Nondestructive spin-resolved imaging of ultracold atomic gases requires calculating the differences of the refractive indices seen by two circular probe polarizations. Perfect overlap of the two images, corresponding to two different polarizations, is required well below the feature size of interest. In this paper, we demonstrate that the birefringence of atoms in magnetic field gradients results in polarization-dependent aberrations in the image, which deteriorates the overlap. To that end, we develop a model that couples atomic tensor polarizability with position-dependent spin orientation and yields aberration predictions for accumulated phase shifts in arbitrary field geometries. Applied to data from an ultra-cold atomic cloud trapped in a Ioffe-Pritchard trap, the model quantitatively reproduces the observed distortion across a range of temperatures. A residual offset of \sim1\;\mu\mathrm{m} ∼ 1 μ m remains even under uniform field conditions, likely due to optical asymmetries. For images obtained through off-axis holography, the full complex field of the probe enables post-processing removal of all magnetically induced aberrations through a single numerically calculated Fourier-space phase mask.
Nondestructive spin-resolved imaging of ultracold atomic gases requires calculating the differences of the refractive indices seen by two circular probe polarizations. Perfect overlap of the two images, corresponding to two different polarizations, is required well below the feature size of interest. In this paper, we demonstrate that the birefringence of atoms in magnetic field gradients results in polarization-dependent aberrations in the image, which deteriorates the overlap. To that end, we develop a model that couples atomic tensor polarizability with position-dependent spin orientation and yields aberration predictions for accumulated phase shifts in arbitrary field geometries. Applied to data from an ultra-cold atomic cloud trapped in a Ioffe-Pritchard trap, the model quantitatively reproduces the observed distortion across a range of temperatures. A residual offset of \sim1;\mu\mathrm{m} ∼ 1 μ m remains even under uniform field conditions, likely due to optical asymmetries. For images obtained through off-axis holography, the full complex field of the probe enables post-processing removal of all magnetically induced aberrations through a single numerically calculated Fourier-space phase mask.
We introduce a noninvasive imaging technique based on spin-dependent off-axis holography for spin-1 Bose-Einstein condensates. Utilizing a dual reference beam strategy, this method records two orthogonal circular polarization components of a single probe beam. The circular birefringence of spin-polarized atoms induces differing complex phase shifts in the polarization components of the light, which are reconstructed from the interference patterns captured on camera. Our approach enables spin- and density-resolved imaging of both phase and amplitude information in situ on a submillisecond timescale with minimal disturbance to the condensate. We explore the technique's efficacy under various background static fields, demonstrating its sensitivity to the quantization axis of the atoms and confirming its effectiveness.
In this thesis, we develop, validate and apply a non-destructive, spin-sensitive probing method for ultracold gases of sodium. By exploiting the polarization dependence of the atom-light interaction, the method combines optical hardware with computational reconstruction to access spin-resolved density and magnetization distributions from a single, minimally destructive exposure. The thesis is structured in three parts; firstly, we describe the experimental platform for making, probing and manipulating sodium spinor Bose–Einstein condensates, including laser cooling, optical and magnetic trapping, and radio-frequency techniques for coherent spin preparation. In the second part, we develop the core measurement technique of spin-dependent off-axis holography is developed, and evaluate its robustness to technical noise and the magnetic field variations. The reconstruction and analysis pipeline is presented in detail, with special emphasis on the background noise suppression using an inpainting technique based on principal component analysis. In the final part, the method is applied to investigate dynamics in spin-1 ultracold atomic sodium. To that end, we introduce the theory of three-level spin systems and propose magnetization-preparation and precise Zeeman-sublevel readout schemes, which are experimentally verified. These tools are then used to investigate spin diffusion and spin mixing dynamics, and the formation and evolution of spin domains. This work establishes spin-dependent off-axis holography as a powerful tool for probing spinor quantum gases. The techniques developed here enable efficient and minimally destructive imaging of spin dynamics, and provide new opportunities for studying non-equilibrium spin phenomena and magnetism in ultracold atomic systems.
We introduce a novel, non-invasive imaging technique based on spin-dependent off-axis holography (SOAH) for spin-1 Bose-Einstein condensates (BECs). Utilizing a dual reference beam strategy, this method records two orthogonal circular polarization components of a single probe beam. The circular birefringence of spin-polarized atoms induces differing complex phase shifts in the polarization components of the light, which are reconstructed from the interference patterns captured on camera. Our approach enables spin- and density-resolved imaging of both phase and amplitude information \emph{in-situ} on a sub-millisecond time scale with minimal disturbance to the condensate. We explore the technique's efficacy under various background static fields, demonstrating its sensitivity to the quantization axis of the atoms and confirming its effectiveness.
