We review the recent developments and the current status in the field of quantum-gas cavity QED. Since the first experimental demonstration of atomic self-ordering in a system composed of a Bose–Einstein condensate coupled to a quantized electromagnetic mode of a high-Q optical cavity, the field has rapidly evolved over the past decade. The composite quantum-gas-cavity systems offer the opportunity to implement, simulate, and experimentally test fundamental solid-state Hamiltonians, as well as to realize non-equilibrium many-body phenomena beyond conventional condensed-matter scenarios. This hinges on the unique possibility to design and control in open quantum environments photon-induced tunable-range interaction potentials for the atoms using tailored pump lasers and dynamic cavity fields. Notable examples range from Hubbard-like models with long-range interactions exhibiting a lattice-supersolid phase, over emergent magnetic orderings and quasicrystalline symmetries, to the appearance of dynamic gauge potentials and non-equilibrium topological phases. Experiments have managed to load spin-polarized as well as spinful quantum gases into various cavity geometries and engineer versatile tunable-range atomic interactions. This led to the experimental observation of spontaneous discrete and continuous symmetry breaking with the appearance of soft-modes as well as supersolidity, density and spin self-ordering, dynamic spin-orbit coupling, and non-equilibrium dynamical self-ordered phases among others. In addition, quantum-gas-cavity setups offer new platforms for quantum-enhanced measurements. In this review, starting from an introduction to basic models, we pedagogically summarize a broad range of theoretical developments and put them in perspective with the current and near future state-of-art experiments.
We review the recent developments and the current status in the field of quantum-gas cavity QED. Since the first experimental demonstration of atomic self-ordering in a system composed of a Bose–Einstein condensate coupled to a quantized electromagnetic mode of a high-Q optical cavity, the field has rapidly evolved over the past decade. The composite quantum-gas-cavity systems offer the opportunity to implement, simulate, and experimentally test fundamental solid-state Hamiltonians, as well as to realize non-equilibrium many-body phenomena beyond conventional condensed-matter scenarios. This hinges on the unique possibility to design and control in open quantum environments photon-induced tunable-range interaction potentials for the atoms using tailored pump lasers and dynamic cavity fields. Notable examples range from Hubbard-like models with long-range interactions exhibiting a lattice-supersolid phase, over emergent magnetic orderings and quasicrystalline symmetries, to the appearance of dynamic gauge potentials and non-equilibrium topological phases. Experiments have managed to load spin-polarized as well as spinful quantum gases into various cavity geometries and engineer versatile tunable-range atomic interactions. This led to the experimental observation of spontaneous discrete and continuous symmetry breaking with the appearance of soft-modes as well as supersolidity, density and spin self-ordering, dynamic spin-orbit coupling, and non-equilibrium dynamical self-ordered phases among others. In addition, quantum-gas-cavity setups offer new platforms for quantum-enhanced measurements. In this review, starting from an introduction to basic models, we pedagogically summarize a broad range of theoretical developments and put them in perspective with the current and near future state-of-art experiments.
Ultracold atomic gases loaded into optical cavities constitute one of the most versatile platforms for the study of out-of-equilibrium dynamics and quantum simulation of many- body systems. In this thesis, we explore these two possibilities, motivated by current state-of-the-art atom-cavity experiments, uncovering novel phenomena and opening up new theoretical and experimental avenues into the intriguing world of quantum many- body physics. First, we study a gas of ultracold atoms coupled to three optical resonators. We show that the inherent Z2 symmetries, associated with each atom-cavity coupling, can be combined into a global SO(3) rotational symmetry which can be spontaneously broken. We determine the phase diagram of the system, which shows the emergence and breaking of the continuous symmetries and displays first- and second-order phase transitions. We argue that by coupling the atoms equally to n different modes, it will in general be possible to generate a global SO(n) symmetry. Second, we investigate the dynamics of a spinor BEC inside an optical cavity. We focus on a two-component Dicke model with complex light-matter couplings, accounting for photon losses. We compute the steady-state phase diagram and find dynamical in- stabilities in the form of limit cycles, heralded by the presence of exceptional points and level attraction. We show that the instabilities are induced by dissipative processes that generate nonreciprocal couplings between the two collective spins. Lastly, we explore the dynamics of a BEC inside an optical cavity in the presence of an optical lattice. We derive an effective master equation by adiabatically eliminating the cavity field. In the bad-cavity regime, we find an infinite-temperature steady state, but with relaxation dynamics that can be highly nontrivial. For small hopping, the interplay between dissipation and strong interactions leads to an algebraic relaxation of the system, whereas for large hopping, the approach to the steady state is exponential. In the good- cavity regime, we show that the system allows for optical pumping between momentum modes, enabling cavity cooling.
