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arXiv:2504.01885 · Physical Review Letters

Observing Spatial Charge and Spin Correlations in a Strongly Interacting Fermi Gas

Cyprien Daix, Maxime Dixmerias, Yuan-Yao He, Joris Verstraten, Tim de Jongh, Bruno Peaudecerf, Shiwei Zhang, Tarik Yefsah

Published Jan 26, 2026• 6 citations
arXivHTMLPDF

Abstract

In this Letter, we explore two-dimensional attractive Fermi gases at the microscopic level by probing spatial charge and spin correlations in situ. Using atom-resolved continuum quantum gas microscopy, we directly observe fermion pairing and study the evolution of two- and three-point correlation functions as interspin attraction is increased. The precision of our measurement allows us to reveal nonlocal anticorrelations in the pair correlation function, fundamentally forbidden by the mean-field result based on BCS theory but whose existence we confirm in exact auxiliary-field quantum Monte Carlo calculations. We demonstrate that the BCS prediction is critically deficient not only in the superfluid crossover regime but also deep in the weakly attractive side. Guided by our measurements, we find a remarkable relation between two- and three-point correlations that establishes the dominant role of pair correlations. Finally, leveraging local single-pair losses, we independently characterize the short-range behavior of pair correlations, via the measurement of Tan's contact, and find excellent agreement with numerical predictions. Our measurements provide a novel microscopic view into strongly correlated two-dimensional Fermi gases in the continuum.

