multiple transitions and peak linewidths. Our work lays the groundwork and design equations for deploying high-quality qubits towards sensing the composite nature of spin excitations in magnetic systems.