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arXiv:2503.07354 · PRX Quantum

Quasiparticle Poisoning of Superconducting Qubits with Active Gamma Irradiation

C.P. Larson, E. Yelton, Kenneth Dodge, Koichi Okubo, J. Batarekh, Vito Iaia, Noah Kurinsky, B. L. T. Plourde

Published Jul 14, 2025• 9 citations
arXivHTMLPDF

Abstract

When a high-energy particle, such as a γ ray or muon, impacts the substrate of a superconducting qubit chip, large numbers of electron-hole pairs and phonons are created. The ensuing dynamics of the electrons and holes changes the local offset-charge environment for qubits near the impact site. The phonons that are produced have energy above the superconducting gap in the films that compose the qubits, leading to quasiparticle excitations above the superconducting ground state when the phonons impinge on the qubit electrodes. An elevated density of quasiparticles degrades qubit coherence, leading to errors in qubit arrays. Because these pair-breaking phonons spread throughout much of the chip, the errors can be correlated across a large portion of the array, posing a significant challenge for quantum error correction. In order to study the dynamics of γ -ray impacts on superconducting qubit arrays, we use a γ -ray source outside the dilution refrigerator to controllably irradiate our devices. By using charge-sensitive transmon qubits, we can measure both the offset-charge shifts and quasiparticle poisoning due to the γ irradiation at different doses. We study correlations between offset-charge shifts and quasiparticle poisoning for different qubits in the array and compare these with numerical modeling of charge and phonon dynamics following a γ -ray impact. We thus characterize the poisoning footprint of these impacts and quantify the performance of structures for mitigating phonon-mediated quasiparticle poisoning.

