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arXiv:2503.08629 · Physical Review A

Optical probes of coherence in two-dimensional Bose gases of polaritons

Joseph Jachinowski, Hassan Alnatah, David W. Snoke, P. B. Littlewood

Published Jun 15, 2026• 0 citations
arXivHTMLPDF

Abstract

Due to their photonic components, exciton-polariton systems provide a convenient platform to study the coherence properties of weakly-interacting Bose gases. In particular, optical interferometry enables the measurement of the first-order coherence function which provides information about the intrinsic correlations of the system. In this paper, we derive a universal curve for the coherent fraction of a noninteracting, equilibrium, homogeneous, two-dimensional Bose gas, with density expressed in units of the observation area, and compare to recent experimental results. Although there is a sharp transition from normal to superfluid phases in the thermodynamic limit, the coherent fraction of the gas varies continuously across this transition due to the finite system size. We find that the theory agrees nearly perfectly with the experimental data in the low-density limit with no free parameters other than the effective temperature, highly constrained by the measurements. At higher density, the experiments are consistent with standard weakly-interacting Bose gas theory. By having a theory that treats both the optical diffraction and Bose coherence, we can clearly see the effect of the quantum statistics on the coherence.

DOI
10.1103/77n7-c7mg

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Due to their photonic components, exciton-polariton systems provide a convenient platform to study the coherence properties of weakly-interacting Bose gases. In particular, optical interferometry enables the measurement of the first-order coherence function which provides information about the intrinsic correlations of the system. In this paper, we derive a universal curve for the coherent fraction of a noninteracting, equilibrium, homogeneous, two-dimensional Bose gas, with density expressed in units of the observation area, and compare to recent experimental results. Although there is a sharp transition from normal to superfluid phases in the thermodynamic limit, the coherent fraction of the gas varies continuously across this transition due to the finite system size. We find that the theory agrees nearly perfectly with the experimental data in the low-density limit with no free parameters other than the effective temperature, highly constrained by the measurements. At higher density, the experiments are consistent with standard weakly-interacting Bose gas theory. By having a theory that treats both the optical diffraction and Bose coherence, we can clearly see the effect of the quantum statistics on the coherence.
Abstract The emergence of spatial coherence in a confined two-dimensional Bose gas of exciton polaritons with tuneable interactions offers a unique opportunity to explore the role of interactions in a phase transition in a driven-dissipative quantum system, where both the phase transition and thermalisation are mediated by interactions. We investigate, experimentally and numerically, the spatial coherence and steady-state properties of the gas over a wide range of interaction strengths by varying the photonic/excitonic fraction of the polaritons and their density. We find that the first order spatial correlation function exhibits algebraic decay consistent with the Berezinskii-Kosterlitz-Thouless (BKT) phase transition. The exponent of the algebraic decay is inversely proportional to the coherent fraction of polaritons, in analogy to superfluid fraction of equilibrium quantum gases above the BKT transition, but with a different proportionality constant. Our work paves the way for future investigations of the phenomenon of phase transitions and superfluidity in a driven-dissipative setting.
We study the quasi-two-dimensional Bose gas in harmonic traps at temperatures above the Kosterlitz-Thouless transition, where the gas is in the normal phase. We show that mean-field theory takes into account the dominant interaction effects for experimentally relevant trap geometries. Comparing with quantum Monte Carlo calculations, we quantify the onset of the fluctuation regime, where correlations beyond mean-field become important. Although the density profile depends on the microscopic parameters of the system, we show that the correlation density (the difference between the exact and the mean-field density) is accurately described by a universal expression, obtained from classical-field calculations of the homogeneous strictly two-dimensional gas. Deviations from universality, due to the finite value of the interaction or to the trap geometry, are shown to be small for current experiments. We further study coherence and pair correlations on a microscopic scale. Finite-size effects in the off-diagonal density matrix allow us to characterize the crossover from Kosterlitz-Thouless to Bose-Einstein behavior for small particle numbers. Bose-Einstein condensation occurs below a characteristic number of particles which rapidly diverges with vanishing interactions.
