We introduce Zernike polynomials as a novel degree of freedom for encoding quantum information in the spatial structure of photons. Building on their orthogonality and completeness over the unit disk, we develop a framework for generating, manipulating, and detecting photons in Zernike modes, and propose methods for realizing single-photon and two-photon Zernike wave packets. We demonstrate analytically that two-photon states generated via spontaneous parametric down-conversion exhibit mode entanglement in the Zernike basis, with correlations arising from selection rules enforced by Clebsch-Gordan coefficients. Our results open a new pathway for structured spatial entanglement, complementary to schemes based on Laguerre-Gaussian or Hermite-Gaussian modes, and suggest practical experimental implementations based on holographic modulation and optical Fourier techniques.
We introduce Zernike polynomials as a novel degree of freedom for encoding quantum information in the spatial structure of photons. Building on their orthogonality and completeness over the unit disk, we develop a framework for generating, manipulating, and detecting photons in Zernike modes, and propose methods for realizing single-photon and two-photon Zernike wave packets. We demonstrate analytically that two-photon states generated via spontaneous parametric down-conversion exhibit mode entanglement in the Zernike basis, with correlations arising from selection rules enforced by Clebsch-Gordan coefficients. Our results open a new pathway for structured spatial entanglement, complementary to schemes based on Laguerre-Gaussian or Hermite-Gaussian modes, and suggest practical experimental implementations based on holographic modulation and optical Fourier techniques.
In this thesis, I present experimental and theoretical work which assesses and develops a range of tools that are required for performing quantum information processing, particularly in photonic systems. I investigate the three degrees of freedom of a single photon—its polarisation, spatialmomentum and time-frequency distributions. For polarisation, I show that using wave plates to implement arbitrary, single-qubit rotations is more complicated than is commonly appreciated. In the spatial-momentum and time-frequency domains, I develop ways to perform tomographic analysis of quantum states, and I report the first demonstrations of these techniques. In the time-frequency domain, the tomography technique utilises entanglement in the photon polarisation as a resource to store and provide access to the time-frequency information. In my first two experiments, I use spontaneous parametric down-conversion to produce entanglement between pairs of single photons in all three degrees of freedom. I demonstrate the first characterisation of entanglement in spatial modes and the time-frequency domain, the first quantitative measurement of entangled qutrit states, and the highest quality entangled states yet measured in both polarisation and spatial modes. I also report the first realisation of complete hyperentanglement, and a full, black-box tomography of a 36-dimensional two-photon state—the largest system to be characterised in this way to date. In my final experiment, I model and implement a new architecture for a controlled-Z gate which is much simpler to align than previous implementations. This gate requires only one non-classical interference condition, the visibility of which is the main limitation to its performance. I show that the gate operates effectively as a means of both creating entanglement and discriminating between the four elements in a basis of maximally entangled, Bell-type states. Indeed, its observed performance as a Bell analyser would be sufficient to build a quantum state teleporter which would guarantee that the recipient would be left with a better copy of an unknown input state than any eavesdropper. In a series of numerical simulations, I investigate some of the practicalities that arise when using tomographic reconstruction techniques, including how to estimate errors, which measurements to make and what is actually the optimal reconstruction. In particular, I show that tomographies perform better when based on the results from over-complete sets of measurements. Finally, I discuss the important issue of how to compare two processes, particularly when trying to assess the quality of a measured process by comparing it to some expected ideal. Judging possible candidate measures against a set of experimentally and theoretically motivated
The experimental realization of multidimensional quantum states may lead to unexplored and interesting physics, as well as advanced quantum communication protocols. The orbital angular momentum of photons is a well suitable discrete degree of freedom for implementing high-dimensional quantum systems. The standard method to generate and manipulate such photon modes is to use bulk and fixed optics. Here the authors demonstrate the utilization of a spatial light modulator to manipulate the orbital angular momentum of entangled photons generated in spontaneous parametric downconversion. They show that their setup allows them to realize photonic entanglement of up to 21 dimensions, which in principle can be extended to even larger dimensions.
The two-photon state generated by spontaneous parametric down-conversion (SPDC) exhibit spatial entanglement embedded in the corresponding mode function. The control of the spatial characteristics of the generated two-photon state is an issue of paramount importance. For example, the spatial entanglement of the two down converted photons forms the basis of quantum imaging, and entanglement in orbital angular momentum has opened a new scenario for implementing multidimensional Hilbert spaces. We put forward several techniques to engineer the spatial structure of entangled two-photon states generated in SPDC. The first strategy we consider for spatial control of the quantum state makes use of the direct manipulation of the pump beam. This technique makes feasible to prepare arbitrary engineered entangled states in any d-dimensional Hilbert space. The second strategy is based on the proper preparation of the down-converting crystal itself, namely quantum state manipulation by quasi-phase-matching (QPM) engineering. We use properly designed transversely varying QPM gratings in nonlinear crystals.
