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arXiv:2504.12677 · Physical Review A

Excitation transfer and many-body dark states in waveguide quantum electrodynamics

Wei Chen, Guin-Dar Lin, H. H. Jen

Published Sep 18, 2025• 2 citations
arXivHTMLPDF

Abstract

In one-dimensional waveguide quantum electrodynamics systems, quantum emitters interact through infinite-range, dispersive, and dissipative dipole-dipole interactions mediated by guided photonic modes. These long-range periodic interactions give rise to rich many-body physics absent in free space. In this work, we construct a set of symmetrized multiexcitation dark states and derive analytic expressions for their time-evolution projections. This framework captures the essential dynamics of excitation transport and storage while significantly reducing computational complexity compared to full master equation simulations. Our analysis reveals a fundamental bound on energy redistribution governed by the structure of dark states and collective dissipation and discovers that optimal excitation transfer between emitter ensembles converges toward an initial pumped fraction of ${N}_{\text{p}}/N\ensuremath{\approx}0.55$ for large system sizes. We further examine the robustness of this mechanism under realistic imperfections, including positional disorder, nonradiative decay, and dephasing. These results highlight the role of many-body dark states in enabling efficient and controllable energy transfer, offering new insights into dissipative many-body dynamics in integrated quantum platforms.

DOI
10.1103/tgbv-x4qz

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In one-dimensional waveguide quantum electrodynamics systems, quantum emitters interact through infinite-range, dispersive, and dissipative dipole-dipole interactions mediated by guided photonic modes. These long-range periodic interactions give rise to rich many-body physics absent in free space. In this work, we construct a set of symmetrized multiexcitation dark states and derive analytic expressions for their time-evolution projections. This framework captures the essential dynamics of excitation transport and storage while significantly reducing computational complexity compared to full master equation simulations. Our analysis reveals a fundamental bound on energy redistribution governed by the structure of dark states and collective dissipation and discovers that optimal excitation transfer between emitter ensembles converges toward an initial pumped fraction of Np/N\ensuremath≈0.55{N}_{\text{p}}/N\ensuremath{\approx}0.55Np​/N\ensuremath≈0.55 for large system sizes. We further examine the robustness of this mechanism under realistic imperfections, including positional disorder, nonradiative decay, and dephasing. These results highlight the role of many-body dark states in enabling efficient and controllable energy transfer, offering new insights into dissipative many-body dynamics in integrated quantum platforms.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
Waveguide quantum electrodynamics (QED) studies the interaction between quantum emitters and guided photons in one dimension. When the waveguide hosts interacting photons, it becomes a platform to explore many-body quantum optics. However, the influence of photonic correlations on emitter dynamics remains poorly understood. In this work, we study the collective decay and coherent interactions of quantum emitters coupled to a one-dimensional Bose-Hubbard waveguide, an array of coupled photonic modes with repulsive on-site interactions that supports superfluid and Mott insulating phases. We show that photon-photon interactions alone can trigger a superradiant burst, independent of emitter spacing and transition frequency. In the off-resonant regime, emitters exhibit two distinct types of mediated interactions. Delocalized superfluid excitations yield persistent, long-range couplings, challenging the noninteracting paradigm, where long-range (dissipative) couplings occur in band, whereas short-range and coherent interactions occur in a bandgap. In the Mott limit, quasiparticles generate short-range interactions mediated by doublons and holons. Our work bridges many-body physics and waveguide QED, revealing how photonic many-body states shape emitter dynamics.
