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arXiv:2508.08164 · Physical Review A

Atomic thermometry in optical lattice clocks: Model discrepancies and their impact on lattice light shifts

Irene Goti, Tommaso Petrucciani, Stefano Condio, Filippo Levi, Davide Calonico, Marco Pizzocaro

Published Oct 19, 2026• 0 citations
arXivHTMLPDF

Abstract

Accurate measurement of atomic temperature is fundamental for a wide range of applications, from quantum sensing to precision metrology. In optical lattice clocks, precise characterization of atomic temperature is required to minimize systematic uncertainties at the $10^{-18}$ level. In this work, we investigate atomic temperature measurements in the ytterbium optical clock developed at INRIM, IT-Yb1, employing sideband and transverse Doppler spectroscopy across a wide range of trapping conditions in a one-dimensional optical lattice. By implementing clock-line-mediated Sisyphus cooling [Phys. Rev. Lett. 133, 053401 (2024)], we reduce the atomic temperature and enable operation at shallower lattice depths down to $D = 50\,E_\text{R}$, where $E_\text{R}$ is the photon recoil energy. We compare temperature estimates obtained from the perturbed harmonic oscillator model with those derived using a Born-Oppenheimer model [Phys. Rev. A 101, 053416 (2020)]. Discrepancies of up to a factor of four are observed between the temperature estimates obtained with the two approximations. We assess the impact of these modeling differences on the evaluation of lattice light shifts and find relative frequency deviations of up to $8\times10^{-17}$. Although sufficiently low atomic temperatures and the consistent use of theoretical models reduce these discrepancies to the low $10^{-18}$ level, these results motivate further investigations that will be relevant to state-of-the-art optical lattice clocks.

