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Observation of Critical Scaling in a Nearly Ideal Bose Gas

Leon Espert Miranda

Published Aug 12, 2026• 0 citations
OpenAlex

Abstract

The study of second-order phase transitions is a broad research theme that provides fundamental insights into the physical nature of complex systems. A central aspect deals with the concept of universal behavior. Universality governs, for example, the diverging correlated fluctuations of an order parameter, characterized by a macroscopic correlation length ξ, as well as the divergence of other thermodynamic quantities near the critical point. Extracting the critical exponents associated with these diverging quantities shows that quite different physical systems can exhibit identical scaling behavior, placing them into common universality classes. Bose-Einstein condensation of an ideal (i.e., non-interacting) gas of bosons is a second-order phase transition, and thus provides a valuable platform to investigate universal critical behavior in the quantum gas regime, driven purely by quantum statistics rather than inter-particle interactions. While historically studied in ultracold atomic and molecular gases, Bose-Einstein condensation can now be realized in a two-dimensional photonic gas at room temperature using dye-filled microcavities. The microcavity imposes a low-energy cutoff, providing a non-vanishing ground state and an effective mass for the intracavity photons, which thermalize via repeated absorption and emission processes with the dye reservoir rather than inter-particle interactions. Consequently, this platform establishes an almost perfectly ideal, two-dimensional quantum gas of light. In combination with versatile trapping techniques, it provides a highly tunable platform to explore the thermodynamics of quantum gases. This thesis presents a quantitative study of spatial correlations in a uniformly trapped two-dimensional photon gas. The uniform confinement is achieved by a custom mirror-structuring technique, resulting in box-like trapping potentials. The temporal and spatial coherence properties of the gas are validated in both the thermal and condensed regimes using an interferometric measurement technique. Because the applicability of scanning interferometry limits measurements of critical scaling behavior, an alternative method is introduced to extract the first-order spatial coherence directly from the far-field angular distribution of the cavity emission in a single experimental shot. This technique enables the extraction of the spatial correlation length ξ and a precise evaluation of its scaling behavior in the vicinity of the critical point Nc. The measurements presented here demonstrate, for the first time, the determination of a critical exponent in the (ideal) Bose gas universality class. The obtained critical exponent of ν = 0.52 ± 0.04 for the two-dimensional ideal Bose gas is consistent with theoretical expectations. Crucially, this critical exponent is found to be robust and independent of the system size within experimental uncertainties, demonstrating the universality of the scaling behavior. Finally, the limits of this universal behavior are explored by demonstrating the breakdown of critical scaling when the thermalizing coupling between the photons and dye molecules in the cavity is reduced, driving the photon gas out of thermal equilibrium.

