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arXiv:2508.13410

$p$-orbital self-organization of ultracold atoms coupled to optical cavities

Hui Ru Tan, Pengfei Zhang, Jianmin Yuan, Yongqiang Li

Published Aug 19, 2025• 0 citations
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Abstract

Atoms coupled to optical cavities provide a novel platform for understanding high-orbital exotic phenomena in strongly correlated materials. In this study, we investigate strongly correlated ultracold bosonic gases that are coupled to two orthogonally arranged optical cavities and driven by a blue-detuned running-wave laser field. Our results demonstrate that atoms initially in the $s$-orbital state can be scattered into $p_x$- and $p_y$-orbital states in either a symmetric or asymmetric manner, depending on the frequencies of the two cavities. For the symmetric configuration, we observe that atoms are scattered into the $p_x$- and $p_y$-orbitals equally. In the asymmetric case, photons emitted into one cavity mode suppress the scattering into the orthogonal mode. Notably, the coupling of atoms with multiple cavity modes leads to the emergence of high-orbital self-organized phases, accompanied by orbital-density waves that break different symmetries.

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ppp-orbital self-organization of ultracold atoms coupled to optical cavities
Atoms coupled to optical cavities provide a novel platform for understanding high-orbital exotic phenomena in strongly correlated materials. In this study, we investigate strongly correlated ultracold bosonic gases that are coupled to two orthogonally arranged optical cavities and driven by a blue-detuned running-wave laser field. Our results demonstrate that atoms initially in the sss-orbital state can be scattered into pxp_xpx​- and pyp_ypy​-orbital states in either a symmetric or asymmetric manner, depending on the frequencies of the two cavities. For the symmetric configuration, we observe that atoms are scattered into the pxp_xpx​- and pyp_ypy​-orbitals equally. In the asymmetric case, photons emitted into one cavity mode suppress the scattering into the orthogonal mode. Notably, the coupling of atoms with multiple cavity modes leads to the emergence of high-orbital self-organized phases, accompanied by orbital-density waves that break different symmetries.
The orbital degree of freedom plays an important role in understanding exotic phenomena of strongly correlated materials. In this work, we study strongly correlated ultracold bosonic gases coupled to a high-finesse cavity, pumped by a blue-detuned laser in the transverse direction. By controlling the reflection of the pump laser, we find that atoms can be selectively transferred to the odd-parity ppp-orbital band or to the even-parity ddd-orbital band of a two-dimensional square lattice, accompanied by pronounced cavity-photon excitations. By interacting with the cavity field, atoms self-organize to form stable higher-orbital superfluid and Mott-insulating phases with orbital-density waves, as a result of cavity-induced orbital-flip hoppings. Our study opens a route to manipulate orbital degrees of freedom in strongly correlated quantum gases via coupling to optical cavities.
When placing an ultracold atomic gas inside a cavity, the light-matter coupling is enhanced and nonlinear atomic dynamics is generated, offering a promising platform for quantum simulation of models with short- and long-range interactions. Recently, superradiant self-organized phases for ultracold atomic gases inside a cavity, pumped by a blue detuned optical lattice, have been observed. Here, we explore the formation of quantum many-body phases of bosonic atoms inside an optical cavity, subject to transverse blue detuned pumping. We investigate the strongly interacting regime, which can be reached by tuning the s-wave scattering length using external fields. We analyze the interplay between superradiant self-organization with superfluid and Mott insulator phases, without the need of including higher lying bands, as the Wannier functions are dynamically linked to the cavity light via backaction. We observe different kinds of structural phase transitions driven by the light inside the cavity and the interplay with atomic collisions. We observe the mode softening at the critical points in the quantum phase transitions which can be measured in future experiments. We obtain our results within a full self-consistent theoretical framework, the light-matter density matrix renormalization group (DMRG), which employs the computation of light dependent Wannier functions for the full quantum optical lattice in combination with DMRG for the atomic dynamics. The methods introduced here can be used to analyze the effects of strong quantum correlations in strongly interacting light-matter systems.
