We introduce a quantum channel to model the dissipative dynamics resulting from the coupling between spin and motional degrees of freedom in chains of neutral atoms with Rydberg interactions. The quantum channel acts on the reduced spin state obtained under the frozen gas approximation, modulating its elements with time-dependent coefficients. These coefficients can be computed exactly in the perturbative regime, enabling efficient modeling of spin-motion dephasing in systems too large for exact methods. We benchmark the accuracy of our approach against exact diagonalization for small systems, identifying its regime of validity and the onset of perturbative breakdown. We then apply the quantum channel to compute fidelity loss during transport of single-spin excitations across extended Rydberg chains in regimes intractable via exact diagonalization. By revealing the quantum-classical crossover, these results establish a bound on the maximum chain length for efficient entanglement distribution. The quantum channel significantly reduces the complexity of simulating spin dynamics coupled to motional degrees of freedom, providing a practical tool for estimating the impact of spin-motion coupling in near-term experiments with Rydberg atom arrays.
We introduce a quantum channel to model the dissipative dynamics resulting from the coupling between spin and motional degrees of freedom in chains of neutral atoms with Rydberg interactions. The quantum channel acts on the reduced spin state obtained under the frozen gas approximation, modulating its elements with time-dependent coefficients. These coefficients can be computed exactly in the perturbative regime, enabling efficient modeling of spin-motion dephasing in systems too large for exact methods. We benchmark the accuracy of our approach against exact diagonalization for small systems, identifying its regime of validity and the onset of perturbative breakdown. We then apply the quantum channel to compute fidelity loss during transport of single-spin excitations across extended Rydberg chains in regimes intractable via exact diagonalization. By revealing the quantum-classical crossover, these results establish a bound on the maximum chain length for efficient entanglement distribution. The quantum channel significantly reduces the complexity of simulating spin dynamics coupled to motional degrees of freedom, providing a practical tool for estimating the impact of spin-motion coupling in near-term experiments with Rydberg atom arrays.
We numerically study the transport of Rydberg excitations in chains of neutral atoms. We realize an effective flip-flop interaction using off-resonant driving fields. By tuning the relative distances between atoms and applying atom-selective detuning fields, we fulfill the perfect transport condition. This condition enables the transfer of a single Rydberg excitation from one end of the chain to the other, allowing the distribution of entanglement across the chain at the quantum speed limit. Through numerical simulations, we identify the set of control parameters that maximizes the transport probability under experimentally relevant conditions. We study the various competing trade-offs involved in the hierarchy of approximations used to map the native Rydberg spin model onto the effective model driving spin transport. Our results suggest that entanglement can be distributed over chains of more than 50 atoms spanning hundreds of microns at room temperature. This study informs the selection of parameters for the experimental realization of perfect transport in Rydberg chains, providing an approach to distribute entanglement among distant atoms in quantum processors.
This thesis explores the effects of decoherence and dephasing on single- and many- body dynamics of spin-systems. A particular realisation of the spin systems that the work focuses on are highly excited, Rydberg states of atoms. A software library ARC (Alkali Rydberg Calculator) for calculating properties of Rydberg states in alkali metals is presented, with particular attention to the multi- atom and multi-level effects that influence many-body dynamics in realistic systems, and properties related to terahertz imaging with alkali atom Rydberg states. Dressed-state electromagnetically induced transparency (EIT) is proposed as a way of preparing uniform-phase spin-waves in ladder excitation schemes, making the collective excitation storage insensitive to motional dephasing. Proof of concept dressed state EIT experiments are presented. Strong resonant dressing is also theoretically analysed as a way of preparing velocity superposition of spin-waves. The developed theoretical model is in a good agreement with existing experimental data on single-photon many-atom quantum beats in diamond excitation schemes. By modelling the strongly driven Rydberg ensembles, many-body dynamics of driven-dissipative spin systems is analysed. Working in the limit of strong dephasing, the effects of fluctuations, the shape of interaction potential, spatial correlations and motion on non-equilibrium phase diagrams and the occurrence of bistability are examined. An ensemble averaged mean field model is introduced as an exact solution for completely uncorrelated ensembles. It is shown that the van der Waals interaction does not allow the occurrence of bistability, for which a finite dipolar core is required. The short-range interaction potential shape is found to have a profound influence on non-equilibrium phase diagrams, controlling the size of fluctuations in the dynamics. For a frozen system, several methods for identifying and quantifying bistable phases are introduced, and phase diagrams are reconstructed. It is shown that the temperature of external degrees of freedom, i.e. spin motion, can drive a non-equilibrium transition into the bistable phase.
