Creation and manipulation of non-classical states of light is rapidly becoming the focus of modern attosecond science. Here, we demonstrate numerically how interaction with such states can trigger the emergence of a many-body system with spontaneously broken symmetry by considering a modification of the well-known problem of superradiance encountered already by Dicke. Similarly to him, we investigate photon emission by ensembles of indistinguishable atoms. In contrast to him, however, we leverage symmetry-based selection rules to suppress emission of single photons by single atoms. A steady state is therefore only reached following a spontaneous transition into a collective symmetry-broken state of atoms and photonic modes. This transition permanently locks the atomic dipoles to the quantum field experienced by the system at a particular instant, transforming the entire setup into a potent quantum sensor reproducing the phase of the recorded quantum fluctuation.
Creation and manipulation of non-classical states of light is rapidly becoming the focus of modern attosecond science. Here, we demonstrate numerically how interaction with such states can trigger the emergence of a many-body system with spontaneously broken symmetry by considering a modification of the well-known problem of superradiance encountered already by Dicke. Similarly to him, we investigate photon emission by ensembles of indistinguishable atoms. In contrast to him, however, we leverage symmetry-based selection rules to suppress emission of single photons by single atoms. A steady state is therefore only reached following a spontaneous transition into a collective symmetry-broken state of atoms and photonic modes. This transition permanently locks the atomic dipoles to the quantum field experienced by the system at a particular instant, transforming the entire setup into a potent quantum sensor reproducing the phase of the recorded quantum fluctuation.
The many-body decay of extended collections of two-level systems remains an open problem. Here, we investigate whether an array of emitters coupled to a one-dimensional bath undergoes Dicke superradiance. This is a process whereby a completely inverted system becomes correlated via dissipation, leading to the release of all the energy in the form of a rapid photon burst. We derive the minimal conditions for the burst to happen as a function of the number of emitters, the chirality of the waveguide, and the single-emitter optical depth, both for ordered and disordered ensembles. Many-body superradiance occurs because the initial fluctuation that triggers the emission is amplified throughout the decay process. In one-dimensional baths, this avalanchelike behavior leads to a spontaneous mirror symmetry breaking, with large shot-to-shot fluctuations in the number of photons emitted to the left and right. Superradiant bursts may thus be a smoking gun for the generation of correlated photon states of exotic quantum statistics.
In 1973 Klaus Hepp and Elliott Lieb showed that a tightly confined ensemble of atoms placed in a quantised single-mode optical cavity will have their emission of light enhanced by constructive interference of emission events if the photons emitted are indistinguishable. This effect, known as superradiance, has proven difficult to realise experimentally due to the strong light-matter coupling required to produce such behaviour. However, over the last decade there have been several successful realisations which engineer superradiance by driving Raman transitions between atomic ground states of multilevel atoms. In this case, superradiance emerges via a quantum phase transition mediated by the laser driving power. In this work, we consider a generalisation of this model referred to as the unbalanced Dicke model. It has recently been implemented experimentally and is characterised by two lasers driving two distinct Raman transitions. We show that, in the semiclassical limit of a large number of atoms, the unbalanced Dicke model exhibits a wealth of nonlinear dynamics which describe novel dynamical phases of matter. Examples of nonlinear behaviour observed are pitchfork, saddle-node, and Hopf bifurcations, as well as two types of chaos. We explore the quantum mechanical manifestations of these bifurcations and additional physical effects which appear in the presence of quantum fluctuations. In this way, the model creates a playground in which to explore the onset of classical nonlinear dynamics from an open quantum system.
