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arXiv:2504.06221

Quantum-stabilized states in magnetic dipolar quantum gases

Lauriane Chomaz

Published Apr 8, 2025• 0 citations
arXivHTMLPDF

Abstract

A decade ago, a universal stabilization mechanism driven by quantum fluctuations was discovered in ultracold Bose gases of highly magnetic atoms. This mechanism prevents these systems from collapsing and instead allows exotic states of matter to arise, including ultradilute quantum droplets, crystallized quantum states, and specifically supersolids. We review the experimental and theoretical progress in understanding these quantum-stabilized states, their emergence, and intriguing properties.

DOI
10.48550/arxiv.2504.06221

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A decade ago, a universal stabilization mechanism driven by quantum fluctuations was discovered in ultracold Bose gases of highly magnetic atoms. This mechanism prevents these systems from collapsing and instead allows exotic states of matter to arise, including ultradilute quantum droplets, crystallized quantum states, and specifically supersolids. We review the experimental and theoretical progress in understanding these quantum-stabilized states, their emergence, and intriguing properties.
Ultracold Bose gases of highly magnetic atoms exhibit unique interaction properties that lead to striking many-body behaviors, both at and beyond the mean field. A decade ago, a universal stabilization mechanism driven by quantum fluctuations was discovered in these gases. This mechanism prevents the systems from collapsing and instead allows exotic states of matter to arise, including ultradilute quantum droplets, crystallized quantum states, and especially supersolids. After introducing key features of dipolar quantum Bose gases—including their interactions, ground states, and excitations in a mean-field framework, as well as the onset of quantum-fluctuation stabilization—we review the progress made in understanding the emergence and intriguing properties of these quantum stabilized states. Both theory and experiments are discussed.
Quantum fluctuations can stabilize Bose-Einstein condensates (BEC) against the mean-field collapse. Stabilization of the condensate has been observed in quantum degenerate Bose-Bose mixtures and dipolar BECs. The fine-tuning of the interatomic interactions can lead to the emergence of two new states of matter: liquid-like self-bound quantum droplets and supersolid crystals formed from these droplets. We review the properties of these exotic states of matter and summarize the experimental progress made using dipolar quantum gases and Bose-Bose mixtures. We conclude with an outline of important open questions that could be addressed in the future.
Since the achievement of quantum degeneracy in gases of chromium atoms in 2004, the experimental investigation of ultracold gases made of highly magnetic atoms has blossomed. The field has yielded the observation of many unprecedented phenomena, in particular those in which long-range and anisotropic dipole-dipole interactions (DDIs) play a crucial role. In this review, we aim to present the aspects of the magnetic quantum-gas platform that make it unique for exploring ultracold and quantum physics as well as to give a thorough overview of experimental achievements. Highly magnetic atoms distinguish themselves by the fact that their electronic ground-state configuration possesses a large electronic total angular momentum. This results in a large magnetic moment and a rich electronic transition spectrum. Such transitions are useful for cooling, trapping, and manipulating these atoms. The complex atomic structure and large dipolar moments of these atoms also lead to a dense spectrum of resonances in their two-body scattering behaviour. These resonances can be used to control the interatomic interactions and, in particular, the relative importance of contact over dipolar interactions. These features provide exquisite control knobs for exploring the few- and many-body physics of dipolar quantum gases. The study of dipolar effects in magnetic quantum gases has covered various few-body phenomena that are based on elastic and inelastic anisotropic scattering. Various many-body effects have also been demonstrated. These affect both the shape, stability, dynamics, and excitations of fully polarised repulsive Bose or Fermi gases. Beyond the mean-field instability, strong dipolar interactions competing with slightly weaker contact interactions between magnetic bosons yield new quantum-stabilised states, among which are self-bound droplets, droplet assemblies, and supersolids. Dipolar interactions also deeply affect the physics of atomic gases with an internal degree of freedom as these interactions intrinsically couple spin and atomic motion. Finally, long-range dipolar interactions can stabilise strongly correlated excited states of 1D gases and also impact the physics of lattice-confined systems, both at the spin-polarised level (Hubbard models with off-site interactions) and at the spinful level (XYZ models). In the present manuscript, we aim to provide an extensive overview of the various related experimental achievements up to the present.
These lecture notes contain an introduction to quantum simulation of bosonic systems in the continuum, focusing on weakly interacting Bose-Bose mixtures with competing mean-field interactions. When the values of such interactions are fine-tuned to almost completely cancel the mean-field energy, quantum fluctuations become apparent and dominate the behavior of the system, stabilizing an ultradilute quantum liquid phase. An analogous situation appears in single-component dipolar quantum gases. We review the mechanism that gives rise to this exotic quantum liquid, which can form droplets that are self-bound in the absence of any external confinement, and discuss their properties and dynamics in both the mixture and the dipolar cases. In dipolar gases, arrays of dipolar droplets stabilized by quantum fluctuations can establish global phase coherence and form supersolids. In bosonic mixtures, supersolidity can emerge already at the mean-field level through spin-orbit coupling. We discuss the properties of such spin-orbit-coupled supersolids, comparing them to their dipolar counterparts. Specifically, we focus on their periodic density modulation, phase coherence, and peculiar excitation spectrum, which hosts both superfluid and crystal excitations. Finally, we conclude by discussing open research directions in the areas of quantum liquid droplets and spin-orbit-coupled supersolids, in particular at the interface of the two research topics.
Gases of doubly dipolar particles, with both magnetic and electric dipole moments, offer intriguing novel possibilities. We show that the interplay between doubly dipolar interactions, quantum stabilization, and external confinement results in a rich ground-state physics of supersolids and incoherent droplet arrays in doubly dipolar condensates. Our study reveals novel possibilities for engineering quantum droplets and droplet supersolids, including supersolid-supersolid transitions and the realization of supersolid arrays of pancake droplets.
Dipolar quantum gases, encompassing atoms and molecules with significant dipole moments, exhibit unique long-range and anisotropic dipole-dipole interactions (DDI), distinguishing them from systems dominated by short-range contact interactions. This review explores their behavior across dimensions, focusing on magnetic atoms in quasi-2D in comparison to 3D. In 3D, strong DDI leads to phenomena like anisotropic superfluidity, quantum droplets stabilized by Lee-Huang-Yang corrections, and supersolid states with density modulations. In 2D, we discuss a new scenario where DDI induces angle-dependent Berezinskii-Kosterlitz-Thouless transitions and potential supersolidity, as suggested by recent experimental realizations of strongly dipolar systems in quasi-2D geometries. We identify key challenges for future experimental and theoretical work on strongly dipolar 2D systems. The review concludes by highlighting how these unique 2D dipolar systems could advance fundamental research as well as simulate novel physical phenomena.