Noise and decoherence are ubiquitous in the dynamics of quantum systems coupled to an external environment. In the regime where environmental correlations decay rapidly, the evolution of a subsytem is well described by a Lindblad quantum master equation. In this work, we introduce a quantum algorithm for simulating unital Lindbladian dynamics by sampling unitary quantum channels without extra ancillas. Using ancillary qubits we show that this algorithm allows approximating general Lindbladians as well. For interacting dephasing Lindbladians coupling two subsystems, we develop a decoupling scheme that reduces the circuit complexity of the simulation. This is achieved by sampling from a time-correlated probability distribution - determined by the evolution of one subsystem, which specifies the stochastic circuit implemented on the complementary subsystem. We demonstrate our approach by studying a model of bosons coupled to fermions via dephasing, which naturally arises from anharmonic effects in an electron-phonon system coupled to a bath. Our method enables tracing out the bosonic degrees of freedom, reducing part of the dynamics to sampling an IQP circuit. The sampled bitstrings then define a corresponding fermionic problem, which in the non-interacting case can be solved efficiently classically. We comment on the computational complexity of this class of dissipative problems, using the known fact that sampling from IQP circuits is believed to be difficult classically.
Abstract To transport high-quality quantum state between two distant qubits through one-dimensional spin chains, the perfect state transfer (PST) method serves as the first choice, due to its natively perfect transfer fidelity that is independent of the system dimension. However, the PST requires a precise modulation of the local pulse parameters as well as an accurate timing of dynamic evolution, and is thus very sensitive to variations in practice. Here, we propose a protocol for achieving quantum-preserved transport of excitations using an array of Rydberg-dressed atoms, enabled by optimal control of minimally global parameters. By treating the weak coupling of two marginal array atoms as a perturbation, an effective spin-exchange model with highly tunable interactions between the external weak and the inner strong driving atoms can be established, which allows for coherent excitation transfer even with large atomic position fluctuation. We furthermore show that the existence of long-time excitation propagation unattainable for systems under antiblockade facilitation conditions. Our results highlight an easily-implemented scheme for studying the dynamics of spin systems using Rydberg atoms and may guide the avenue to the engineering of complex many-body dynamics.
In the first part of this thesis, we investigate the dynamics of open quantum systems coupled in a purely dephasing way to their environment, which is a paradigmatic example of decoherent dynamics. We focus more specifically on the emergence of non-Markovian effects in the dynamics of such open systems. After reviewing different measures of non-Markovianity, we obtain an analytical expression for the reduced density operator of a finite-dimensional open system coupled with its environment through time-dependent purely dephasing interactions. When the system is initially uncorrelated with its environment, we obtain the time-local master equation that describes its dynamics. In this case, we also derive an exact expression for the witness of non-Markovianity based on the volume of accessible states of the open system. These results are then applied to spin systems coupled to either a spin or a bosonic environment. For spin environments, we study non-Markovianity for different ranges of interaction and in different thermodynamical limits. Moreover, the generation of entanglement between the open system and its environment as well as between spins within the open system is investigated. For bosonic environments, we study the effect of the initial state of the environment on non-Markovianity. We also show that time-dependent modulations of the system-environment coupling can dramatically alter the non-Markovian behavior of the open system. Finally, we consider the case of an open quantum system simultaneously coupled to spin and bosonic baths. In that case, we study how the coupling between the different baths and of the presence of initial correlations in the environment affect the non-Markovianity displayed by the open quantum system. The second part of this thesis is a contribution to the investigation of how quantum systems can be used to process information. More precisely, we focus on the implementation of gate-based quantum computing using neutral atoms trapped in optical or magnetic lattices and interacting through dipole-dipole interactions when excited to Rydberg states. In this context, we present protocols implementing two-qubit quantum gates between atoms far apart in the lattice. To this end, we propose to use a chain of non-coding ancilla atoms to transfer the state of the control qubit to an atom near the target qubit. Before discussing entangling gates between distant qubits, we present two protocols that implement state transfer along a chain of two-level atoms relying respectively on single- and two-atom laser pulses combined with dipole blockade. After reviewing protocols implementing CZ and CNOT gates between nearby qubits using dipole-dipole interactions, we show how the state-transfer protocols previously presented can be used to perform entangling gates between distant qubits. The performance of the state-transfer and gate protocols are assessed using the process fidelity. Moreover, we provide a theoretical explanation for the behavior of the process fidelity with respect to dissipation and imperfect blockade.
We investigate the evolution of interacting Rydberg gases in the limit of strong noise and dissipation. Starting from a description in terms of a Markovian quantum master equation we derive effective equations of motion that govern the dynamics on a 'coarse-grained' timescale where fast dissipative degrees of freedom have been adiabatically eliminated. Specifically, we consider two scenarios which are of relevance for current theoretical and experimental studies—Rydberg atoms in a two-level (spin) approximation subject to strong dephasing noise as well as Rydberg atoms under so-called electromagnetically induced transparency (EIT) conditions and fast radiative decay. In the former case we find that the effective dynamics is described by classical rate equations up to second order in an appropriate perturbative expansion. This drastically reduces the computational complexity of numerical simulations in comparison to the full quantum master equation. When accounting for the fourth order correction in this expansion, however, we find that the resulting equation breaks the preservation of positivity and thus cannot be interpreted as a proper classical master rate equation. In the EIT system we find that the expansion up to second order retains information not only on the 'classical' observables, but also on some quantum coherences. Nevertheless, this perturbative treatment still achieves a non-trivial reduction of complexity with respect to the original problem.