In the first part of this thesis, we investigate the dynamics of open quantum systems coupled in a purely dephasing way to their environment, which is a paradigmatic example of decoherent dynamics. We focus more specifically on the emergence of non-Markovian effects in the dynamics of such open systems. After reviewing different measures of non-Markovianity, we obtain an analytical expression for the reduced density operator of a finite-dimensional open system coupled with its environment through time-dependent purely dephasing interactions. When the system is initially uncorrelated with its environment, we obtain the time-local master equation that describes its dynamics. In this case, we also derive an exact expression for the witness of non-Markovianity based on the volume of accessible states of the open system. These results are then applied to spin systems coupled to either a spin or a bosonic environment. For spin environments, we study non-Markovianity for different ranges of interaction and in different thermodynamical limits. Moreover, the generation of entanglement between the open system and its environment as well as between spins within the open system is investigated. For bosonic environments, we study the effect of the initial state of the environment on non-Markovianity. We also show that time-dependent modulations of the system-environment coupling can dramatically alter the non-Markovian behavior of the open system. Finally, we consider the case of an open quantum system simultaneously coupled to spin and bosonic baths. In that case, we study how the coupling between the different baths and of the presence of initial correlations in the environment affect the non-Markovianity displayed by the open quantum system. The second part of this thesis is a contribution to the investigation of how quantum systems can be used to process information. More precisely, we focus on the implementation of gate-based quantum computing using neutral atoms trapped in optical or magnetic lattices and interacting through dipole-dipole interactions when excited to Rydberg states. In this context, we present protocols implementing two-qubit quantum gates between atoms far apart in the lattice. To this end, we propose to use a chain of non-coding ancilla atoms to transfer the state of the control qubit to an atom near the target qubit. Before discussing entangling gates between distant qubits, we present two protocols that implement state transfer along a chain of two-level atoms relying respectively on single- and two-atom laser pulses combined with dipole blockade. After reviewing protocols implementing CZ and CNOT gates between nearby qubits using dipole-dipole interactions, we show how the state-transfer protocols previously presented can be used to perform entangling gates between distant qubits. The performance of the state-transfer and gate protocols are assessed using the process fidelity. Moreover, we provide a theoretical explanation for the behavior of the process fidelity with respect to dissipation and imperfect blockade.
In the first part of this thesis, we investigate the dynamics of open quantum systems coupled in a purely dephasing way to their environment, which is a paradigmatic example of decoherent dynamics. We focus more specifically on the emergence of non-Markovian effects in the dynamics of such open systems. After reviewing different measures of non-Markovianity, we obtain an analytical expression for the reduced density operator of a finite-dimensional open system coupled with its environment through time-dependent purely dephasing interactions. When the system is initially uncorrelated with its environment, we obtain the time-local master equation that describes its dynamics. In this case, we also derive an exact expression for the witness of non-Markovianity based on the volume of accessible states of the open system. These results are then applied to spin systems coupled to either a spin or a bosonic environment. For spin environments, we study non-Markovianity for different ranges of interaction and in different thermodynamical limits. Moreover, the generation of entanglement between the open system and its environment as well as between spins within the open system is investigated. For bosonic environments, we study the effect of the initial state of the environment on non-Markovianity. We also show that time-dependent modulations of the system-environment coupling can dramatically alter the non-Markovian behavior of the open system. Finally, we consider the case of an open quantum system simultaneously coupled to spin and bosonic baths. In that case, we study how the coupling between the different baths and of the presence of initial correlations in the environment affect the non-Markovianity displayed by the open quantum system. The second part of this thesis is a contribution to the investigation of how quantum systems can be used to process information. More precisely, we focus on the implementation of gate-based quantum computing using neutral atoms trapped in optical or magnetic lattices and interacting through dipole-dipole interactions when excited to Rydberg states. In this context, we present protocols implementing two-qubit quantum gates between atoms far apart in the lattice. To this end, we propose to use a chain of non-coding ancilla atoms to transfer the state of the control qubit to an atom near the target qubit. Before discussing entangling gates between distant qubits, we present two protocols that implement state transfer along a chain of two-level atoms relying respectively on single- and two-atom laser pulses combined with dipole blockade. After reviewing protocols implementing CZ and CNOT gates between nearby qubits using dipole-dipole interactions, we show how the state-transfer protocols previously presented can be used to perform entangling gates between distant qubits. The performance of the state-transfer and gate protocols are assessed using the process fidelity. Moreover, we provide a theoretical explanation for the behavior of the process fidelity with respect to dissipation and imperfect blockade.