We investigate the physics of a gas of ultracold atoms coupled to three single-mode optical cavities and transversely pumped with a laser. Recent work has demonstrated that, for two cavities, the Z2{\mathbb{Z}}_{2}Z2​ symmetries of each cavity can be combined into a global U(1) symmetry [J. L\'eonard et al., Nature (London) 543, 87 (2017)]. Here we show that when adding an extra cavity mode, the low-energy description of this system can additionally exhibit an SO(3) rotational symmetry which can be spontaneously broken. This leads to a superradiant phase transition in all the cavities simultaneously, and the appearance of Goldstone and amplitude modes in the excitation spectrum. We determine the phase diagram of the system, which shows the emergence and breaking of the continuous symmetries and displays first- and second-order phase transitions. We also obtain the excitation spectrum for each phase and discuss the atomic self-organized structures that emerge in the different superradiant phases. We argue that coupling the atoms equally to nnn different modes will in general generate a global SO(n)\text{SO}(n)SO(n) symmetry if the mode frequencies can be tuned to the same value.
Ultracold atoms coupled to optical cavities offer a powerful platform for studying strongly correlated many-body physics. Here, we propose an experimental scheme for creating biatomic molecules via cavity-enhanced photoassociation from an atomic condensate. This setup realizes long-range three-body interactions mediated by tripartite cavity-atom-molecule coupling. Beyond a critical pump strength, a self-organized square lattice phase for molecular condensate emerges, resulting in hybrid atom-molecule superradiance with spontaneous U(1)U(1)U(1) symmetry breaking. Distinct from previously observed ultracold bosonic (fermionic) atomic superradiance, our findings demonstrate bosonic enhancement characterized by a cubic scaling of steady-state photon number with total atom number. Additionally, strong photon-matter entanglement is shown to effectively characterize superradiant quantum phase transition. Our findings deepen the understanding of quantum superchemistry and exotic many-body nonequilibrium dynamics in cavity-coupled quantum gases.
We numerically simulate strongly correlated ultracold bosons coupled to a high-finesse cavity field, pumped by a laser beam in the transverse direction. Assuming a weak classical\mathit{classical}classical optical lattice added in the cavity direction, we model this system by a generalized Bose-Hubbard model, which is solved by means of bosonic dynamical mean-field theory. The complete phase diagram is established, which contains two novel self-organized quantum phases, lattice supersolid and checkerboard solid, in addition to conventional phases such as superfluid and Mott insulator. At finite but low temperature, thermal fluctuations are found to enhance the buildup of the self-organized phases. We demonstrate that cavity-mediated long-range interactions can give rise to stable lattice supersolid and checkerboard solid phases even in the regime of strong sss-wave scattering. In the presence of a harmonic trap, we discuss coexistence of these self-organized phases, as relevant to experiments.
Ultracold atomic gases loaded into optical cavities constitute one of the most versatile platforms for the study of out-of-equilibrium dynamics and quantum simulation of many- body systems. In this thesis, we explore these two possibilities, motivated by current state-of-the-art atom-cavity experiments, uncovering novel phenomena and opening up new theoretical and experimental avenues into the intriguing world of quantum many- body physics. First, we study a gas of ultracold atoms coupled to three optical resonators. We show that the inherent Z2 symmetries, associated with each atom-cavity coupling, can be combined into a global SO(3) rotational symmetry which can be spontaneously broken. We determine the phase diagram of the system, which shows the emergence and breaking of the continuous symmetries and displays first- and second-order phase transitions. We argue that by coupling the atoms equally to n different modes, it will in general be possible to generate a global SO(n) symmetry. Second, we investigate the dynamics of a spinor BEC inside an optical cavity. We focus on a two-component Dicke model with complex light-matter couplings, accounting for photon losses. We compute the steady-state phase diagram and find dynamical in- stabilities in the form of limit cycles, heralded by the presence of exceptional points and level attraction. We show that the instabilities are induced by dissipative processes that generate nonreciprocal couplings between the two collective spins. Lastly, we explore the dynamics of a BEC inside an optical cavity in the presence of an optical lattice. We derive an effective master equation by adiabatically eliminating the cavity field. In the bad-cavity regime, we find an infinite-temperature steady state, but with relaxation dynamics that can be highly nontrivial. For small hopping, the interplay between dissipation and strong interactions leads to an algebraic relaxation of the system, whereas for large hopping, the approach to the steady state is exponential. In the good- cavity regime, we show that the system allows for optical pumping between momentum modes, enabling cavity cooling.