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arXiv:2504.19679

Quantum-Noise Induced Localization and Motional Squeezing in a Rydberg Quantum Simulator

Bock, Benno, Daniel Brady, Michael Fleischhauer

Published Apr 28, 2025• 0 citations
arXivHTMLPDF

Abstract

We investigate the interplay between mechanical forces and the internal-state dynamics of Rydberg excitations in atom-tweezer arrays. Dipole interactions between Rydberg atoms facilitate excitation spreading, but at the same time couple electronic (spin) degrees of freedom with motional (phonon) states. With increasing spin-phonon coupling, the growth dynamics of a cluster of excited Rydberg atoms changes from ballistic spreading to Bloch-like oscillations and eventually to Anderson-like localization. We show that these effects are caused by quantum fluctuations in the phonon field: The dynamics of a Rydberg cluster can be mapped to a single particle in a semi-infinite lattice subject to phonon-induced energy shifts. The mean-field contribution of this energy shift leads to a linear potential gradient, resulting into Bloch-like oscillations. In addition, quantum fluctuations of phonons create a random local potential causing a transition from a regime of Bloch oscillations to localization. The spin-phonon coupling leads furthermore to highly correlated and non-classical phonon states in the form of squeezed states of the position of the Rydberg atoms. Depending on the form of the dipolar interaction potential, either in- or out-of-phase correlated oscillations of atoms emerge.

DOI
10.48550/arxiv.2504.19679

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We investigate the interplay between mechanical forces and the internal-state dynamics of Rydberg excitations in atom-tweezer arrays. Dipole interactions between Rydberg atoms facilitate excitation spreading, but at the same time couple electronic (spin) degrees of freedom with motional (phonon) states. With increasing spin-phonon coupling, the growth dynamics of a cluster of excited Rydberg atoms changes from ballistic spreading to Bloch-like oscillations and eventually to Anderson-like localization. We show that these effects are caused by quantum fluctuations in the phonon field: The dynamics of a Rydberg cluster can be mapped to a single particle in a semi-infinite lattice subject to phonon-induced energy shifts. The mean-field contribution of this energy shift leads to a linear potential gradient, resulting into Bloch-like oscillations. In addition, quantum fluctuations of phonons create a random local potential causing a transition from a regime of Bloch oscillations to localization. The spin-phonon coupling leads furthermore to highly correlated and non-classical phonon states in the form of squeezed states of the position of the Rydberg atoms. Depending on the form of the dipolar interaction potential, either in- or out-of-phase correlated oscillations of atoms emerge.
Atoms confined in optical tweezer arrays constitute a platform for the implementation of quantum computers and simulators. State-dependent operations are realized by exploiting electrostatic dipolar interactions that emerge, when two atoms are simultaneously excited to high-lying electronic states, so-called Rydberg states. These interactions also lead to state-dependent mechanical forces, which couple the electronic dynamics of the atoms to their vibrational motion. We explore these vibronic couplings within an artificial molecular system in which Rydberg states are excited under so-called facilitation conditions. This system, which is not necessarily self-bound, undergoes a structural transition between an equilateral triangle and an equal-weighted superposition of distorted triangular states (Jahn-Teller regime) exhibiting spin-phonon entanglement on a micrometer distance. This highlights the potential of Rydberg tweezer arrays for the study of molecular phenomena at exaggerated length scales.
We explore the relaxation dynamics of elementary spin clusters in a kinetically constrained spin system. Inspired by experiments with Rydberg lattice gases, we focus on the situation in which an excited spin leads to a "facilitated" excitation of a neighboring spin. We show that even weak interactions that extend beyond nearest neighbors can have a dramatic impact on the relaxation behavior: they generate a linear potential, which under certain conditions leads to the onset of Bloch oscillations of spin clusters. These hinder the expansion of a cluster and, more generally, the relaxation of many-body states toward equilibrium. This shows that nonergodic behavior in kinetically constrained systems may occur as a consequence of the interplay between reduced connectivity of many-body states and weak interparticle interactions. We furthermore show that the emergent Bloch oscillations identified here can be detected in experiment through measurements of the Rydberg atom density and discuss how spin-orbit coupling between internal and external degrees of freedom of spin clusters can be used to control their relaxation behavior.
Polarons, which arise from the self-trapping interaction between electrons and lattice distortions in a solid, have been known and extensively investigated for nearly a century. Nevertheless, the study of polarons continues to be an active and evolving field, with ongoing advancements in both fundamental understanding and practical applications. Here, we present a microscopic model that exhibits a diverse range of dynamic behavior, arising from the intricate interplay between two excitation-phonon coupling terms. The derivation of the model is based on an experimentally feasible Rydberg-dressed system with dipole-dipole interactions, making it a promising candidate for realization in a Rydberg atoms quantum simulator for excitation dynamics interacting with optical phonons. Remarkably, our analysis reveals a growing asymmetry in Bloch oscillations, leading to a macroscopic transport of nonspreading excitations under a constant force. Finally, we demonstrate the robustness of our findings against on-site random potential.
We investigate the dynamics of a one-dimensional spin system with facilitation constraint that can be studied using Rydberg atoms in arrays of optical tweezer traps. The elementary degrees of freedom of the system are domains of Rydberg excitations that expand ballistically through the lattice. Because of mechanical forces, Rydberg excited atoms are coupled to vibrations within their traps. At zero temperature and large trap depth, it is known that virtually excited lattice vibrations only renormalize the timescale of the ballistic propagation. However, when vibrational excitations are initially present-i.e., when the external motion of the atoms is prepared in an excited Fock state, coherent state or thermal state-resonant scattering between spin domain walls and phonons takes place. This coherent and deterministic process, which is free from disorder, leads to a reduction of the power-law exponent characterizing the expansion of spin domains. Furthermore, the spin domain dynamics is sensitive to the coherence properties of the atoms' vibrational state, such as the relative phase of coherently superimposed Fock states. Even for a translationally invariant initial state the latter manifests macroscopically in a phase-sensitive asymmetric expansion.
The rapid advancement of quantum science and technology has established Rydberg-atom arrays as a premier platform for exploring quantum many-body physics with exceptional precision and controllability. Traditionally, each atom is modeled as a spin degree of freedom with its spatial motion effectively frozen. This simplification has facilitated the discovery of a rich variety of novel equilibrium and nonequilibrium phases, including ZN{\mathbb{Z}}_{\text{N}}ZN​ symmetry-breaking orders and quantum scars. In this work, we investigate the consequences of incorporating atomic vibrations in optical tweezers, which give rise to spin-phonon coupling. For systems in thermal equilibrium, we find that this coupling leads to a new symmetry-breaking phase in the weak driving limit, as a result of induced three-spin interactions. Furthermore, we show that the violation of quantum thermalization in Z2{\mathbb{Z}}_{2}Z2​-ordered states is suppressed when spin-phonon coupling is introduced. Our results are readily testable in state-of-the-art Rydberg-atom array experiments.
Rydberg atoms in optical lattices and tweezers is now a well-established platform for simulating quantum spin systems. However, the role of the atoms' spatial wave function has not been examined in detail experimentally. Here, we show a strong spin-motion coupling emerging from the large variation of the interaction potential over the wave function spread. We observe its clear signature on the ultrafast many-body nanosecond-dynamics of atoms excited to a Rydberg S state, using picosecond pulses, from an unity-filling atomic Mott-insulator. We also propose an approach to tune arbitrarily the strength of the spin-motion coupling relative to the motional energy scale set by trapping potentials. Our work provides a new direction for exploring the dynamics of strongly correlated quantum systems by adding the motional degree of freedom to the Rydberg simulation toolbox.