Ultracold atoms coupled to optical cavities offer a powerful platform for studying strongly correlated many-body physics. Here, we propose an experimental scheme for creating biatomic molecules via cavity-enhanced photoassociation from an atomic condensate. This setup realizes long-range three-body interactions mediated by tripartite cavity-atom-molecule coupling. Beyond a critical pump strength, a self-organized square lattice phase for molecular condensate emerges, resulting in hybrid atom-molecule superradiance with spontaneous $U(1)$ symmetry breaking. Distinct from previously observed ultracold bosonic (fermionic) atomic superradiance, our findings demonstrate bosonic enhancement characterized by a cubic scaling of steady-state photon number with total atom number. Additionally, strong photon-matter entanglement is shown to effectively characterize superradiant quantum phase transition. Our findings deepen the understanding of quantum superchemistry and exotic many-body nonequilibrium dynamics in cavity-coupled quantum gases.
Ultracold atoms coupled to optical cavities offer a powerful platform for studying strongly correlated many-body physics. Here, we propose an experimental scheme for creating biatomic molecules via cavity-enhanced photoassociation from an atomic condensate. This setup realizes long-range three-body interactions mediated by tripartite cavity-atom-molecule coupling. Beyond a critical pump strength, a self-organized square lattice phase for molecular condensate emerges, resulting in hybrid atom-molecule superradiance with spontaneous U(1) symmetry breaking. Distinct from previously observed ultracold bosonic (fermionic) atomic superradiance, our findings demonstrate bosonic enhancement characterized by a cubic scaling of steady-state photon number with total atom number. Additionally, strong photon-matter entanglement is shown to effectively characterize superradiant quantum phase transition. Our findings deepen the understanding of quantum superchemistry and exotic many-body nonequilibrium dynamics in cavity-coupled quantum gases.
Coherent light-matter interactions between a quantum gas and light in a high-finesse cavity can drive self-ordering phase transitions. To date, such phenomena have involved exclusively single-atom coupling to light, resulting in coupled charge-density or spin-density wave and superradiant order. In this work, we engineer simultaneous coupling of cavity photons to both single atoms and fermionic pairs, which are also mutually coupled due to strong correlations in the unitary Fermi gas. This interplay gives rise to an interference between the charge-density wave and a pair-density wave, where the short-range pair correlation function is spontaneously modulated in space. We observe this effect by tracking the onset of superradiance as the photon-pair coupling is varied in strength and sign, revealing constructive or destructive interference of the three orders with a coupling mediated by strong light-matter and atom-atom interactions. Our observations are compared with mean-field theory where the coupling strength between atomic- and pair-density waves is controlled by higher-order correlations in the Fermi gas. These results demonstrate the potential of cavity quantum electrodynamics to produce and observe exotic orders in strongly correlated matter, paving the way for the quantum simulation of complex quantum matter using ultracold atoms. Cavity-mediated interactions lead to collective effects and ordering in ultracold atomic systems. Here, the authors demonstrate the interplay of different ordered states of ultracold Fermi gases in a cavity, resulting from an intriguing coexistence of photon coupling with both atoms and atom-pairs.
Coherent light-matter interactions between a quantum gas and light in a high-finesse cavity can drive self-ordering phase transitions. To date, such phenomena have involved exclusively single-atom coupling to light, resulting in coupled charge-density or spin-density wave and superradiant order. In this work, we engineer simultaneous coupling of cavity photons to both single atoms and fermionic pairs, which are also mutually coupled due to strong correlations in the unitary Fermi gas. This interplay gives rise to an interference between the charge-density wave and a pair-density wave, where the short-range pair correlation function is spontaneously modulated in space. We observe this effect by tracking the onset of superradiance as the photon-pair coupling is varied in strength and sign, revealing constructive or destructive interference of the three orders with a coupling mediated by strong light-matter and atom-atom interactions. Our observations are compared with mean-field theory where the coupling strength between atomic- and pair-density waves is controlled by higher-order correlations in the Fermi gas. These results demonstrate the potential of cavity quantum electrodynamics to produce and observe exotic orders in strongly correlated matter, paving the way for the quantum simulation of complex quantum matter using ultracold atoms.