The study of second-order phase transitions is a broad research theme that provides fundamental insights into the physical nature of complex systems. A central aspect deals with the concept of universal behavior. Universality governs, for example, the diverging correlated fluctuations of an order parameter, characterized by a macroscopic correlation length ξ, as well as the divergence of other thermodynamic quantities near the critical point. Extracting the critical exponents associated with these diverging quantities shows that quite different physical systems can exhibit identical scaling behavior, placing them into common universality classes. Bose-Einstein condensation of an ideal (i.e., non-interacting) gas of bosons is a second-order phase transition, and thus provides a valuable platform to investigate universal critical behavior in the quantum gas regime, driven purely by quantum statistics rather than inter-particle interactions. While historically studied in ultracold atomic and molecular gases, Bose-Einstein condensation can now be realized in a two-dimensional photonic gas at room temperature using dye-filled microcavities. The microcavity imposes a low-energy cutoff, providing a non-vanishing ground state and an effective mass for the intracavity photons, which thermalize via repeated absorption and emission processes with the dye reservoir rather than inter-particle interactions. Consequently, this platform establishes an almost perfectly ideal, two-dimensional quantum gas of light. In combination with versatile trapping techniques, it provides a highly tunable platform to explore the thermodynamics of quantum gases. This thesis presents a quantitative study of spatial correlations in a uniformly trapped two-dimensional photon gas. The uniform confinement is achieved by a custom mirror-structuring technique, resulting in box-like trapping potentials. The temporal and spatial coherence properties of the gas are validated in both the thermal and condensed regimes using an interferometric measurement technique. Because the applicability of scanning interferometry limits measurements of critical scaling behavior, an alternative method is introduced to extract the first-order spatial coherence directly from the far-field angular distribution of the cavity emission in a single experimental shot. This technique enables the extraction of the spatial correlation length ξ and a precise evaluation of its scaling behavior in the vicinity of the critical point Nc. The measurements presented here demonstrate, for the first time, the determination of a critical exponent in the (ideal) Bose gas universality class. The obtained critical exponent of ν = 0.52 ± 0.04 for the two-dimensional ideal Bose gas is consistent with theoretical expectations. Crucially, this critical exponent is found to be robust and independent of the system size within experimental uncertainties, demonstrating the universality of the scaling behavior. Finally, the limits of this universal behavior are explored by demonstrating the breakdown of critical scaling when the thermalizing coupling between the photons and dye molecules in the cavity is reduced, driving the photon gas out of thermal equilibrium.
In current experiments with cold quantum gases in periodic potentials, interference fringe contrast is typically the easiest signal in which to look for effects of nontrivial many-body dynamics. In order better to calibrate such measurements, we analyze the background effect of thermal decoherence as it occurs in the absence of dynamical interparticle interactions. We study the effect of optical lattice potentials, as experimentally applied, on the condensed fraction of a noninteracting Bose gas in local thermal equilibrium at finite temperatures. We show that the experimentally observed decrease of the condensate fraction in the presence of the lattice can be attributed, up to a threshold lattice height, purely to ideal-gas thermodynamics; conversely, we confirm that sharper decreases in first-order coherence observed in stronger lattices are indeed attributable to many-body physics. Our results also suggest that the fringe visibility ``kinks'' observed in Gerbier et al., Phys. Rev. Lett. 95, 050404 (2005) may be explained in terms of the competition between increasing lattice strength and increasing mean gas density, as the Gaussian profile of the red-detuned lattice lasers also increases the effective strength of the harmonic trap.
Phase transitions between different states of matter can profoundly modify the order in physical systems, with the emergence of ferromagnetic or topological order constituting important examples. Correlations allow the quantification of the degree of order and the classification of different phases. Here we report measurements of first-order spatial correlations in a harmonically trapped two-dimensional photon gas below, at and above the critical particle number for Bose–Einstein condensation, using interferometric measurements of the emission of a dye-filled optical microcavity. For the uncondensed gas, the transverse coherence decays on a length scale determined by the thermal de Broglie wavelength of the photons, which shows the expected scaling with temperature. At the onset of Bose–Einstein condensation, true long-range order emerges, and we observe quantum statistical effects as the thermal wave packets overlap. The excellent agreement with equilibrium Bose gas theory prompts microcavity photons as promising candidates for studies of critical scaling and universality in optical quantum gases.
Phase transitions between different states of matter can profoundly modify the order in physical systems, with the emergence of ferromagnetic or topological order constituting important examples. Correlations allow the quantification of the degree of order and the classification of different phases. Here we report measurements of first-order spatial correlations in a harmonically trapped two-dimensional photon gas below, at and above the critical particle number for Bose-Einstein condensation, using interferometric measurements of the emission of a dye-filled optical microcavity. For the uncondensed gas, the transverse coherence decays on a length scale determined by the thermal de Broglie wavelength of the photons, which shows the expected scaling with temperature. At the onset of Bose-Einstein condensation, true long-range order emerges, and we observe quantum statistical effects as the thermal wave packets overlap. The excellent agreement with equilibrium Bose gas theory prompts microcavity photons as promising candidates for studies of critical scaling and universality in optical quantum gases.Phase transitions in quantum matter are related to correlation effects and they can change the ordering of material. Here the authors measure the first-order spatial correlation and the de Broglie wavelength for both thermal and condensed form of a photonic Bose gas in a dye-filled optical microcavity.