The recent experimental observation of spinor self-ordering of ultracold atoms in optical resonators has set the stage for the exploration of emergent magnetic orders in quantum-gas−cavity systems. Based on this platform, we introduce a generic scheme for the implementation of quantum spin Hamiltonians composed of various kinds of couplings, including Heisenberg and Dzyaloshinskii-Moriya interactions. These interactions with spatially modulated coupling coefficients are mediated by cavity photons. Specifically, our model is comprised of a two-component Bose-Einstein condensate, driven by two classical pump lasers and coupled to a single dynamic mode of a linear cavity in a double Λ scheme. We exemplify the emergence of an achiral antiferromagnetic domain-wall phase and a chiral spin-spiral order beyond critical laser strengths. The transition between these two phases can be observed in a single experimental setup by tuning the reflectivity of a mirror. We also discuss straightforward extensions of our scheme for the implementation of other classes of spin Hamiltonians.
Experimental platforms based on ultracold atomic gases have significantly advanced the quantum simulation of complex systems, yet the exploration of phenomena driven by long-range interactions remains a formidable challenge. Currently available methods utilizing dipolar quantum gases or multimode cavities allow us to implement long-range interactions with a 1 / r 3 character or with a spatial profile fixed by the mode structure of the vacuum electromagnetic field surrounding the atoms, respectively. Here, we propose an experimental scheme employing laser-painted cavity-mediated interactions, which enables the realization of atom-atom interactions that are fully tunable in range, shape, and sign. Our approach combines the versatility of cavity quantum electrodynamics with the precision of laser manipulation, thus providing a highly flexible platform for simulating and understanding long-range interactions in quantum many-body systems. Our analytical predictions are supported by numerical simulations describing the full dynamics of the atoms, the laser, and the cavity. These reveal the self-organization of domains in the density of the atomic cloud, confirming the finite-range nature of the induced interactions. We demonstrate that there is a wide and experimentally accessible parameter regime in which our protocol works robustly, with negligible heating of the quantum gas. The methodology not only paves the way for exploring new territories in quantum simulation but also enhances the understanding of fundamental physics, potentially leading to the discovery of novel quantum states and phases. Published by the American Physical Society 2024
The recent experimental observation of spinor self-ordering of ultracold atoms in optical resonators has set the stage for the exploration of emergent magnetic orders in quantum-gas-cavity systems. Based on this platform, we introduce a generic scheme for the implementation of long-range quantum spin Hamiltonians composed of various types of couplings, including Heisenberg and Dzyaloshinskii-Moriya interactions. Our model is composed of an effective two-component Bose-Einstein condensate, driven by two classical pump lasers and coupled to a single dynamic mode of a linear cavity in a double Λ scheme. Cavity photons mediate the long-range spin-spin interactions with spatially modulated coupling coefficients, where the latter ones can be tuned by modifying spatial profiles of the pump lasers. As experimentally relevant examples, we demonstrate that by properly choosing the spatial profiles of the pump lasers achiral domain-wall antiferromagnetic and chiral spin-spiral orders emerge beyond critical laser strengths. The transition between these two phases can be observed in a single experimental setup by tuning the reflectivity of a mirror. We also discuss extensions of our scheme for the implementation of other classes of spin Hamiltonians.
Abelian and non-Abelian gauge potentials and quantum gauge theories play central roles in our understanding of Nature. Gauge potentials are also of great significance in condensed matter physics. In fact, minimal coupling of electrons to an Abelian or non-Abelian gauge potential is the essential ingredient for the realization of topological states of matter. Due to the high controllability of ultracold atoms, they are commonly exploited to test fundamental theories of physics, simulate intractable systems, and realize exotic many-body states. Nonetheless, the charge neutrality of atoms places severe constraints on ultracold atomic systems, since neutral particles do not couple to gauge potentials the way charged particles do. That said, coupling a multi-component quantum gas to laser light can lead to the emergence of artificial Abelian and non-Abelian gauge potentials minimally coupled to the center-of-mass momenta of ultracold neutral atoms, paving the way for realizing topological states of matter and simulating gauge theories in quantum gases. All previous proposals for inducing gauge potentials have been developed in the semiclassical regime, where the radiation field is treated classically. I have developed a two-photon Raman scheme in the strong atom-photon coupling (i.e., quantum) regime, based on two counter-propagating modes of a ring cavity, to induce both synthetic magnetic field and spin-orbit coupling for a single neutral atom inside the cavity. The spin-orbit interaction is only weakly dependent on the occupation of the cavity modes, whereas the strength of the magnetic field is proportional to the square of the total number of photons in the cavity and can be made arbitrarily large, which is desirable for realizing the quantum Hall phase. I have then extended this single-atom cavity quantum-electrodynamics scheme to many bosons in the weak atom-photon coupling regime. In addition to inducing spin-orbit coupling for the individual atoms, the cavity fields also mediate infinite-ranged interactions between atoms, whose strengths and signs can readily be tuned experimentally. The interplay between these cavity-mediated interactions and the intrinsic two-body interactions determines the many-body ground state and its elementary excitations, with novel consequences such as the stabilization of an attractive Bose-Einstein condensate which otherwise is unstable.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.