In this thesis, I present the experimental realisation of the two-dimensional Hubbard model with ultracold fermionic Potassium-40 atoms in optical lattices. By tuning the dimensionality, kinetic and interaction in the optical lattices, we perform an analogue quantum simulation to explore the phase diagram of the Hubbard model. \n \nThe first key result is the experimental observation of particle-hole symmetry, namely a phase mapping between repulsive and attractive interactions. We compare a density-ordered, Mott-insulating phase with repulsive interaction to a spin-ordered, preformed pair phase and found excellent agreement with the theoretical prediction. The precise control and excellent detection capability of our quantum gas apparatus allow us to validate the particle-hole symmetry, and utilise it to explore quantum phases with a novel approach. \n \nNext, we investigate the spin-ordering on the repulsive side. By implementing a novel scheme based on coherent manipulation of spin correlations, we probe the anti-ferromagnetic ordering in the low-temperature phase diagram. The momentum-resolved spin correlations permit the reconstruction of spatial correlators without site-resolved imaging fidelity. \n \nFinally, we probe the attractive side of the phase diagram with a focus in pairing phenomenon, in which we draw a close analogy with BCS-BEC crossovers present in high-temperature superconducting cuprates and trapped ultracold Fermi gases. From the pair correlation function derived from thermodynamics observables, we observe the competition between the effective Pauli repulsion in fermionic systems and the on-site attraction we implemented.
In this thesis, I present the experimental realisation of the two-dimensional Hubbard model with ultracold fermionic Potassium-40 atoms in optical lattices. By tuning the dimensionality, kinetic and interaction in the optical lattices, we perform an analogue quantum simulation to explore the phase diagram of the Hubbard model. \n \nThe first key result is the experimental observation of particle-hole symmetry, namely a phase mapping between repulsive and attractive interactions. We compare a density-ordered, Mott-insulating phase with repulsive interaction to a spin-ordered, preformed pair phase and found excellent agreement with the theoretical prediction. The precise control and excellent detection capability of our quantum gas apparatus allow us to validate the particle-hole symmetry, and utilise it to explore quantum phases with a novel approach. \n \nNext, we investigate the spin-ordering on the repulsive side. By implementing a novel scheme based on coherent manipulation of spin correlations, we probe the anti-ferromagnetic ordering in the low-temperature phase diagram. The momentum-resolved spin correlations permit the reconstruction of spatial correlators without site-resolved imaging fidelity. \n \nFinally, we probe the attractive side of the phase diagram with a focus in pairing phenomenon, in which we draw a close analogy with BCS-BEC crossovers present in high-temperature superconducting cuprates and trapped ultracold Fermi gases. From the pair correlation function derived from thermodynamics observables, we observe the competition between the effective Pauli repulsion in fermionic systems and the on-site attraction we implemented.
Among the most compelling targets for quantum simulation are strongly correlated phases and electronic-structure problems, where interactions organize electrons into collective states and produce intricate low-temperature phase diagrams. Cuprate superconductors are a canonical example: at low doping, superconductivity emerges from a metallic regime that exhibits a pseudogap above the critical temperature. Ultracold atoms in optical lattices provide a well-controlled, tunable setting to probe the microscopic mechanisms behind this behavior and, in fermion-native architectures, to implement electronic structure dynamics directly. This thesis demonstrates both large scale systematic analog quantum simulations in the most interesting regime of doped antiferromagnets and elementary high-fidelity gates as the basis for a digital or hybrid fermionic quantum processors in an optical lattice. Working with ultracold Lithium-6 in a two–dimensional optical superlattice, we first map the parameter space of the Fermi–Hubbard model over a wide range of temperatures and dopings. More than 40000 single-site spin- and density-resolved snapshots, spanning over a dense grid of doping levels and temperatures in a numerically challenging parameter space, reveal antiferromagnetic correlations extending across the system size and into the pseudogap regime. Temperatures down to T/t=0.2 are realized, determined by benchmarking the data to state-of-the-art numerical methods. By evaluating spin–charge correlators up to fifth order, we experimentally uncover a universal scaling behavior across the pseudogap crossover, governed by a single, doping-dependent temperature scale. These findings provide the first microscopic evidence of universal scaling in multi-point correlators and establish stringent benchmarks for future theoretical developments. On the same apparatus, we demonstrate that the controlled motion of fermions in double wells enables high-fidelity entanglement. Double-well potentials are used to engineer coherent pair-tunnelling and spin-exchange interactions that act as native SWAP^α operations. We demonstrate the collisional gate fidelities up to 99.8% and Bell-state lifetimes exceeding ten seconds, limited mainly by residual inhomogeneities in the optical potential. A composite pulse sequence isolates the pair-exchange channel, realizing the elementary building block required for fermionic quantum-chemistry algorithms. With the addition of site-selective addressing, our results mark a key step towards a fully digital, scalable fermionic quantum computer based on the controlled motion and entanglement of fermionic neutral atoms. The work establishes a hybrid analog-digital architecture: analog evolution under the Hubbard Hamiltonian yields thermodynamic states whose magnetic properties match and extend theoretical benchmarks, while digital collisional gates provide building blocks for error-corrected quantum computation and complex state preparation.