DOI
10.1103/2t2k-3ftx

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In this Letter, we explore two-dimensional attractive Fermi gases at the microscopic level by probing spatial charge and spin correlations in situ. Using atom-resolved continuum quantum gas microscopy, we directly observe fermion pairing and study the evolution of two- and three-point correlation functions as interspin attraction is increased. The precision of our measurement allows us to reveal nonlocal anticorrelations in the pair correlation function, fundamentally forbidden by the mean-field result based on BCS theory but whose existence we confirm in exact auxiliary-field quantum Monte Carlo calculations. We demonstrate that the BCS prediction is critically deficient not only in the superfluid crossover regime but also deep in the weakly attractive side. Guided by our measurements, we find a remarkable relation between two- and three-point correlations that establishes the dominant role of pair correlations. Finally, leveraging local single-pair losses, we independently characterize the short-range behavior of pair correlations, via the measurement of Tan's contact, and find excellent agreement with numerical predictions. Our measurements provide a novel microscopic view into strongly correlated two-dimensional Fermi gases in the continuum.
We demonstrate atom-resolved detection of itinerant bosonic ^{23}Na and fermionic ^{6}Li quantum gases, enabling the direct in situ measurement of interparticle correlations. In contrast to prior work on lattice-trapped gases, here we realize microscopy of quantum gases in the continuum. We reveal Bose-Einstein condensation with single-atom resolution, measure the enhancement of two-particle g^{(2)} correlations of thermal bosons, and observe the suppression of g^{(2)} for fermions; the Fermi or exchange hole. For strongly interacting Fermi gases confined to two dimensions, we directly observe nonlocal fermion pairs in the BEC-BCS crossover. We obtain the pair size and the short-range contact directly from the pair correlations. In situ thermometry is enabled via the fluctuation-dissipation theorem. Our technique opens the door to the atom-resolved study of strongly correlated quantum gases of bosons, fermions, and their mixtures.
This thesis presents a series of experimental studies that leverage atom-resolved imaging to probe fundamental properties of ultracold Fermi gases in continuous space. We demonstrate the viability of this continuum microscopy by reliably observing the expansion of a Gaussian wave packet and the Fermi hole of a two-dimensional ideal Fermi gas, measuring its second- and third-order correlation functions. Building upon this foundation, we introduce a novel local thermometer based on the relationship between fluctuations and correlations. This method enables accurate global and local temperature measurement without requiring trap calibration. Further investigations reveal sub-extensive fluctuations absent from the well-known fluctuation-dissipation theorem. We describe how these fluctuations are linked to entanglement entropy and observe a violation of the area law. Following this we connect the spatial organization of non-interacting fermions to random matrix theory via the Fredholm determinant. Measurements of the counting statistics and nearest-neighbor spacing are compared with numerical predictions, showing excellent agreement. Finally, we explore the physics of two-dimensional interacting fermions in the BEC-BCS crossover. Our measurements of two- and three-point correlation functions show significant discrepancies with mean-field BCS theory, but are corroborated by exact quantum Monte Carlo calculations. We also perform a precise measurement of Tan's contact. As a whole, this work provides a unique and unprecedented microscopic perspective on the fundamentals of Fermi gases, and establishes quantum gas microscopy as a powerful and versatile tool for exploring quantum gases in the continuum.
The two-species Fermi gas with attractive short-range interactions in two spatial dimensions provides a paradigmatic system for the understanding of strongly correlated Fermi superfluids in two dimensions. It is known to exhibit a BEC to BCS crossover as a function of ln(k_{F}a), where a is the scattering length, and to undergo a Berezinskii-Kosterlitz-Thouless superfluid transition below a critical temperature T_{c}. However, the extent of a pseudogap regime in the strongly correlated regime of ln(k_{F}a)∼1, in which pairing correlations persist above T_{c}, remains largely unexplored with controlled theoretical methods. Here, we use finite-temperature auxiliary-field quantum Monte Carlo methods on discrete lattices in the canonical ensemble formalism to calculate thermodynamical observables in the strongly correlated regime. We extrapolate to continuous time and the continuum limit to eliminate systematic errors and present results for particle numbers ranging from N=42 to N=162. We estimate T_{c} by a finite-size scaling analysis, and observe clear pseudogap signatures above T_{c} and below a temperature T^{*} in both the spin susceptibility and free-energy gap. We also present results for the contact, a fundamental thermodynamic property of quantum many-body systems with short-range interactions.
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The Hubbard model of attractively interacting fermions provides a paradigmatic setting for fermion pairing. It features a crossover between Bose-Einstein condensation of tightly bound pairs and Bardeen-Cooper-Schrieffer superfluidity of long-range Cooper pairs, and a "pseudo-gap" region where pairs form above the superfluid critical temperature. We directly observe the nonlocal nature of fermion pairing in a Hubbard lattice gas, using spin- and density-resolved imaging of [Formula: see text]1000 fermionic potassium-40 atoms under a bilayer microscope. Complete fermion pairing is revealed by the vanishing of global spin fluctuations with increasing attraction. In the strongly correlated regime, the fermion pair size is found to be on the order of the average interparticle spacing. Our study informs theories of pseudo-gap behavior in strongly correlated fermion systems.
This work studies zero-temperature Fermi gases with short-ranged and attractive interactions with focus on the dimensionality aspects by confining the system from three to two dimensions. Interacting Fermi gases are superfluids characterized as being strongly correlated if the scattering length is much larger than the other scales present. In the many-body context, this category of systems requires a careful treatment since mean-field approaches are not expected to hold under the conditions which define the strong pairing. For this reason, we employ quantum Monte Carlo methods to study the dimensionality effects in two-component Fermi gases in the Bardeen-Cooper-Schrieffer to Bose-Einstein condensate (BCS-BEC) crossover. To be able to investigate such aspects, we consider a three-dimensional gas with periodic boundary conditions in the xy plane and a confining potential in the z direction capable of reducing the dimensionality of the system, which defines a dimensional BCS-BEC crossover. We calculate the equation of state as the energy per particle as a function of the dimensionality and as a function of the interaction parameter, which are characterized by the oscillator length in the z direction and the scattering length respectively. The greater confinement in the system lowers the interparticle distances, which increases the effects of the attractive interactions between antiparallel-spin fermions.We also calculate the density profile in the z direction over the crossover for different confinements and different interaction parameters to quantify their influence on the spatial distribution of the particles. This study connects the perspectives between theoretical and experimental works in low-dimensional ultracold Fermi gases by utilizing an approach that is similar to what it is realized in modern experiments.