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arXiv:2311.00064 · Physical Review Letters

Coherent Spin-Phonon Scattering in Facilitated Rydberg Lattices

Matteo Magoni, Chris Nill, Igor Lesanovsky

Published Mar 25, 2024• 9 citations
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Abstract

We investigate the dynamics of a one-dimensional spin system with facilitation constraint that can be studied using Rydberg atoms in arrays of optical tweezer traps. The elementary degrees of freedom of the system are domains of Rydberg excitations that expand ballistically through the lattice. Because of mechanical forces, Rydberg excited atoms are coupled to vibrations within their traps. At zero temperature and large trap depth, it is known that virtually excited lattice vibrations only renormalize the timescale of the ballistic propagation. However, when vibrational excitations are initially present-i.e., when the external motion of the atoms is prepared in an excited Fock state, coherent state or thermal state-resonant scattering between spin domain walls and phonons takes place. This coherent and deterministic process, which is free from disorder, leads to a reduction of the power-law exponent characterizing the expansion of spin domains. Furthermore, the spin domain dynamics is sensitive to the coherence properties of the atoms' vibrational state, such as the relative phase of coherently superimposed Fock states. Even for a translationally invariant initial state the latter manifests macroscopically in a phase-sensitive asymmetric expansion.

DOI
10.1103/physrevlett.132.133401

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We investigate the dynamics of a one-dimensional spin system with facilitation constraint that can be studied using Rydberg atoms in arrays of optical tweezer traps. The elementary degrees of freedom of the system are domains of Rydberg excitations that expand ballistically through the lattice. Because of mechanical forces, Rydberg excited atoms are coupled to vibrations within their traps. At zero temperature and large trap depth, it is known that virtually excited lattice vibrations only renormalize the timescale of the ballistic propagation. However, when vibrational excitations are initially present-i.e., when the external motion of the atoms is prepared in an excited Fock state, coherent state or thermal state-resonant scattering between spin domain walls and phonons takes place. This coherent and deterministic process, which is free from disorder, leads to a reduction of the power-law exponent characterizing the expansion of spin domains. Furthermore, the spin domain dynamics is sensitive to the coherence properties of the atoms' vibrational state, such as the relative phase of coherently superimposed Fock states. Even for a translationally invariant initial state the latter manifests macroscopically in a phase-sensitive asymmetric expansion.
We study the dynamics of a one-dimensional Rydberg lattice gas under facilitation (anti-blockade) conditions which implements a so-called kinetically constrained spin system. Here an atom can only be excited to a Rydberg state when one of its neighbors is already excited. Once two or more atoms are simultaneously excited mechanical forces emerge, which couple the internal electronic dynamics of this many-body system to external vibrational degrees of freedom in the lattice. This electron-phonon coupling results in a so-called phonon dressing of many-body states which in turn impacts on the facilitation dynamics. In our theoretical study we focus on a scenario in which all energy scales are sufficiently separated such that a perturbative treatment of the coupling between electronic and vibrational states is possible. This allows to analytically derive an effective Hamiltonian for the evolution of clusters of consecutive Rydberg excitations in the presence of phonon dressing. We analyze the spectrum of this Hamiltonian and show --- by employing Fano resonance theory --- that the interaction between Rydberg excitations and lattice vibrations leads to the emergence of slowly decaying bound states that inhibit fast relaxation of certain initial states.
We explore the dynamics of Rydberg excitations in an optical tweezer array under antiblockade (or facilitation) conditions. Because of the finite temperature the atomic positions are randomly spread, an effect that leads to quenched correlated disorder in the interatomic interaction strengths. This drastically affects the facilitation dynamics as we demonstrate experimentally on the elementary example of two atoms. To shed light on the role of disorder in a many-body setting we show that here the dynamics is governed by an Anderson-Fock model, i.e., an Anderson model formulated on a lattice with sites corresponding to many-body Fock states. We first consider a one-dimensional atom chain in a limit that is described by a one-dimensional Anderson-Fock model with disorder on every other site, featuring both localized and delocalized states. We then illustrate the effect of disorder experimentally in a situation in which the system maps on a two-dimensional Anderson-Fock model on a trimmed square lattice. We observe a clear suppression of excitation propagation, which we ascribe to the localization of the many-body wave functions in Hilbert space.