Coupling between quantum emitters and modes of light is foundational to studies of quantum systems. Coherent interactions between matter and light have greatly advanced the development of quantum technologies. When an ensemble of atoms interacts with light that is confined within a cavity---a resonator for photons---light also mediates atom-atom interactions, leading to collective phenomena that cannot be extrapolated from microscopic behaviors. Understanding how interactions among quantum particles lead to macroscopic phenomena, such as phase transitions and breaking of symmetries, remains a challenge in modern physics. In this dissertation, I present results addressing this challenge in the context of mesoscopic arrays of optical-tweezer-trapped atoms interfaced with a high-finesse optical cavity. In particular, the physics we investigate arises from the collective scattering of light. Utilizing the ability to place atoms with nanometer-scale precision, we engineer superradiant and subradiant states, where control over interference of the emission from multiple atoms leads to collectively enhanced or suppressed amounts of scattered light. Building on this work, we investigate the emergence of optomechanical self-organization, mediated by superradiance in the cavity electromagnetic field. By coupling atoms to the same cavity mode, the atoms exert forces on one another through the exchange of photons, leading them to autonomously order themselves spatially. We characterize mesoscopic fluctuations and their effect on symmetry-breaking dynamics associated with self-organization. Finally, we extend this framework to theoretically investigate how the phase of the atom-cavity coupling can be altered to generate higher symmetries. Our analysis reveals first-order phase transitions and instabilities induced by non-reciprocal forces. Altogether, this work establishes a path towards realizing mesoscopic systems of complex phases of matter in cavity quantum electrodynamics with unprecedented programmability.
We review the recent developments and the current status in the field of quantum-gas cavity QED. Since the first experimental demonstration of atomic self-ordering in a system composed of a Bose–Einstein condensate coupled to a quantized electromagnetic mode of a high-Q optical cavity, the field has rapidly evolved over the past decade. The composite quantum-gas-cavity systems offer the opportunity to implement, simulate, and experimentally test fundamental solid-state Hamiltonians, as well as to realize non-equilibrium many-body phenomena beyond conventional condensed-matter scenarios. This hinges on the unique possibility to design and control in open quantum environments photon-induced tunable-range interaction potentials for the atoms using tailored pump lasers and dynamic cavity fields. Notable examples range from Hubbard-like models with long-range interactions exhibiting a lattice-supersolid phase, over emergent magnetic orderings and quasicrystalline symmetries, to the appearance of dynamic gauge potentials and non-equilibrium topological phases. Experiments have managed to load spin-polarized as well as spinful quantum gases into various cavity geometries and engineer versatile tunable-range atomic interactions. This led to the experimental observation of spontaneous discrete and continuous symmetry breaking with the appearance of soft-modes as well as supersolidity, density and spin self-ordering, dynamic spin-orbit coupling, and non-equilibrium dynamical self-ordered phases among others. In addition, quantum-gas-cavity setups offer new platforms for quantum-enhanced measurements. In this review, starting from an introduction to basic models, we pedagogically summarize a broad range of theoretical developments and put them in perspective with the current and near future state-of-art experiments.
When placing an ultracold atomic gas inside a cavity, the light-matter coupling is enhanced and nonlinear atomic dynamics is generated, offering a promising platform for quantum simulation of models with short- and long-range interactions. Recently, superradiant self-organized phases for ultracold atomic gases inside a cavity, pumped by a blue detuned optical lattice, have been observed. Here, we explore the formation of quantum many-body phases of bosonic atoms inside an optical cavity, subject to transverse blue detuned pumping. We investigate the strongly interacting regime, which can be reached by tuning the s-wave scattering length using external fields. We analyze the interplay between superradiant self-organization with superfluid and Mott insulator phases, without the need of including higher lying bands, as the Wannier functions are dynamically linked to the cavity light via backaction. We observe different kinds of structural phase transitions driven by the light inside the cavity and the interplay with atomic collisions. We observe the mode softening at the critical points in the quantum phase transitions which can be measured in future experiments. We obtain our results within a full self-consistent theoretical framework, the light-matter density matrix renormalization group (DMRG), which employs the computation of light dependent Wannier functions for the full quantum optical lattice in combination with DMRG for the atomic dynamics. The methods introduced here can be used to analyze the effects of strong quantum correlations in strongly interacting light-matter systems.
We report on the first experimental realization of the Dicke quantum phase transition realized in the quantum motion of a Bose–Einstein condensate coupled to an optical cavity. Conceptually, the transition is driven by cavity-mediated long-range interactions, giving rise to the emergence of a self-organized supersolid phase. The Dicke phase transition, predicted in 1973, has not been demonstrated experimentally before this work, both due to fundamental and technological reasons. These challenges have been overcome in the present thesis by employing atomic momentum states of a Bose-Einstein condensate, which are coupled via two-photon Raman transitions involving a cavity photon and a free-space pump photon. This open-system implementation of the Dicke model allows to tune all relevant parameters and offers a unique detection scheme to monitor the manybody system in real time. We demonstrate that the phase transition is accompanied by a macroscopically occupied cavity field and a striking change in the atomic momentum distribution, due to spontaneous self-organization of the atomic density on a checkerboard lattice. The boundary of the transition is mapped out by scanning two parameters of the Dicke model, to reveal a phase diagram in close agreement with the model description. Two different ordered configurations are allowed in the superradiant phase, giving rise to the concept of spontaneous symmetry breaking at the phase transition. We experimentally distinguish the symmetry-broken states and study the origin of the symmetry-breaking process. The finite spatial extension of our system induces a small symmetry-breaking field which changes randomly on each experimental realization. The influence of this field is studied and shown to diminish upon dynamically crossing the transition point with increasing transition rates.