DOI
10.1103/2lyd-8swv

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When a high-energy particle, such as a γ ray or muon, impacts the substrate of a superconducting qubit chip, large numbers of electron-hole pairs and phonons are created. The ensuing dynamics of the electrons and holes changes the local offset-charge environment for qubits near the impact site. The phonons that are produced have energy above the superconducting gap in the films that compose the qubits, leading to quasiparticle excitations above the superconducting ground state when the phonons impinge on the qubit electrodes. An elevated density of quasiparticles degrades qubit coherence, leading to errors in qubit arrays. Because these pair-breaking phonons spread throughout much of the chip, the errors can be correlated across a large portion of the array, posing a significant challenge for quantum error correction. In order to study the dynamics of γ -ray impacts on superconducting qubit arrays, we use a γ -ray source outside the dilution refrigerator to controllably irradiate our devices. By using charge-sensitive transmon qubits, we can measure both the offset-charge shifts and quasiparticle poisoning due to the γ irradiation at different doses. We study correlations between offset-charge shifts and quasiparticle poisoning for different qubits in the array and compare these with numerical modeling of charge and phonon dynamics following a γ -ray impact. We thus characterize the poisoning footprint of these impacts and quantify the performance of structures for mitigating phonon-mediated quasiparticle poisoning.
Background radiation can deposit large amounts of energy in the substrate of superconducting qubit arrays. Such events create bursts of energetic phonons that cause transient degradations of coherence, leading to errors. Correlated errors across multiple qubits are problematic for quantum error correction. The authors develop here a numerical model to describe the results of controlled phonon injection experiments. A dense array of qubits is modeled to explore the effectiveness of down-converting metal films for mitigating the effects of gamma ray impacts.
Errors that are correlated across a qubit array pose an obstacle to quantum error correction. We observe elevated correlated poisoning rates in superconducting qubit arrays at the start of a cooldown followed by power-law reductions in time, while the rate of offset charge shifts remains constant, evidence of nonionizing sources of pair-breaking phonon bursts. We also investigate different sample packages, with some exhibiting elevated poisoning due to mechanical impacts from the cryocooler. Possible sources include relaxation of built-up stress in device thin films, substrates, or packaging.
Quasiparticle poisoning following particle impacts poses a significant challenge to the development of fault-tolerant superconducting quantum computers, as a sudden excess of quasiparticles can simultaneously degrade the coherence of multiple qubits across large device arrays. In this work, we present a statistical analysis that models the time evolution of radiation-induced qubit energy relaxation through quasiparticle density dynamics. This study provides insight into quasiparticle loss processes by distinguishing between recombination and trapping decay channels and assessing their respective impact on qubit performance. We precisely measure quasiparticle recombination in multiple transmon qubits and uncover an unexpected dependence of qubit relaxation dynamics on deposited energy. By linking correlated relaxation events across qubits to ballistic phonon propagation, we introduce a statistical localization approach to extract the energy deposited in the substrate, which is in good agreement with Monte Carlo simulation. This work establishes the quantitative framework for using an arbitrary subset of superconducting transmon qubits in a QPU as energy-resolving witness particle detectors.
Quantum error correction can preserve quantum information in the presence of local errors, but correlated errors are fatal. For superconducting qubits, high-energy particle impacts from background radioactivity produce energetic phonons that travel throughout the substrate and create excitations above the superconducting ground state, known as quasiparticles, which can poison all qubits on the chip. We use normal metal reservoirs on the chip back side to downconvert phonons to low energies where they can no longer poison qubits. We introduce a pump-probe scheme involving controlled injection of pair-breaking phonons into the qubit chips. We examine quasiparticle poisoning on chips with and without back-side metallization and demonstrate a reduction in the flux of pair-breaking phonons by over a factor of 20. We use a Ramsey interferometer scheme to simultaneously monitor quasiparticle parity on three qubits for each chip and observe a two-order of magnitude reduction in correlated poisoning due to background radiation.
Superconducting qubits based on Josephson junctions have emerged as a leading hardware platform in the quest to realize large-scale quantum computers. However, qubit decoherence remains a major hurdle on the path toward fault-tolerant quantum computing. In particular, excess quasiparticle (QP) excitations constitute a significant source of dissipation in superconducting quantum devices. The empirically observed QP density in these systems is orders of magnitude larger than that predicted by Bardeen-Cooper-Schrieffer (BCS) theory. Moreover, QP poisoning due to high-energy particle impacts can cause correlated errors that simultaneously affect multiple qubits, thereby impeding quantum error correction. Although QP-induced decoherence has been extensively studied in widely implemented transmon qubits, its impact on fluxonium qubits, a leading alternative architecture, remains far less explored. In this thesis, we investigate energy relaxation in fluxonium qubits induced by controlled QP poisoning using an on-chip Josephson injector junction that generates Cooper-pair-breaking phonons and photons. We separately measure the relaxation and excitation rates, instead of the conventional energy relaxation time. For specific injection parameters, we observe an apparent reversal of the rates, with the excitation rate exceeding the relaxation rate. We further measure the rates as a function of external flux to disentangle the effects of QP tunneling across the small junction and the junction array superinductor. Across all measured samples, differing in qubit spectra and injection conditions, we infer roughly an order of magnitude higher QP density at the small junction than in the array junctions. Our findings advance the understanding of QP-induced decoherence in fluxonium qubits and provide insight for reconciling discrepancies in reported bounds on QP densities, potentially enabling the development of QP mitigation strategies tailored to fluxonium qubits.
Impacts from high-energy particles cause correlated errors in superconducting qubits by increasing the quasiparticle density in the vicinity of the Josephson junctions (JJs). Such errors are particularly harmful as they cannot be easily remedied via conventional error correcting codes. Recent experiments reduced correlated errors by making the difference in superconducting gap energy across the JJ larger than the qubit transition energy. In this work, we assess gap engineering near the JJ (δΔJJδΔ_{\mathrm{JJ}}δΔJJ​) and the capacitor/ground-plane (δΔM1δΔ_{\mathrm{M1}}δΔM1​) by exposing arrays of transmon qubits to two sources of radiation. For ααα-particles from an 241^{241}241Am source, we observe T1T_1T1​ errors correlated in space and time, supporting a hypothesis that hadronic cosmic rays are a major contributor to the 10−1010^{-10}10−10 error floor observed in Ref. 1. For electrons from a pulsed linear accelerator, we observe temporally correlated T1T_1T1​ and T2T_2T2​ errors, this measurement is insensitive to spatial correlations. We observe that the severity of correlated T1T_1T1​ errors is reduced for qubit arrays with a greater degree of gap engineering at the JJ. For both T1T_1T1​ and T2T_2T2​ errors, the recovery time is hastened by an increased δΔM1δΔ_{\mathrm{M1}}δΔM1​, which we attribute to the trapping of quasiparticles into the capacitor/ground-plane. We construct a model of quasiparticle dynamics that qualitatively agrees with our observations. This work reinforces the multifaceted influence of radiation on superconducting qubits and provides strategies for improving radiation resilience.