Ultracold atomic gases provide a fantastic platform to implement quantum simulators and investigate a variety of models initially introduced in condensed matter physics or other areas. One of the most promising applications of quantum simulation is the study of strongly correlated Fermi gases, for which exact theoretical results are not always possible with state-of-the-art approaches. Here, we review recent progress of the quantum simulation of the emblematic Fermi–Hubbard model with ultracold atoms. After introducing the Fermi–Hubbard model in the context of condensed matter, its implementation in ultracold atom systems, and its phase diagram, we review landmark experimental achievements, from the early observation of the onset of quantum degeneracy and superfluidity to the demonstration of the Mott insulator regime and the emergence of long-range anti-ferromagnetic order. We conclude by discussing future challenges, including the possible observation of high- T c superconductivity, transport properties, and the interplay of strong correlations and disorder or topology.
Analog quantum simulation provides a unique toolkit to investigate quantum many-body problems of whose solutions may be incredibly challenging. In particular, using ultracold fermionic atoms in optical lattices it realizes the Fermi Hubbard model, which is a fundamental model in condensed matter physics exhibiting properties relevant to many intriguing strongly-correlated systems. However, most quantum simulators of the Hubbard model have so far restricted to the square geometries. In addition, access to low temperatures where the exotic quantum phases are predicted to develop has still remained elusive. In this thesis, we engineer a novel optical lattice with dynamically tunable geometries and significantly reduced technical noises. We extend for the first time the study of quantum magnetism into the exotic phases in a Fermi Hubbard system with tunable geometric frustration. As we continuously tune our system from a square to a triangular lattice geometry, we observe a transition from a Néel antiferromagnet to a 120-degree spin spiral state. We then study, again for the first time, how doping affects a frustrated quantum magnet. To our surprise, we found an emergent ferromagnetic state with strong particle doping, which is absent on the hole-doped side and is in stark contrast with the particle-hole symmetric doping dependence in a square lattice. To shed light on the role of itinerant dopants in the emergence of these new magnetic properties, we furthermore leverage the unique single-particle resolution capabilities of our platform to probe higher-order density and spin correlations. These measurements hint at a new type of magnetism induced by kinetic frustration, which manifests as local antiferromagnetic correlations around hole dopants and and ferromagnetic correlations around particle dopants. Unlike magnetism induced by exchange or superexchange interactions, the energy associated with this mechanism is the kinetic energy, closely related to the famous rigorous results by Nagaoka. Furthermore, the dynamical tunability of the lattice allows adibatic engineering of quantum states in optical lattices. We discuss the preliminery efforts to prepare strongly-correlated states with significantly reduced temperatures, which may pave the way towards low temperature states in the Hubbard model.
Strongly-correlated electron systems generate some of the richest phenomena and most challenging theoretical problems studied in physics. One approach to understanding these systems is with ultracold fermionic atoms in optical lattices, which can provide a level of control and ways of observing strongly-correlated fermionic systems that are not accessible with conventional materials. This thesis describes the development of an experimental technique where a quantum gas of fermionic 6Li atoms is prepared in a two-dimensional optical lattice and each atom can be frozen in place and imaged with single-site resolution. Combining a vacuum-compatible large numerical aperture microscope with Raman sideband cooling enables site-resolved fluorescence imaging with high fidelity. We observe several phases of the Hubbard model, including band and Mott insulators. The observed in-situ occupation distributions of atoms in the lattice are compared to theory with unprecedented detail and are used to determine the thermodynamic properties of the system. By combining site-resolved imaging with a spin-removal technique, we observe antiferromagnetic correlations in the Hubbard model with single-site resolution. We observe, for the first time in cold atom systems, beyond-nearest-neighbor magnetic correlations, which provide a direct measurement of the correlation length. We also present detailed measurements of the formation of correlations during lattice loading.
Ultracold atoms in optical lattices provide an extremely clean and controllable setting to explore quantum many-body phases of matter. Here we give a brief review of the strong-correlation physics that has been realized using such ultracold atoms in optical lattices ranging from the realization of Hubbard models to studies of quantum magnetism and the detection of single atoms with lattice site resolution. All this has opened up fundamentally new opportunities for the investigation of quantum many-body systems. Introduction Over the past years, ultracold atoms in optical lattices have emerged as versatile new systems to explore the physics of quantum many-body systems. On the one hand, they can be helpful in gaining a better understanding of known phases of matter and their dynamical behavior; on the other hand, they allow one to realize completely novel quantum systems that have not been studied before in nature [1, 2, 3]. Commonly, the approach of exploring quantum many-body systems in such a way is referred to as “quantum simulations.” Examples of some of the first strongly interacting many-body phases that have been realized both in lattices and in the continuum include the quantum phase transition from a superfluid to a Mott insulator [4, 5, 6], fermionic Mott insulators [7, 8], the achievement of a Tonks- Girardeau gas [9, 10], and the realization of the Bose-Einsten condensate (BEC)– Bardeen-Cooper-Schrieffer (BCS) crossover (see also Chapter 12) in Fermi gas mixture [11] using Feshbach resonances [12]. In almost all of these experiments, detection was limited to time-of-flight imaging or more refined derived techniques that mainly characterized the momentum distribution of the quantum gas [2]. For several years, researchers in the field have therefore aspired to employ in situ single-particle detection methods for the analysis of ultracold quantum gases. Only recently has it become possible to implement such imaging techniques, marking a milestone for the characterization and manipulation of ultracold quantum gases [13, 14, 15, 16, 17]. In our discussion, we will focus on one of the most successful of these techniques based on high-resolution fluorescence imaging. Despite being a rather new technique, such quantum gas microscopy has already proven to be an enabling technology for probing and manipulating quantum many-body systems. For the first time, controllable and strongly interacting many-body systems, as realized with ultracold atoms, could be observed on a local scale [17, 16].