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arXiv:2507.20692 · Physical review. B./Physical review. B

Dynamical phase transition in a strongly hybridized phonon-triplon chain

Mohsen Yarmohammadi

Published Oct 6, 2025• 5 citations
arXivHTMLPDF

Abstract

We study a dimerized spin-1/2 chain, such as ${\mathrm{CuGeO}}_{3}$, hosting triplon excitations coupled to optical phonons under weak terahertz laser driving. Both phonons and triplons weakly lose energy into the surrounding baths, forming a nonequilibrium steady state. In the strong phonon-triplon coupling regime, phonons near the two-triplon continuum hybridize strongly with triplons. Using mean-field Lindblad dynamics, we show that strong hybridization induces sharp first-order phase transitions---either single or simultaneous double---in the emission spectrum, mainly due to nonlinearities in the chain and the instantaneous breaking of spatial inversion symmetry, as captured by the phonon displacement. Using mean-field Floquet analysis of harmonic modes in both sectors, we analytically confirm the existence of these phase transitions. Furthermore, we map the complete steady-state phase diagram by varying key control parameters and provide experimentally relevant parameters for observing these transitions in laser-driven ${\mathrm{CuGeO}}_{3}$.

DOI
10.1103/c3tb-h5hv

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We study a dimerized spin-1/2 chain, such as CuGeO3{\mathrm{CuGeO}}_{3}CuGeO3​, hosting triplon excitations coupled to optical phonons under weak terahertz laser driving. Both phonons and triplons weakly lose energy into the surrounding baths, forming a nonequilibrium steady state. In the strong phonon-triplon coupling regime, phonons near the two-triplon continuum hybridize strongly with triplons. Using mean-field Lindblad dynamics, we show that strong hybridization induces sharp first-order phase transitions---either single or simultaneous double---in the emission spectrum, mainly due to nonlinearities in the chain and the instantaneous breaking of spatial inversion symmetry, as captured by the phonon displacement. Using mean-field Floquet analysis of harmonic modes in both sectors, we analytically confirm the existence of these phase transitions. Furthermore, we map the complete steady-state phase diagram by varying key control parameters and provide experimentally relevant parameters for observing these transitions in laser-driven CuGeO3{\mathrm{CuGeO}}_{3}CuGeO3​.
In the realm of open quantum systems, steady states and high-harmonic generation (HHG) existing far from equilibrium have become core pillars of ultrafast science. Most solid-state research explores charge HHG with limited investigations into spin degrees of freedom. In this study, we theoretically address spin HHG in the steady state resulting from the terahertz laser-driven spin-phonon coupling in a dissipative dimerized spin-1/2 chain. Instead of directly driving spins using time-dependent magnetic fields, we employ the magnetophononic mechanism, where the laser first drives the lattice, and then the excited lattice subsequently drives the spins. We investigate the role of various model parameters for optimizing HHG. Increasing the laser amplitude amplifies spin HHG beyond the perturbative regime, enhancing both harmonic amplitudes and orders. We find that configuring the drive frequency far below the spin band yields the highest harmonic order. Additionally, we provide a theory matching the numerical results under weak spin-phonon coupling and propose an experimental procedure to probe the emission spectrum of spin HHG.
We consider the dynamical properties of a gapped quantum spin system coupled to the electric field of a laser, which drives the resonant excitation of specific phonon modes that modulate the magnetic interactions. We deduce the quantum master equations governing the time-evolution of both the lattice and spin sectors, by developing a Lindblad formalism with bath operators providing an explicit description of their respective phonon-mediated damping terms. We investigate the nonequilibrium steady states (NESS) of the spin system established by a continuous driving, delineating parameter regimes in driving frequency, damping, and spin-phonon coupling for the establishment of physically meaningful NESS and their related nontrivial properties. Focusing on the regime of generic weak spin-phonon coupling, we characterize the NESS by their frequency and wave-vector content, explore their transient and relaxation behavior, and discuss the energy flow, the system temperature, and the critical role of the type of bath adopted. Our study lays a foundation for the quantitative modeling of experiments currently being designed to control coherent many-body spin states in quantum magnetic materials.
We study the direct laser drive of infrared-active phonons that are quadratically coupled to a spinless fermion chain. Feedback is incorporated by phonon dressing of the electronic dispersion, which enables effective nonlinearities in the phonon dynamics. We uncover a first-order phase transition in the phononic steady state in which hysteretic effects allow either large or small phonon occupation depending on the drive protocol. We discuss the implications of these findings for probing phase transitions in real driven materials.
We perform a systematic analysis of the influence of phonon driving on the superconducting Hol- stein model coupled to heat baths by studying both the transient dynamics and the nonequilibrium steady state (NESS) in the weak and strong electron-phonon coupling regimes. Our study is based on the nonequilibrium dynamical mean-field theory, and for the NESS we present a Floquet formu- lation adapted to electron-phonon systems. The analysis of the phonon propagator suggests that the effective attractive interaction can be strongly enhanced in the parametric resonant regime because of the Floquet side bands. While this may be expected to enhance the superconductivity (SC), our fully self-consistent calculations, which include the effects of heating and nonthermal distributions, show that the parametric phonon driving generically results in a suppression or complete melting of the SC order. In the strong coupling regime, the NESS always shows a suppression of the SC gap, the SC order parameter and the superfluid density as a result of the driving, and this tendency is most prominent at the parametric resonance. Using the real-time nonequilibrium DMFT formalism, we also study the dynamics towards the NESS, which shows that the heating effect dominates the transient dynamics, and SC is weakened by the external modulations, in particular at the parametric resonance. In the weak coupling regime, we find that the SC fluctuations above the transition tem- perature are generally weakened under the driving. The strongest suppression occurs again around the parametric resonance because of the efficient energy absorption.
We investigate nonequilibrium criticality and chaos in a two-photon-driven optomechanical system. The parametric drive preserves a discrete Z2\mathbb{Z}_2Z2​ symmetry of the optical field, while radiation-pressure coupling transfers the resulting nonlinear dynamics to a mechanical oscillator. Combining semiclassical stability analysis, exact Liouvillian spectra, and stochastic quantum trajectories, we show that this driven-dissipative optomechanical model supports both first- and second-order dissipative phase transitions. At negative detuning a second-order transition yields spontaneous breaking of the cavity-parity symmetry in the thermodynamic limit. At positive detuning the same symmetry breaking coexists with a first-order transition, signaled by metastability and by an additional symmetric Liouvillian mode. At stronger pump power the mean-field dynamics loses all stable fixed points and develops limit cycles and chaotic attractors with positive Lyapunov exponent. Quantum trajectories in this regime display chaotic-like motion, enhanced steady-state entropy, and delocalization over many entropic Liouvillian modes. These results establish two-photon-driven optomechanics as a platform where dissipative criticality, symmetry breaking, and quantum signatures of chaos emerge within the same experimentally accessible setting.
We find nonequilibrium phase transitions accompanied by multiple (nested) hysteresis behaviors in superconductors coupled to baths under a time-periodic light driving. The transitions are demonstrated with a full phase diagram in the domain of the driving amplitude and frequency by means of the Floquet many-body theory. In the weak-driving regime with a frequency smaller than half of the superconducting gap, excited quasiparticles are accumulated at the far edges of the bands, realizing a distribution reminiscent of the Eliashberg effect, which suddenly becomes unstable in the strong-driving regime due to multiphoton-assisted tunneling across the gap mediated by the in-gap Floquet sidebands. We also show that superconductivity is enhanced in the weak-driving regime without effective cooling, which is attributed to the modulation of the spectrum due to Floquet sidebands.