We investigate the interplay between mechanical forces and the internal-state dynamics of Rydberg excitations in atom-tweezer arrays. Dipole interactions between Rydberg atoms facilitate excitation spreading, but at the same time couple electronic (spin) degrees of freedom with motional (phonon) states. With increasing spin-phonon coupling, the growth dynamics of a cluster of excited Rydberg atoms changes from ballistic spreading to Bloch-like oscillations and eventually to Anderson-like localization. We show that these effects are caused by quantum fluctuations in the phonon field: The dynamics of a Rydberg cluster can be mapped to a single particle in a semi-infinite lattice subject to phonon-induced energy shifts. The mean-field contribution of this energy shift leads to a linear potential gradient, resulting into Bloch-like oscillations. In addition, quantum fluctuations of phonons create a random local potential causing a transition from a regime of Bloch oscillations to localization. The spin-phonon coupling leads furthermore to highly correlated and non-classical phonon states in the form of squeezed states of the position of the Rydberg atoms. Depending on the form of the dipolar interaction potential, either in- or out-of-phase correlated oscillations of atoms emerge.
Rydberg lattice under facilitation conditions can feature kinetic constraints, leading to ballistic and nonergodic behavior at different detuning intensities. Here, we demonstrate that a resonant driving field can achieve effects similar to those under facilitation conditions. We focus on the relaxation dynamics of spin clusters in a periodically driven Rydberg spin lattice. Through an effective Hamiltonian for the domain walls of the spin cluster, it is shown that when the driving frequency is resonant with the Rydberg interaction, the spin cluster exhibits ballistic expansion with half the spreading rate compared to the case of facilitation conditions. However, near the resonant point, the spin cluster displays confinement behavior of the Bloch-like oscillations. These results demonstrate the rich dynamic behaviors in the driven Rydberg spin lattices and may find applications in quantum state manipulation.
Quantum spin systems with kinetic constraints have become paradigmatic for exploring collective dynamical behavior in many-body systems. Here we discuss a facilitated spin system which is inspired by recent progress in the realization of Rydberg quantum simulators. This platform allows to control and investigate the interplay between facilitation dynamics and the coupling of spin degrees of freedom to lattice vibrations. Developing a minimal model, we show that this leads to the formation of polaronic quasiparticle excitations which are formed by many-body spin states dressed by phonons. We investigate in detail the properties of these quasiparticles, such as their dispersion relation, effective mass, and the quasiparticle weight. Rydberg lattice quantum simulators are particularly suited for studying this phonon-dressed kinetically constrained dynamics as their exaggerated length scales permit the site-resolved monitoring of spin and phonon degrees of freedom.
The rapid advancement of quantum science and technology has established Rydberg-atom arrays as a premier platform for exploring quantum many-body physics with exceptional precision and controllability. Traditionally, each atom is modeled as a spin degree of freedom with its spatial motion effectively frozen. This simplification has facilitated the discovery of a rich variety of novel equilibrium and nonequilibrium phases, including ZN{\mathbb{Z}}_{\text{N}}ZN​ symmetry-breaking orders and quantum scars. In this work, we investigate the consequences of incorporating atomic vibrations in optical tweezers, which give rise to spin-phonon coupling. For systems in thermal equilibrium, we find that this coupling leads to a new symmetry-breaking phase in the weak driving limit, as a result of induced three-spin interactions. Furthermore, we show that the violation of quantum thermalization in Z2{\mathbb{Z}}_{2}Z2​-ordered states is suppressed when spin-phonon coupling is introduced. Our results are readily testable in state-of-the-art Rydberg-atom array experiments.