In this thesis, we develop, validate and apply a non-destructive, spin-sensitive probing method for ultracold gases of sodium. By exploiting the polarization dependence of the atom-light interaction, the method combines optical hardware with computational reconstruction to access spin-resolved density and magnetization distributions from a single, minimally destructive exposure. The thesis is structured in three parts; firstly, we describe the experimental platform for making, probing and manipulating sodium spinor Bose–Einstein condensates, including laser cooling, optical and magnetic trapping, and radio-frequency techniques for coherent spin preparation. In the second part, we develop the core measurement technique of spin-dependent off-axis holography is developed, and evaluate its robustness to technical noise and the magnetic field variations. The reconstruction and analysis pipeline is presented in detail, with special emphasis on the background noise suppression using an inpainting technique based on principal component analysis. In the final part, the method is applied to investigate dynamics in spin-1 ultracold atomic sodium. To that end, we introduce the theory of three-level spin systems and propose magnetization-preparation and precise Zeeman-sublevel readout schemes, which are experimentally verified. These tools are then used to investigate spin diffusion and spin mixing dynamics, and the formation and evolution of spin domains. This work establishes spin-dependent off-axis holography as a powerful tool for probing spinor quantum gases. The techniques developed here enable efficient and minimally destructive imaging of spin dynamics, and provide new opportunities for studying non-equilibrium spin phenomena and magnetism in ultracold atomic systems.
Polarization-dependent phase-contrast imaging is used to resolve the spatial magnetization profile of an optically trapped ultracold gas. This probe is applied to Larmor precession of degenerate and nondegenerate spin-1 87Rb gases. Transverse magnetization of the Bose-Einstein condensate persists for the condensate lifetime, with a spatial response to magnetic field inhomogeneities consistent with a mean-field model of interactions. In comparison, the magnetization of the non-condensed gas decoheres rapidly. Rotational symmetry implies that the Larmor frequency of a spinor condensate be density independent, and thus suitable for precise magnetometry with high spatial resolution.
This thesis presents a novel magnetic resonance imaging (MRI) technique for spinor Bose-Einstein condensates (BEC) with the paramagnetic Faraday effect. This quantum-photon interface couples the spin of the BEC to the polarisation of an off-resonant laser, which in a magnetic field gradient allows a 1D density profile of the BEC to be reconstructed. As opposed to conventional imaging techniques that are destructive or diffraction limited, this technique is minimally destructive to the BEC and not diffraction limited. Multishot in situ imaging of a single condensate is therefore possible, paving the way for time-resolved studies and 2D/3D reconstructions. A theoretical model for Faraday imaging is developed using the tensor polarisability formalism for the atom-light interaction, and the signal-to-noise ratio is derived. Resolution limits induced by Stern-Gerlach separation are considered, encouraging rapid measurements with strong magnetic field gradients. Analysing the trapping potential reveals that the `magic-zero' wavelength 790nm produces no dipole force and enables a tightly focused probe laser to be used without perturbing the trap. Polarisation-maintaining fibers were seen to impart large fluctuations depending on the incident polarisation, which were minimised. The broad diode laser emission background is seen to reduce the lifetime of the BEC, which was corrected with an interference filter. Short-time Fourier transforms are used to process the photodetected signal, showing the evolution of the polarisation rotation frequency and amplitude. Frequency-modulation is observed at the power line frequency, corresponding to magnetic field fluctuations induced by nearby equipment. Birefringence of optical elements results in elliptical polarisation of the probe and an effective magnetic field, which is cancelled using a quarter-waveplate. The quadratic Zeeman effect causes rapid amplitude modulation, and is eliminated by applying a microwave dressing field. Radiative spin echo is achieved in a magnetic field gradient, proving that dephasing is coherent, and that multishot imaging possible. Magnetic resonance imaging (MRI) is performed on a partially-evaporated atom cloud, distinguishing the thermal and condensed fractions. A split dipole trap is used to create two spatially separated BECs, which are individually resolved during MRI. The resolution is only limited by the strength of the applied magnetic field gradient, and is not subject to the diffraction limit. Custom coils will enable MRI of condensates at the sub-micron scale.