In contrast to free space, in waveguides the dispersive and dissipative dipole–dipole interactions among quantum emitters exhibit a periodic behavior over remarkably long distances. We propose a novel setup, to our knowledge, exploiting this long-range periodicity in order to create highly excited subradiant states and facilitate fast controlled collective energy transport among far-apart ensembles coupled to a waveguide. For sufficiently large ensembles, collective superradiant emission into the fiber modes dominates over its free space counterpart. We show that, for a large number of emitters, a fast transverse coherent pulse can create almost perfect subradiant states with up to 50% excitation. On the other hand, for a coherent excitation of one sub-ensemble above an overall excitation fraction of 50% we find a nearly lossless and fast energy transfer to the ground state sub-ensemble. This transport can be enhanced or suppressed by controlling the positions of the ensembles relative to each other, while it can also be realized with a random position distribution. In the optimally enhanced case this fast transfer appears as superradiant emission with subsequent superabsorption, yet, without a superradiant decay after the absorption. The highly excited subradiant states, as well as the superradiant excitation transfer, appear as suitable building blocks in applications such as active atomic clocks, quantum batteries, quantum information protocols, and quantum metrology procedures such as fiber-based Ramsey schemes.
At the quantum many-body level, atom-light interfaces generally remain challenging to solve for or understand in a nonperturbative fashion. Here we consider a waveguide quantum electrodynamics model, where two-level atoms interact with and via propagating photons in a one-dimensional waveguide, and specifically investigate the interplay of atomic position disorder, multiple scattering of light, quantum nonlinear interactions, and dissipation. We develop qualitative arguments and present numerical evidence that such a system exhibits a many-body localized (MBL) phase, provided that atoms are less than half excited. Interestingly, while MBL is originally formulated with respect to closed systems, this system is intrinsically open. However, as dissipation originates from transport of energy to the system boundaries and the subsequent radiative loss, the lack of transport in the MBL phase makes the waveguide QED system look essentially closed and makes applicable the notions of MBL. Conversely, we show that if the system is initially in a delocalized phase due to a large excitation density, then rapid initial dissipation can leave the system unable to efficiently transport energy at later times, resulting in a dynamical transition to an MBL phase. These phenomena can be feasibly realized in state-of-the-art experimental setups.
Driven-dissipative quantum emitters provide a powerful platform for controllable excitation storage and release, with promising applications in quantum batteries and quantum storage. Yet, transient excitation transfer in collective many-body systems is often obscured by the intricate interplay among coherent driving, dissipation, and correlation dynamics. Here, we uncover a scalable excitation-storage mechanism in two emitter ensembles coupled to a semi-infinite waveguide. A coherently driven ensemble acts as an effective excitation reservoir, while a second ensemble positioned near a dissipative node serves as a subradiant storage medium. Surprisingly, when the driven ensemble largely exceeds the storage ensemble in size, the transfer dynamics enters a nearly correlation-free regime, allowing the driven ensemble to behave effectively as a classical excitation source. This reveals a simple scaling law for optimal excitation transfer, under which the storage ensemble approaches near-complete population inversion as the driven ensemble size increases. Building on this mechanism, we propose a three-stage storage-and-release protocol enabling fast excitation storage and controllable photon emission. Our results demonstrate how coherent and dissipative collective interactions can be jointly harnessed for quantum energy storage and programmable nonequilibrium dynamics in waveguide QED platforms.
Waveguide quantum electrodynamics studies photon-mediated interactions of quantum emitters in a one-dimensional radiation channel. Although signatures of such interactions have been observed previously in a variety of physical systems, observation of coherent cooperative dynamics has been obscured by radiative decay of atoms into the waveguide. Employing transmon qubits as artificial atoms coupled to a microwave coplanar waveguide, here we observe dynamical oscillations in an open system where a designated probe qubit interacts with an entangled dark state of an array of qubits which effectively traps radiation as an atomic cavity. The qubit-cavity system is shown to achieve a large cooperativity of C=172 due to collective enhancement of photon-mediated interactions, entering the strong coupling regime. The quantum coherence of the dark state cavity is also explored through its nonlinear response at the single-excitation level. With realistic refinements, this system is suitable for studying the many-body dynamics of large (N>10) quantum spin chains, synthesizing highly non-classical radiation fields on demand, and implementing universal quantum logic operations with high fidelity on information encoded within decoherence-free subspaces.