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The study of second-order phase transitions is a broad research theme that provides fundamental insights into the physical nature of complex systems. A central aspect deals with the concept of universal behavior. Universality governs, for example, the diverging correlated fluctuations of an order parameter, characterized by a macroscopic correlation length ξ, as well as the divergence of other thermodynamic quantities near the critical point. Extracting the critical exponents associated with these diverging quantities shows that quite different physical systems can exhibit identical scaling behavior, placing them into common universality classes. Bose-Einstein condensation of an ideal (i.e., non-interacting) gas of bosons is a second-order phase transition, and thus provides a valuable platform to investigate universal critical behavior in the quantum gas regime, driven purely by quantum statistics rather than inter-particle interactions. While historically studied in ultracold atomic and molecular gases, Bose-Einstein condensation can now be realized in a two-dimensional photonic gas at room temperature using dye-filled microcavities. The microcavity imposes a low-energy cutoff, providing a non-vanishing ground state and an effective mass for the intracavity photons, which thermalize via repeated absorption and emission processes with the dye reservoir rather than inter-particle interactions. Consequently, this platform establishes an almost perfectly ideal, two-dimensional quantum gas of light. In combination with versatile trapping techniques, it provides a highly tunable platform to explore the thermodynamics of quantum gases. This thesis presents a quantitative study of spatial correlations in a uniformly trapped two-dimensional photon gas. The uniform confinement is achieved by a custom mirror-structuring technique, resulting in box-like trapping potentials. The temporal and spatial coherence properties of the gas are validated in both the thermal and condensed regimes using an interferometric measurement technique. Because the applicability of scanning interferometry limits measurements of critical scaling behavior, an alternative method is introduced to extract the first-order spatial coherence directly from the far-field angular distribution of the cavity emission in a single experimental shot. This technique enables the extraction of the spatial correlation length ξ and a precise evaluation of its scaling behavior in the vicinity of the critical point Nc. The measurements presented here demonstrate, for the first time, the determination of a critical exponent in the (ideal) Bose gas universality class. The obtained critical exponent of ν = 0.52 ± 0.04 for the two-dimensional ideal Bose gas is consistent with theoretical expectations. Crucially, this critical exponent is found to be robust and independent of the system size within experimental uncertainties, demonstrating the universality of the scaling behavior. Finally, the limits of this universal behavior are explored by demonstrating the breakdown of critical scaling when the thermalizing coupling between the photons and dye molecules in the cavity is reduced, driving the photon gas out of thermal equilibrium.
Critical exponents characterize the divergent scaling of thermodynamic quantities near phase transitions and allow for the classification of physical systems into universality classes. While quantum gases thermalizing by interparticle interactions fall into the XY model universality class, the ideal Bose gas has been predicted to form a distinct universality class whose signatures have not yet been revealed experimentally. Here, we report the observation of critical scaling in a two-dimensional trapped quantum gas of essentially noninteracting photons, which thermalize by radiative contact to a reservoir of molecules inside a microcavity. By measuring the spatial correlations near the condensation transition, we determine the critical exponent for the correlation length to be ν=0.52(4)ν= 0.52(4)ν=0.52(4). Our results constitute a first experimental test of the long-standing scaling predictions for the Bose gas universality class.
Phase transitions between different states of matter can profoundly modify the order in physical systems, with the emergence of ferromagnetic or topological order constituting important examples. Correlations allow the quantification of the degree of order and the classification of different phases. Here we report measurements of first-order spatial correlations in a harmonically trapped two-dimensional photon gas below, at and above the critical particle number for Bose-Einstein condensation, using interferometric measurements of the emission of a dye-filled optical microcavity. For the uncondensed gas, the transverse coherence decays on a length scale determined by the thermal de Broglie wavelength of the photons, which shows the expected scaling with temperature. At the onset of Bose-Einstein condensation, true long-range order emerges, and we observe quantum statistical effects as the thermal wave packets overlap. The excellent agreement with equilibrium Bose gas theory prompts microcavity photons as promising candidates for studies of critical scaling and universality in optical quantum gases.Phase transitions in quantum matter are related to correlation effects and they can change the ordering of material. Here the authors measure the first-order spatial correlation and the de Broglie wavelength for both thermal and condensed form of a photonic Bose gas in a dye-filled optical microcavity.
Phase transitions between different states of matter can profoundly modify the order in physical systems, with the emergence of ferromagnetic or topological order constituting important examples. Correlations allow the quantification of the degree of order and the classification of different phases. Here we report measurements of first-order spatial correlations in a harmonically trapped two-dimensional photon gas below, at and above the critical particle number for Bose–Einstein condensation, using interferometric measurements of the emission of a dye-filled optical microcavity. For the uncondensed gas, the transverse coherence decays on a length scale determined by the thermal de Broglie wavelength of the photons, which shows the expected scaling with temperature. At the onset of Bose–Einstein condensation, true long-range order emerges, and we observe quantum statistical effects as the thermal wave packets overlap. The excellent agreement with equilibrium Bose gas theory prompts microcavity photons as promising candidates for studies of critical scaling and universality in optical quantum gases.
Bose-Einstein condensation (BEC) is the transition to a macroscopic occupation of the ground state of a system of bosonic particles. In 1995 the first experimental realization of BEC was achieved by condensing a dilute atomic gas [1,2]. It was long thought only massive particles could undergo BEC. However, in 2010 it was shown that photon BEC was achieved in an optical dye-filled microcavity [3]. In 2015, we became the second group to successfully repeat these experiments.\n\nBEC is a phase transition and thus it occurs at thermal equilibrium. To achieve a thermal photon gas the cavity is filled with a fluorescent dye solution. The dye molecules thermalize the photons by means of repeated absorption-emission cycles. We optically pump the cavity. With the pump we determine the number of photons absorbed by the dye, consequently defining a nonvanishing chemical potential. This ensures a conserved photon number. The photons are trapped by the harmonic potential induced by the concave cavity mirrors. Due to the cutoff energy determined by the cavity length, the trapped photons have a dispersion similar to that of a massive particle in a quantum harmonic oscillator. The cavity length is tuned such that the free spectral range is larger than the bandwidth of the dye. Therefore, only one longitudinal mode fits inside the cavity, making the photon gas effectively two-dimensional. We end up with a thermalized two-dimensional photon gas that has the eigenenergies of a quantum harmonic oscillator. The Bose-Einstein distribution function predicts a critical photon number. Pumping the thermal photon gas beyond this critical number will lead to photon BEC.\n\nWe measure the spectral- and spatial distributions of our two-dimensional photon gas. In both distributions we observe photon BEC. Results show the characteristics of a phase transition: the appearance of a sharp peak on top of the thermal cloud that coincides with a converging chemical potential to zero. Both the spectral- and spatial distribution are in agreement with the theoretical distribution of photons with an effective mass in a quantum harmonic oscillator. Expansion of the condensate has been measured. This could indicate nonlinear optical effects such as thermal lensing or repulsive photon-photon interactions.
Ideal Bose-Einstein condensation (BEC) remains a paradigmatic example of a continuous phase transition and a cornerstone for understanding quantum degenerate bosonic matter. We demonstrate that critical behavior of the ideal Bose gas near the BEC phase transition falls into three distinct classes, determined exclusively by the low-energy scaling of the density of states. Depending on its scaling exponent, which is controlled by dimensionality and confinement, the transition displays either the usual algebraic divergences of thermodynamic susceptibilities, divergent behavior with marginal logarithmic corrections, or a more subtle form of criticality, where only the correlation length diverges. Our work provides a unified framework for criticality in noninteracting bosonic systems. This classification applies broadly to atomic, photonic, polaritonic, and magnonic condensates, where dimensionality, confinement, and spectral engineering can strongly reshape the density of states.
The condensation of photons in a dye-filled optical microcavity represents a landmark achievement in macroscopic quantum phenomena, bridging quantum optics and statistical mechanics. While ordinary Bose-Einstein condensation (BEC) of massive particles is governed by well-established critical exponents, photon condensation occurs in an open, dissipative system where thermalization is mediated through repeated absorption and re-emission cycles by dye molecules. In this paper, we systematically investigate whether photon condensation exhibits independent critical exponents. We define the scaling of the condensed photon density as n_gamma proportional to |T - T_c|^(beta_gamma) and examine whether the critical exponent beta_gamma deviates significantly from the classical values associated with standard three-dimensional or trapped two-dimensional Bose systems. Through a rigorous theoretical formulation based on master equations, grand canonical statistical mechanics, and renormalization group techniques, we explore the universal properties of this light-matter phase transition. Establishing a distinct set of critical exponents for photon condensation could lay the foundational stone for a new universal class of non-equilibrium quantum phase transitions, offering profound implications for fundamental physics and advanced quantum technologies.