Multi-particle entangled states are becoming more and more interesting for different applications in quantum information, such as quantum multi-particle teleportation, entangled based cryptography and quantum communication schemes based on multi-particle states, but also for fundamental reasons such as testing local realism by means of the Greenberger-Horne-Zeilinger states (GHZ) arguments . The advantage of multiparticle entanglement versus the most common two particle one lies in the fact that the greater the number of particles involved in the entangled state, the more clearly the quantum effects are exhibited. Our final goal is to exploit the multi-photon entangled states for quantum metrology. By the interaction of those states with nanostructures (mostly nanoholes, but in a future also nanospheres), we expect to reach sub-wavelength sensitivity phase measurements beating the Standard Quantum Limit as well as to detect plasmonic effects. In this thesis we present our work consisting on designing and building an experimental setup for the generation of states of 4-photon entangled in the transverse linear momentum. In the first part we explain some basics in the form of a technical introduction. We then adapt a general theoretical model to our particular case, explaining the physics of the process of generation of entangled states of photons. We proceed explaining the details of our setup, as well as the procedure of measurement. We then present the results of our tests in a "standard" 2-photon regime to show the correct functioning of the setup itself. Some more sophisticated measurements using structured light in the form of a first-order Hermite-Gaussian mode has been performed to generate entanglement in higher spatial modes are also presented. We conclude with theoretical and experimental details regarding the 4-photon experiments feasible with our setup. Our source is based on Spontaneous Parametric Down-Conversion (SPDC). In the last two decades it has been extensively studied for the generation of two-photon entangled states, since Kwiat et al. published in 1995 the new scheme based on polarization entangled photons. Most of the studies regarding entangled states involving more than two photons are indeed based on quantum correlations in the polarization or in the path of the down converted beams. The great advantage of entangling a spatial degree of freedom (as we do) is related to the dimensionality of the Hilbert space in which the state is defined. In the particular case of linear momentum, which is a continuous variable, we are dealing with infinite dimensions. Since in each dimension of the state one quanta of information can be encoded, the advantage of having multidimension entanglement for the field of quantum communication and computing is clear. The specs of our setup include a periodically-poled KTP crystals offering high conversion efficiency and cut for type-0 SPDC. The photons generated are well known to be inherently entangled in different degrees of freedom such as polarization, energy-time, linear momentum, and orbital angular momentum. Since each single SPDC event generates one photon pair, in order to reach four photon we entangle two consecutive SPDC events per each state. Furthermore, it is possible to manipulate (to enhance) the dimensionality of the entanglement by properly tailoring the pump spatial profile. The key point for the generation of four-photon entangled states is that, under some conditions, two consecutive pairs generated via SPDC cannot be described as two independent pairs but necessarily as a four-photon state showing genuine entanglement. This can happen when using a pulsed laser to generate the entangled photons; in particular, in the regime in which the coherence time of the down-converted photons τc is (much) longer than the temporal length of the pumping pulse Δt. In this condition the emission of a second pair is stimulated by the presence of the first one. That effect can be ultimately seen as a constructive multi-particle interference effect, the deep origin of which has to be sought in the boson statistic of photons.
Photons with complicated spatial mode structures can be applied for different quantum information tasks. Here, we show the entanglement of photons with complex singularity patterns called Hermite-Laguerre-Gaussian (HLG) modes. Measuring one photon of the entangled pairs by HLG mode basis to define its singularity pattern, we can steer the singularity structure of its partner, while the initial singularity structure of the photons is undefined. We also calculate the HLG specific quantum-correlation function. It can be used to extend the quantum key distribution protocols and to tune experiments dealing with high-order transverse modes. In addition we discuss orbital angular momentum properties of the HLG modes and summarize some features of the singularity pattern of the HLG modes with varying angle parameter.
We present the novel embodiment of a photonic qubit that makes use of one continuous spatial degree of freedom of a single photon and relies on the parity of the photon's transverse spatial distribution. Using optical spontaneous parametric down-conversion to produce photon pairs, we demonstrate the controlled generation of entangled-photon states in this new space. Specifically, two Bell states, and a continuum of their superpositions, are generated by simple manipulation of a classical parameter, the optical-pump spatial parity, and not by manipulation of the entangled photons themselves. An interferometric device, isomorphic in action to a polarizing beam splitter, projects the spatial-parity states onto an even-odd basis. This new physical realization of photonic qubits could be used as a foundation for future experiments in quantum information processing.