Coupling between quantum emitters and modes of light is foundational to studies of quantum systems. Coherent interactions between matter and light have greatly advanced the development of quantum technologies. When an ensemble of atoms interacts with light that is confined within a cavity---a resonator for photons---light also mediates atom-atom interactions, leading to collective phenomena that cannot be extrapolated from microscopic behaviors. Understanding how interactions among quantum particles lead to macroscopic phenomena, such as phase transitions and breaking of symmetries, remains a challenge in modern physics. In this dissertation, I present results addressing this challenge in the context of mesoscopic arrays of optical-tweezer-trapped atoms interfaced with a high-finesse optical cavity. In particular, the physics we investigate arises from the collective scattering of light. Utilizing the ability to place atoms with nanometer-scale precision, we engineer superradiant and subradiant states, where control over interference of the emission from multiple atoms leads to collectively enhanced or suppressed amounts of scattered light. Building on this work, we investigate the emergence of optomechanical self-organization, mediated by superradiance in the cavity electromagnetic field. By coupling atoms to the same cavity mode, the atoms exert forces on one another through the exchange of photons, leading them to autonomously order themselves spatially. We characterize mesoscopic fluctuations and their effect on symmetry-breaking dynamics associated with self-organization. Finally, we extend this framework to theoretically investigate how the phase of the atom-cavity coupling can be altered to generate higher symmetries. Our analysis reveals first-order phase transitions and instabilities induced by non-reciprocal forces. Altogether, this work establishes a path towards realizing mesoscopic systems of complex phases of matter in cavity quantum electrodynamics with unprecedented programmability.
Understanding how frustration and symmetry breaking shape collective behavior is a central problem in quantum many-body systems. In this work, we investigate this problem in large one- and two-dimensional arrays of coupled Dicke models on a periodic lattice, where strong light-matter coupling gives rise to a superradiant phase and competition between neighboring order parameters induces spontaneous translational symmetry breaking. Such Dicke lattice models constitute a fundamentally new class of quantum many-body systems, as they simultaneously realize the thermodynamic limit associated with the lattice size and an intrinsic thermodynamic limit arising from collective on-site interactions with quantum emitters. We show that frustration drives photonic density-wave ordering, and that the resulting broken periodicity can be predicted from the excitation spectrum of the symmetric phase, without requiring computationally prohibitive thermodynamic energy minimization. Furthermore, we demonstrate that an emergent Nambu-Goldstone mode arises near the critical point in a one-dimensional chain despite the presence of only discrete symmetry, and uncover the mechanism that enables this otherwise forbidden gapless excitation. We also find quasi-periodic ordering in the superradiant phase, reminiscent of quasicrystals, and demonstrate that synthetic magnetic flux provides a powerful knob to control the nature of translational symmetry breaking. Our results establish a new direction in quantum many-body physics where the coexistence of local and global thermodynamic limits gives rise to unconventional symmetry breaking and emergent collective behavior.
We study the collective spontaneous emission of a linear atomic chain excited by a single photon. The interaction between the atoms and the common vacuum field can significantly change the eigenenergy and the spontaneous emission rate of the system. Due to the dipole-dipole interactions, the system prepared in a single-photon timed Dicke state is the superposition of superradiant and subradiant eigenstates that can have a nonexponential decay dynamics. We can tune the frequency and linewidth of the superradiant and subradiant emission from a timed Dicke state by changing the direction of the atomic dipole moment or the atomic separation. In addition, the emission direction of the superradiant and subradiant photons also depends on the polarization of the atoms.
Fully-excited two-level atoms separated by less than the transition wavelength cooperatively emit light in a short burst, a phenomenon called superradiance by R. Dicke in 1954. The burst is characterized by a maximum intensity scaling with the square of the number of atoms N and a temporal width reduced by N compared to the single atom spontaneous decay time. Both effects are usually attributed to a synchronization of the electric dipole moments of the atoms occurring during the process of light emission. Contrary to this explanation, it was recently shown by use of a quantum path description that the peak intensity results from the quantum correlations among the atoms when occupying symmetric Dicke states. Here we investigate from this perspective the temporal evolution of the ensemble, starting in the small sample limit, i.e., when the atoms have mutual separations much smaller than the transition wavelength λ and pass down the ladder of symmetric Dicke states. In addition, we explore the temporal evolution for the case of non-interacting atoms with mutual separations much larger than λ. We show that in this case a similar superradiant burst of the emitted radiation is observed if the quantum correlations of the atoms are generated by conditional photon measurements retaining the atomic ensemble within or close to the symmetric subspace.