DOI
10.1103/nzhn-34tp

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Accurate measurement of atomic temperature is fundamental for a wide range of applications, from quantum sensing to precision metrology. In optical lattice clocks, precise characterization of atomic temperature is required to minimize systematic uncertainties at the 10−1810^{-18}10−18 level. In this work, we investigate atomic temperature measurements in the ytterbium optical clock developed at INRIM, IT-Yb1, employing sideband and transverse Doppler spectroscopy across a wide range of trapping conditions in a one-dimensional optical lattice. By implementing clock-line-mediated Sisyphus cooling [Phys. Rev. Lett. 133, 053401 (2024)], we reduce the atomic temperature and enable operation at shallower lattice depths down to D=50 ERD = 50\,E_\text{R}D=50ER​, where ERE_\text{R}ER​ is the photon recoil energy. We compare temperature estimates obtained from the perturbed harmonic oscillator model with those derived using a Born-Oppenheimer model [Phys. Rev. A 101, 053416 (2020)]. Discrepancies of up to a factor of four are observed between the temperature estimates obtained with the two approximations. We assess the impact of these modeling differences on the evaluation of lattice light shifts and find relative frequency deviations of up to 8×10−178\times10^{-17}8×10−17. Although sufficiently low atomic temperatures and the consistent use of theoretical models reduce these discrepancies to the low 10−1810^{-18}10−18 level, these results motivate further investigations that will be relevant to state-of-the-art optical lattice clocks.
Atomic clocks constitute a fundamental tool for time and frequency metrology and their application is widespread in many technological fields. In particular, the International System of units (SI) defines the second on a microwave transition of Caesium atoms. The realization is made by clocks reaching uncertainties of few parts in 10^−16, making the second to be the quantity realized with the smallest uncertainty in the SI. However, a new generation of atomic clocks, called optical clocks, have already demonstrated to surpass Caesium standards both in accuracy and stability. The research performed during my PhD activity has been focused on the development and characterization of Ytterbium (Yb) optical lattice clocks. These systems operate with a large number of ultra-cold neutral atoms having a clock transition in the visible region of the electromagnetic spectrum. The atomic sample is trapped in an periodical optical potential called optical lattice that gives the advantage to interrogate many quantum absorbers for an extended time, with small perturbations, allowing to achieve an unprecedented stability and accuracy. The main experimental work has been carried out in the laboratories of the Istituto Nazionale di Ricerca Metrologica (INRIM) in Turin, where several atomic clocks are present including the Italian primary frequency standard, the Caesium fountain ITCsF2, and where an Yb optical lattice clock is currently being developed. This thesis describes the functioning of the system along with the full characterization of systematic effects, the complete uncertainty budget and its first absolute frequency measurement against the primary frequency standard. The clock exhibited an accuracy of 1.6 × 10^−16 and the comparison with the Cs fountain resulted in a frequency of f171Yb = 518 295 836 590 863.59(31) Hz, limited by the fountain uncertainty. This measurement is in agreement with the ytterbium frequency recommended as a secondary representation of the second in the SI and constitutes the first measurement of a Yb clock in Europe and the second one in the world against a primary frequency standard. Several upgrades have been applied after the absolute measurement. In particular, the design and realization a system capable to frequency stabilize several lasers on a single optical cavity is illustrated. This cavity has been implemented to lock the lasers used to cool and trap the atomic sample at 399, 556 and 759nm using the offset sideband locking technique, a modified version of the Pound–Drever–Hall method that gives an extended frequency tunability. The system proved to be an easy-to-use and reliable tool for the experimental activity showing a linewidth below 300 Hz at 556nm, which is the wavelength that requires the most stringent performance, and a long term drift below 20 kHz per day at 759nm. That is suitable for operating the lattice laser with a light shift uncertainty below 1 × 10−18. During my PhD I have been guest researcher at the National Institute of Standards and Technology (NIST) of Boulder, Colorado, for nine months in 2016. In these laboratories two Yb optical lattice clocks are operative. I worked on the instability measurement of a composite system exploiting the two clocks to suppress the Dick effect, called zero-dead-time (ZDT) clock, which demonstrated a fractional instability of 3 × 10−17 at 1s. The two clocks can also be operated to extend the interrogation time obtaining a spectroscopic feature after 4 s of 120(20)mHz corresponding to a quality factor Q > 4 × 10^15. I also worked on the characterization of several systematic shifts that allowed to complete the uncertainty budget of the clocks at 1.6 × 10^−18. In particular, I contributed to the characterization of lattice light shifts considering the effect of atomic sample temperature and the identification of a metrological regime called operational magic frequency where frequency shifts are insensitive to changes in trap depth.
An optical lattice clock probes a spectrally narrow electronic transition in an ensemble of optically trapped, laser-cooled atoms, for use as a time and frequency standard. To date, several lattice clocks have been demonstrated with superior stability and accuracy compared to primary frequency standards based on microwave transitions. Yet, the question of which atomic system (including the element and isotope) performs best as a lattice clock remains unsettled. This thesis describes the first detailed investigation of an optical lattice clock using a spin-1/2 isotope of the ytterbium atom. A spin-1/2 system possesses several advantages over higher-spin systems, including a simplified level structure (allowing for straightforward manipulation of the nuclear spin state) and the absence of any tensor light shift from the confining optical lattice. Moreover, the ytterbium atom (Yb) stands among the leading lattice clock candidates, offering a high-performance optical clock with some degree of experimental simplicity. The frequency stability of the Yb clock is highlighted by resolving an ultra-narrow clock spectrum with a full-width at half-maximum of 1 Hz, corresponding to a record quality factor Q = ν0/Δν = 5 × 1014. Moreover, this system can be highly accurate, which is demonstrated by characterizing the Yb clock frequency at the 3 × 10-16 level of fractional uncertainty, with further progress toward a ten-fold improvement also presented. To reach this low level of uncertainty required careful consideration of important systematic errors, including the identification of the Stark-canceling wavelength, where the clock’s sensitivity to the lattice intensity is minimized, a precise determination of the static polarizability of the clock transition, and the measurement and control of atom-atom collisions.
Optical lattice clocks have demonstrated unprecedented performance below the 10^-18 fractional level, advancing towards new standards of timekeeping and sensitive probes in fundamental physics. To further advance optical lattice clocks performance, it is crucial to attain lower temperatures which facilitates the use of shallow lattices with reduced light shifts, while retaining large atom numbers to reduce the quantum projection noise. Here, we present Sisyphus cooling using the long-lived 3P0 clock state in alkaline-earth-like ytterbium. Upon excitation on the ultranarrow clock transition, Sisyphus cooling is observed within a spatially periodic potential induced by a 1388-nm optical standing wave that is nearly resonant with the 3P0 → 3D1 transition. Our cooling demonstrates versatility, working both in free space and in a magic-wavelength lattice. It offers the flexibility of being employed in either pulsed or continuous modes, making it suitable to a range of quantum metrology applications.
Optical clocks benefit from tight atomic confinement enabling extended interrogation times as well as Doppler- and recoil-free operation. However, these benefits come at the cost of frequency shifts that, if not properly controlled, may degrade clock accuracy. Numerous theoretical studies have predicted optical lattice clock frequency shifts that scale nonlinearly with trap depth. To experimentally observe and constrain these shifts in an ^{171}Yb optical lattice clock, we construct a lattice enhancement cavity that exaggerates the light shifts. We observe an atomic temperature that is proportional to the optical trap depth, fundamentally altering the scaling of trap-induced light shifts and simplifying their parametrization. We identify an "operational" magic wavelength where frequency shifts are insensitive to changes in trap depth. These measurements and scaling analysis constitute an essential systematic characterization for clock operation at the 10^{-18} level and beyond.
A Wannier-Stark optical lattice clock has demonstrated unprecedented measurement precision for optical atomic clocks. We present a systematic evaluation of the lattice light shift, a necessary next step for establishing this system as an accurate atomic clock. With precise control of the atomic motional states in the lattice, we report accurate measurements of the multipolar and the hyperpolar contributions and the operational lattice light shift with a fractional frequency uncertainty of 3.5×10^{-19}.
For atoms or molecules in optical lattices, conventional thermometry methods are often unsuitable due to low particle numbers or a lack of cycling transitions. However, a differential spectroscopic light shift can map temperature onto the line shape with a low sensitivity to trap anharmonicity. We study narrow molecular transitions to demonstrate precise frequency-based lattice thermometry, as well as carrier cooling. This approach should be applicable down to nanokelvin temperatures. We also discuss how the thermal light shift can affect the accuracy of optical lattice clocks.