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arXiv:2509.22096

A Source of Deterministic Entanglement for Matter-Wave Networks

Li‐Qun Chen, RuGway Wu, Jörg Schmiedmayer

Published Sep 26, 2025• 0 citations
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Abstract

We describe a deterministic and experimentally feasible protocol for generating entangled pairs of ultracold neutral atoms through controlled dissociation of diatomic Feshbach molecules. The dissociation process naturally produces nonlocal quantum correlations in spin, position-momentum, and path degrees of freedom, enabling the deterministic preparation of Einstein-Podolsky-Rosen pairs of massive particles and multiqubit states through hyperentangled encoding. Having each atom of the pair prepared in a matter waveguide, the scheme can be scaled to hundreds of parallel entanglement sources in an array connected to a matter wave optical network of beam splitters, phase shifters, interferometers, tunnel junctions and local detectors. The protocol builds on established techniques, including programmable optical potentials, high-fidelity single-particle control, single-molecule initialization, controlled molecular dissociation, and quantum gas microscopy with near-perfect detection, making it directly implementable with current technology. The proposed architecture naturally integrates with atomtronics circuits and chip-based matter-wave optics, offering a deterministic entanglement source for quantum nonlocality tests, precision metrology, and scalable neutral-atom quantum processors.

DOI
10.48550/arxiv.2509.22096

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We describe a deterministic and experimentally feasible protocol for generating entangled pairs of ultracold neutral atoms through controlled dissociation of diatomic Feshbach molecules. The dissociation process naturally produces nonlocal quantum correlations in spin, position-momentum, and path degrees of freedom, enabling the deterministic preparation of Einstein-Podolsky-Rosen pairs of massive particles and multiqubit states through hyperentangled encoding. Having each atom of the pair prepared in a matter waveguide, the scheme can be scaled to hundreds of parallel entanglement sources in an array connected to a matter wave optical network of beam splitters, phase shifters, interferometers, tunnel junctions and local detectors. The protocol builds on established techniques, including programmable optical potentials, high-fidelity single-particle control, single-molecule initialization, controlled molecular dissociation, and quantum gas microscopy with near-perfect detection, making it directly implementable with current technology. The proposed architecture naturally integrates with atomtronics circuits and chip-based matter-wave optics, offering a deterministic entanglement source for quantum nonlocality tests, precision metrology, and scalable neutral-atom quantum processors.
Recent experimental measurements of atomic intensity correlations through atom shot noise suggest that atomic quadrature phase correlations may soon be measured with a similar precision. We propose a test of local realism with mesoscopic numbers of massive particles based on such measurements. Using dissociation of a Bose-Einstein condensate of diatomic molecules into bosonic atoms, we demonstrate that strongly entangled atomic beams may be produced which possess Einstein-Podolsky-Rosen (EPR) correlations in field quadratures in direct analogy to the position and momentum correlations originally considered by EPR.
High-fidelity entanglement of neutral cold atoms can be achieved by combining several already available techniques such as the creation or dissociation of neutral diatomic molecules, manipulating atoms with microfabricated structures (atom chips), and detecting single atoms with almost 100% efficiency. The fidelity of the resulting entanglement is robust against the details of dissociation process. Manipulating this entanglement with integrated or linear atom optics will open a perspective for quantum-information processing with neutral atoms.
The deterministic control of light-matter interactions at the level of single particles and on subwavelength scales is central to quantum optics and hybrid integrated quantum technologies. However, combining cold atom research with nanophotonic devices in a fully controllable platform remains a major experimental challenge. Here, we demonstrate the deterministic coupling of an ultracold atomic lattice to light propagating in suspended on-chip photonic circuits. These capabilities open avenues to address scalability challenges in neutral-atom quantum computers and simulators, enabling fast optical readout, efficient and subwavelength non-diffracting interaction zones, and genuine compatibility with integrated solid-state photon sources, detectors, and stop-band modulators. Beyond controllable quantum matter, the platform also enables in-situ imaging of evanescent fields of light and nanoscale structures, including prospects for three-dimensional scanning microscopy with non-invasive single-atom probes for quantum sensing applications.
Engineering pairs of massive particles that are simultaneously correlated in their external and internal degrees of freedom is a major challenge, yet essential for advancing fundamental tests of physics and quantum technologies. In this Letter, we experimentally demonstrate a mechanism for generating pairs of atoms in well-defined spin and momentum modes. This mechanism couples atoms from a degenerate Bose gas via a superradiant photon-exchange process in an optical cavity, producing pairs via a single channel or two discernible channels. The scheme is independent of collisional interactions, fast, and tunable. We observe a collectively enhanced production of pairs and probe interspin correlations in momentum space. We characterize the emergent pair statistics and find that the observed dynamics is consistent with being primarily seeded by vacuum fluctuations in the corresponding atomic modes. Together with our observations of coherent many-body oscillations involving well-defined momentum modes, our results offer promising prospects for quantum-enhanced interferometry and quantum simulation experiments using entangled matter waves.