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arXiv:2509.04739 · Physical Review Letters

Cavity QED Based on Strongly Localized Modes: Exponentially Enhancing Single-Atom Cooperativity

Qian Bin, Ying Nian Wu, Jinhua Gao, Ai-Xi Chen, Franco Nori, Xin‐You Lü

Published Aug 14, 2025• 9 citations
arXivHTMLPDF

Abstract

Large single-atom cooperativity in quantum systems is important for quantum information processing. Here, we propose to exponentially enhance the single-atom cooperativity parameter by exploiting the strongly localized effect of modes in cavity quantum electrodynamics (QED) systems. By increasing the wing width of a cavity with special geometry symmetry, the interference property allows us to exponentially improve the quality factor Q without altering the mode volume V for cavities supporting subwavelength light modes. This effectively overcomes the trade-off between Q and V in conventional subwavelength Fabry-Pérot cavities. Consequently, we demonstrate the occurrence of ultralong vacuum Rabi oscillations and the generation of strong photon blockade by enhancing the single-atom cooperativity parameter. This Letter offers a promising approach for advancing coherent manipulation and holds significant potential for applications in establishing longer-distance quantum communication networks, enhancing the precision and stability of quantum sensors, and improving the efficiency of quantum algorithms.

DOI
10.1103/7frd-pf1m

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A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. 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The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. 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Journal of Optics B Quantum and Semiclassical Optics•Feb 1, 2004•0 citations
Large single-atom cooperativity in quantum systems is important for quantum information processing. Here, we propose to exponentially enhance the single-atom cooperativity parameter by exploiting the strongly localized effect of modes in cavity quantum electrodynamics (QED) systems. By increasing the wing width of a cavity with special geometry symmetry, the interference property allows us to exponentially improve the quality factor Q without altering the mode volume V for cavities supporting subwavelength light modes. This effectively overcomes the trade-off between Q and V in conventional subwavelength Fabry-Pérot cavities. Consequently, we demonstrate the occurrence of ultralong vacuum Rabi oscillations and the generation of strong photon blockade by enhancing the single-atom cooperativity parameter. This Letter offers a promising approach for advancing coherent manipulation and holds significant potential for applications in establishing longer-distance quantum communication networks, enhancing the precision and stability of quantum sensors, and improving the efficiency of quantum algorithms.
Abstract We experimentally realize a new cavity quantum electrodynamics (QED) platform with defect-free single-atom array strongly coupled to an optical cavity. The defect-free single-atom array is obtained by rearranging a probabilistically loaded one-dimensional (1D) optical tweezer array with dimensions of 1×401 \times 401×40 1 × 40 . The atom array is enclosed with two cavity mirrors, which compose a miniature optical Fabry-Pérot cavity with cavity length of 1.15 mm. By precisely controlling the position of the atom array, we demonstrate uniform and strong coupling of all atoms in the array with the optical cavity. The average coupling strength between the single atom and the cavity is 2.62 MHz. The vacuum Rabi splitting spectra for single-atom arrays with atom number N changing from 3 to 26 are measured. Thus, the collective enhancement of the coupling strength with N{\sqrt {N}}N​ N -dependence for multiple atoms is validated at the single atom level. Our system holds significant potential for establishing the foundation of distributed quantum computing and advancing fundamental research in many-body physics.
When an atom is strongly coupled to a cavity, the two systems can exchange a single photon through a coherent Rabi oscillation. This process enables precise quantum-state engineering and manipulation of atoms and photons in a cavity, which play a central role in quantum information and measurement. Recently, a new regime of cavity QED was reached experimentally where the strength of the interaction between light and artificial atoms (qubits) becomes comparable to the atomic transition frequency or the resonance frequency of the cavity mode. Here we show that this regime can strongly modify the concept of vacuum Rabi oscillations, enabling multiphoton exchanges between the qubit and the resonator. We find that experimental state-of-the-art circuit-QED systems can undergo two- and three-photon vacuum Rabi oscillations. These anomalous Rabi oscillations can be exploited for the realization of efficient Fock-state sources of light and complex entangled states of qubits.
From fundamental studies of light-matter interaction to applications in quantum networking and sensing, cavity quantum electrodynamics (QED) provides a toolbox to control interactions between atoms and photons. The coherence of interactions is determined by the single-pass atomic absorption and number of photon round-trips. Reducing the cavity loss has enabled resonators supporting 1 million roundtrips but with limited material choices and increased alignment sensitivity. Here, we present a high–numerical aperture, lens-based resonator that pushes the single-atom single-photon absorption probability near its fundamental limit, reducing the mode size at the atom to order λ. This resonator provides a single-atom cooperativity of 1.6 in a cavity where the light circulates ∼10 times. We load single 87 Rb atoms into this cavity, observe strong coupling, and demonstrate cavity-enhanced atom detection with fidelity of 99.55(6)% and survival of 99.89(4)% in 130 μs. Introducing intracavity imaging systems will enable cavity arrays compatible with Rydberg atom array computing technologies, expanding the applicability of the cavity QED toolbox.
Cavity quantum electrodynamics (QED) with cooperativity far greater than unity enables high-fidelity quantum sensing and information processing.The high-cooperativity regime is often reached through the use of short single-mode resonators.More complicated multimode resonators, such as the near-confocal optical Fabry-Pérot cavity, can provide intracavity atomic imaging in addition to high cooperativity.This capability has recently proved important for exploring quantum many-body physics in the driven-dissipative setting.In this work, we show that a confocal-cavity-QED microscope can realize cooperativity in excess of 110.This cooperativity is on par with the very best single-mode cavities (which are far shorter) and 21 times greater than single-mode resonators of similar length and mirror radii.The 1.7-µm imaging resolution is naturally identical to the photon-mediated interaction range.We measure these quantities by determining the threshold of cavity superradiance when small optically tweezed Bose-Einstein condensates are pumped at various intracavity locations.Transmission measurements of an ex situ cavity corroborate these results.We provide a theoretical description that shows how cooperativity enhancement arises from the dispersive coupling to the atoms of many near-degenerate modes.
The paradigm of cavity QED is a two-level emitter interacting with a high-quality factor single-mode optical resonator. The hybridization of the emitter and photon wave functions mandates large vacuum Rabi frequencies and long coherence times; features that so far have been successfully realized with trapped cold atoms and ions, and localized solid-state quantum emitters such as superconducting circuits, quantum dots, and color centers Reiserer and Rempe (Rev Modern Phys 87:1379, 2015), Faraon et al. (Phys Rev 81:033838, 2010). Thermal atoms, on the other hand, provide us with a dense emitter ensemble and in comparison to the cold systems are more compatible with integration, hence enabling large-scale quantum systems. However, their thermal motion and large transit-time broadening is a major bottleneck that has to be circumvented. A promising remedy could benefit from the highly controllable and tunable electromagnetic fields of a nano-photonic cavity with strong local electric-field enhancements. Utilizing this feature, here we investigate the interaction between fast moving thermal atoms and a nano-beam photonic crystal cavity (PCC) with large quality factor and small mode volume. Through fully quantum mechanical calculations, including Casimir-Polder potential (i.e. the effect of the surface on radiation properties of an atom), we show, when designed properly, the achievable coupling between the flying atom and the cavity photon would be strong enough to lead to quantum interference effects in spite of short interaction times. In addition, the time-resolved detection of different trajectories can be used to identify single and multiple atom counts. This probabilistic approach will find applications in cavity QED studies in dense atomic media and paves the way towards realizing large-scale, room-temperature macroscopic quantum systems aimed at out of the lab quantum devices.
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.