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arXiv:2405.07833 · Optica Quantum

Subradiance and superradiant long-range excitation transport among quantum emitter ensembles in a waveguide

Martin Fasser, Laurin Ostermann, Helmut Ritsch, Christoph Hotter

Published Sep 23, 2024• 7 citations
arXivHTMLPDF

Abstract

In contrast to free space, in waveguides the dispersive and dissipative dipole–dipole interactions among quantum emitters exhibit a periodic behavior over remarkably long distances. We propose a novel setup, to our knowledge, exploiting this long-range periodicity in order to create highly excited subradiant states and facilitate fast controlled collective energy transport among far-apart ensembles coupled to a waveguide. For sufficiently large ensembles, collective superradiant emission into the fiber modes dominates over its free space counterpart. We show that, for a large number of emitters, a fast transverse coherent pulse can create almost perfect subradiant states with up to 50% excitation. On the other hand, for a coherent excitation of one sub-ensemble above an overall excitation fraction of 50% we find a nearly lossless and fast energy transfer to the ground state sub-ensemble. This transport can be enhanced or suppressed by controlling the positions of the ensembles relative to each other, while it can also be realized with a random position distribution. In the optimally enhanced case this fast transfer appears as superradiant emission with subsequent superabsorption, yet, without a superradiant decay after the absorption. The highly excited subradiant states, as well as the superradiant excitation transfer, appear as suitable building blocks in applications such as active atomic clocks, quantum batteries, quantum information protocols, and quantum metrology procedures such as fiber-based Ramsey schemes.

DOI
10.1364/opticaq.531434

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In contrast to free space, in waveguides the dispersive and dissipative dipole–dipole interactions among quantum emitters exhibit a periodic behavior over remarkably long distances. We propose a novel setup, to our knowledge, exploiting this long-range periodicity in order to create highly excited subradiant states and facilitate fast controlled collective energy transport among far-apart ensembles coupled to a waveguide. For sufficiently large ensembles, collective superradiant emission into the fiber modes dominates over its free space counterpart. We show that, for a large number of emitters, a fast transverse coherent pulse can create almost perfect subradiant states with up to 50% excitation. On the other hand, for a coherent excitation of one sub-ensemble above an overall excitation fraction of 50% we find a nearly lossless and fast energy transfer to the ground state sub-ensemble. This transport can be enhanced or suppressed by controlling the positions of the ensembles relative to each other, while it can also be realized with a random position distribution. In the optimally enhanced case this fast transfer appears as superradiant emission with subsequent superabsorption, yet, without a superradiant decay after the absorption. The highly excited subradiant states, as well as the superradiant excitation transfer, appear as suitable building blocks in applications such as active atomic clocks, quantum batteries, quantum information protocols, and quantum metrology procedures such as fiber-based Ramsey schemes.
The transversely confined propagating modes of an optical fiber mediate virtually infinite range energy exchanges among atoms placed within their field, which adds to the inherent free space dipole–dipole coupling. Typically, the single atom free space decay rate largely surpasses the emission rate into the guided fiber modes. However, scaling up the atom number as well as the system size amounts to entering a collective emission regime, where fiber-induced superradiant spontaneous emission dominates over free space decay. We numerically study this super- and subradiant decay of highly excited atomic states for one or several transverse fiber modes as present in hollow core fibers. As particular excitation scenarios we compare the decay of a totally inverted state to the case of π /2 pulses applied transversely or along the fiber axis as in standard Ramsey or Rabi interferometry. While a mean field approach fails to correctly describe the initiation of superradiance, a second-order approximation accounting for pairwise atom–atom quantum correlations generally proves sufficient to reliably describe superradiance of ensembles from two to a few hundred particles. In contrast, a full account of subradiance requires the inclusion of all higher order quantum correlations. Considering multiple guided modes introduces a natural effective cut-off for the interaction range emerging from the dephasing of different fiber contributions.
Driven-dissipative quantum emitters provide a powerful platform for controllable excitation storage and release, with promising applications in quantum batteries and quantum storage. Yet, transient excitation transfer in collective many-body systems is often obscured by the intricate interplay among coherent driving, dissipation, and correlation dynamics. Here, we uncover a scalable excitation-storage mechanism in two emitter ensembles coupled to a semi-infinite waveguide. A coherently driven ensemble acts as an effective excitation reservoir, while a second ensemble positioned near a dissipative node serves as a subradiant storage medium. Surprisingly, when the driven ensemble largely exceeds the storage ensemble in size, the transfer dynamics enters a nearly correlation-free regime, allowing the driven ensemble to behave effectively as a classical excitation source. This reveals a simple scaling law for optimal excitation transfer, under which the storage ensemble approaches near-complete population inversion as the driven ensemble size increases. Building on this mechanism, we propose a three-stage storage-and-release protocol enabling fast excitation storage and controllable photon emission. Our results demonstrate how coherent and dissipative collective interactions can be jointly harnessed for quantum energy storage and programmable nonequilibrium dynamics in waveguide QED platforms.
In one-dimensional waveguide quantum electrodynamics systems, quantum emitters interact through infinite-range, dispersive, and dissipative dipole-dipole interactions mediated by guided photonic modes. These long-range periodic interactions give rise to rich many-body physics absent in free space. In this work, we construct a set of symmetrized multiexcitation dark states and derive analytic expressions for their time-evolution projections. This framework captures the essential dynamics of excitation transport and storage while significantly reducing computational complexity compared to full master equation simulations. Our analysis reveals a fundamental bound on energy redistribution governed by the structure of dark states and collective dissipation and discovers that optimal excitation transfer between emitter ensembles converges toward an initial pumped fraction of ${N}_{\text{p}}/N\ensuremath{\approx}0.55$ for large system sizes. We further examine the robustness of this mechanism under realistic imperfections, including positional disorder, nonradiative decay, and dephasing. These results highlight the role of many-body dark states in enabling efficient and controllable energy transfer, offering new insights into dissipative many-body dynamics in integrated quantum platforms.
The radiative properties of quantum emitters are profoundly influenced by their electromagnetic environment. When coupled to a waveguide terminated at one end by a mirror, distant emitters interact strongly via virtual photon exchange, leading to collective superradiant and subradiant states with enhanced or suppressed decay rates. We demonstrate that applying optimal frequency shifts to each emitter enables the formation of perfect single-excitation dark states (i.e. states with zero decay rate) and near-perfect multi-excitation dark states in small ensembles. These collective states can be deterministically prepared with high fidelity using classical driving fields or few-photon pulses propagating along the waveguide. These results, readily implementable in superconducting qubit platforms, open new avenues for quantum information storage, networking and control of light.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
A ring of dipole-coupled quantum emitters positioned at subwavelength distances possesses only a few radiant but many subradiant collective excitations with lifetimes growing exponentially with the atom number. These exhibit a three-dimensionally confined spatial radiation field pattern and form nanoscale high-QQQ optical resonators. Tailoring size, orientation, and distance between two rings allows for increasing the ratio of coherent ring-to-ring energy transfer versus free-space emission by orders of magnitude. In particular, the more dark and delocalized over several sites are excitons, the higher is their fidelity for transport to a second ring.