This thesis investigates two thematic lines of research, both underpinned by non-Markovian system-reservoir interactions in quantum optics. The overarching focus is on modelling the open system dynamics in a non-perturbative fashion, broadly on - though not restricted to - instances when the environment is structured. A theory is developed by means of enlarging the open system over environmental degrees of freedom to include memory effects in its dynamics. This is achieved using an established technique that involves mapping a bosonic environment onto a 1D chain of harmonic oscillators. Within this setting, we apply a Heisenberg equation-of-motion approach to derive an exact set coupled differential equations for the open system and a single auxiliary oscillator of the chain. The combined equations are shown to have their interpretation rooted in a quantum Markov stochastic process. Including the auxiliary chain oscillator as part of the original system then enables us to obtain an exact master equation for the enlarged system, avoiding any need for the Born-Markov approximations. Our method is valid for a dissipative two-state system, with cases of multiple excitations and added driving discussed. Separately, we apply the framework of quantum Darwinism to an atom-cavity system, and, subsequently, to a more general multiple-environment model. In both cases, the time-dependent spread of correlations between the open system and fractions of the environment is analysed during the course of the decoherence process. The degree to which information is redundant across different fractions is checked to infer the emergence of classicality. In the second case, we go further and present a decomposition of information in terms of its quantum and classical correlations. A quantitative measure of redundancy is also studied with regard to its ability to witness non-Markovian behaviour. Besides fundamental interest, our results have application to quantum information processing and quantum technologies, keeping in mind the potential beneficial use of non-Markovian effects in reservoir engineering.
This Thesis discusses the phenomenology of the dynamics of open quantum systems marked by non-Markovian memory effects. Non-Markovian open quantum systems are the focal point of a flurry of recent research aiming to answer, e.g., the following questions: What is the characteristic trait of non-Markovian dynamical processes that discriminates it from forgetful Markovian dynamics? What is the microscopic origin of memory in quantum dynamics, and how can it be controlled? Does the existence of memory effects open new avenues and enable accomplishments that cannot be achieved with Markovian processes? These questions are addressed in the publications forming the core of this Thesis with case studies of both prototypical and more exotic models of open quantum systems. In the first part of the Thesis several ways of characterizing and quantifying non-Markovian phenomena are introduced. Their differences are then explored using a driven, dissipative qubit model. The second part of the Thesis focuses on the dynamics of a purely dephasing qubit model, which is used to unveil the origin of non-Markovianity for a wide class of dynamical models. The emergence of memory is shown to be strongly intertwined with the structure of the spectral density function, as further demonstrated in a physical realization of the dephasing model using ultracold quantum gases. Finally, as an application of memory effects, it is shown that non- Markovian dynamical processes facilitate a novel phenomenon of timeinvariant discord, where the total quantum correlations of a system are frozen to their initial value. Non-Markovianity can also be exploited in the detection of phase transitions using quantum information probes, as shown using the physically interesting models of the Ising chain in a transverse field and a Coulomb chain undergoing a structural phase transition.
Quantum mechanics has both deepened our understanding of the physical reality and allowed development of quantum technologies beating their classical counterparts in efficiency, security, and sensitivity. As a major downside, the quantum properties behind these technologies are very sensitive to the effects the system’s interaction with its environment. The theory of open quantum systems describes how such interaction influences the system, and as a consequence, how the quantum features are lost, controlled, and possibly returned by manipulating the environment. This thesis begins with a short description of the most relevant features and results of the open quantum system theory. We continue by presenting some commonly used measures to quantify the information encoded in quantum systems and the correlations between spatially or temporally separated parties. The literature review ends with discussion of non-Markovianity and memory effects which combine the fields of open quantum systems and quantum information in a natural way. The rest of the thesis presents the main results of Publications I – VII. We study the memory effects and physicality conditions of open system dynamics described by the vast family of phase-covariant master equations. We show how the open quantum system picture can be exploited to design probing protocols to extract information without knowing how the probe and system interact. Such protocols are considered also from the point-of view of efficiently obtaining the information required in the probing, both in theory and by experimental implementation. The experiment serves also as evidence for applicability of recently developed geometric tools to design informationally incomplete measurements for solving so-called membership problems. We present and experimentally realize a protocol where control over intial correlations between polarization and frequency gives full freedom to implement any dephasing dynamics in the open system polarization, thus dictating how its information content changes in time. We study the two-qubit memory effects of dephasing dynamics and compare them to the effect of such noise in the transmission efficiency in superdense coding. Optimal noise configurations in different situations are found. Finally, we characterize the families of initial states for which the decay of quantum correlations depends or does not depend on the noise location.
We study analytically the non-Markovianity of a spin ensemble, with arbitrary number of spins and spin quantum number, undergoing a pure dephasing dynamics. The system is considered as a part of a larger spin ensemble of any geometry with pairwise interactions. We derive exact formulas for the reduced dynamics of the system and for its non-Markovianity as assessed by the witness of Lorenzo et al. [Phys. Rev. A 88, 020102(R) (2013)]. The non-Markovianity is further investigated in the thermodynamic limit when the environment's size goes to infinity. In this limit and for finite-size systems, we find that the Markovian character of the system's dynamics crucially depends on the range of the interactions. We also show that when the system and its environment are initially in a product state, the appearance of non-Markovianity is independent of the entanglement generation between the system and its environment.
We consider the buildup and decay of two-spin entanglement through phase interactions in a finite environment of surrounding spins, as realized in quantum computing platforms based on arrays of atoms, molecules, or nitrogen vacancy centers. The non-Markovian dephasing caused by the spin environment through Ising-type phase interactions can be solved exactly and compared to an effective Markovian treatment based on collision models. In a first case study on a dynamic lattice of randomly hopping spins, we find that non-Markovianity boosts the dephasing rate caused by nearest-neighbor interactions with the surroundings, degrading the maximum achievable entanglement. However, we also demonstrate that additional three-body interactions can mitigate this degradation, and that randomly timed reset operations performed on the two-spin system can help sustain a finite average amount of steady-state entanglement. In a second case study based on a model nuclear magnetic resonance system, we elucidate the role of bath correlations at finite temperature on non-Markovian dephasing. They speed up the dephasing at low temperatures while slowing it down at high temperatures, compared to an uncorrelated bath, which is related to the number of thermally accessible spin configurations with and without interactions.
To study various quantum dynamics, it is important to develop effective methods to detect and distinguish different quantum dynamics. A common non-demolition approach is to couple an auxiliary system (ancilla) to the target system, and to measure the ancilla only. By doing so, the target system becomes an environment for the ancilla. Thus, different quantum dynamics of target systems will correspond to different environment properties. Here, we analytically study XX spin chains presenting different kinds of quantum dynamics, namely localized, delocalized, and dephasing dynamics, and build connections between Markovianity and non-Markovianity-the two most common properties of an environment. For a qubit coupled to the XX chain, we derived the reduced density matrix of the qubit through the projection method. Furthermore, when dephasing noise was introduced to the XX chain, we generalized the projection method by introducing an open-system interaction picture - a modification of the Dirac interaction picture. By calculating the reduced density matrix for the qubit analytically and numerically, we found that the delocalized (localized) chain corresponds to the Markovian (non-Markovian) bath when boundary effects are not considered, and the feature of the chain with dephasing noise as a bath is dependent on the dephasing strength. The three kinds of quantum dynamics can be distinguished by measuring the qubit only.