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arXiv:2503.05446 · Physical Review Letters

Cooperative Squeezing of Internal and Collective Spins in an Atomic Ensemble

Y.N. Zhang, Shenchao Jin, Junlei Duan, Klaus Mølmer, Guiying Zhang, Mingfeng Wang, Yanhong Xiao

Published Nov 20, 2025• 3 citations
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Abstract

Creating highly spin-squeezed states for quantum metrology surpassing the standard quantum limit is a topic of great interest. Spin squeezing has been achieved by either entangling different atoms in an ensemble, or by controlling the multilevel internal spin state of an atom. Here, we experimentally demonstrate combined internal and collective spin squeezing in a hot atomic ensemble with ∼10^{11} rubidium atoms. By synergistically combining these two types of squeezing and carefully aligning their squeezing quadratures, we have achieved a metrologically relevant spin squeezing of -6.21±0.84 dB, significantly outperforming the results obtained by utilizing either type of squeezing alone in our system. Our approach provides a new perspective on fully harnessing the degrees of freedom inherent in quantum states of an atomic ensemble.

DOI
10.1103/xkt1-y58b

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Creating highly spin-squeezed states for quantum metrology surpassing the standard quantum limit is a topic of great interest. Spin squeezing has been achieved by either entangling different atoms in an ensemble, or by controlling the multilevel internal spin state of an atom. Here, we experimentally demonstrate combined internal and collective spin squeezing in a hot atomic ensemble with ∼10^{11} rubidium atoms. By synergistically combining these two types of squeezing and carefully aligning their squeezing quadratures, we have achieved a metrologically relevant spin squeezing of -6.21±0.84 dB, significantly outperforming the results obtained by utilizing either type of squeezing alone in our system. Our approach provides a new perspective on fully harnessing the degrees of freedom inherent in quantum states of an atomic ensemble.
Spin squeezing generated via inter-atom entanglement in multilevel atomic ensembles provides a powerful resource for quantum-enhanced metrology. Existing schemes that harness internal atomic degrees of freedom to boost squeezing typically encode the collective squeezing in complex superpositions of magnetic sublevels, which complicates state control and limits practical applications. Here, we propose a coherent control scheme that simultaneously enhances collective spin squeezing and maps the resulting atom-atom entanglement onto two well-defined magnetic sublevels suitable for subsequent metrology experiments. Our protocol sandwiches a quantum non-demolition measurement between two internal one-axis-twisting interactions arranged in an echo sequence. We show that this approach can optimally leverage internal states to boost the inter-atom entanglement and, at the same time, encode it in two magnetic sublevels, which is readily convertible into metrologically useful spin squeezing. Our results offer a straightforward and efficient strategy for generating highly entangled yet readily accessible quantum states in multilevel atomic systems.
Quantum control of many body atomic spins is often pursued in the context of an atom-light quantum interface, where a quantized light field acts as a "quantum bus" that can be used to entangle distant atoms. One key challenge is to improve the coherence of the atom-light interface and the amount of atom-light entanglement it can generate, given the constraints of working with multilevel atoms and optical fields in a 3D geometry. We have explored new ways to achieve this, through rigorous optimization of the spatial geometry, and through control of the internal atomic state. Our basic setup consists of a quantized probe beam passing through an atom cloud held in a dipole trap, first generating spin-probe entanglement through the Faraday interaction, and then using backaction from a measurement of the probe polarization to squeeze the collective atomic spin. The relevant figure of merit is the metrologically useful spin squeezing determined by the enhancement in the resolution of rotations of the collective spin, relative to the commonly used spin coherent state. With an optimized free-space geometry, and by using a 2-color probe scheme to suppress tensor light shifts, we achieve 3(2) dB of metrologically useful spin squeezing. We can further increase atom-light coupling by implementing internal state control to prepare spin states with larger initial projection noise relative to the spin coherent state. Under the right conditions this increase in projection noise can lead to stronger measurement backaction and increased atom-atom entanglement. With further internal state control the increased atom-atom entanglement can then be mapped to a basis where it corresponds to improved squeezing of, e.g., the physical spin-angular momentum or the collective atomic clock pseudospin. In practice, controlling the collective spin of N ~ 10⁶ atoms in this fashion is an extraordinarily difficult challenge because errors in the control of individual atoms tend to be highly correlated. By employing precise internal state control, we have prepared and detected projection noise limited "cat" states (which have initial projection noise that is larger by a factor of 2f = 8 for Cs relative to the spin coherent state) and estimate that we can generate up to 6.0(5) dB of metrologically useful spin squeezing, demonstrating the advantage of using the internal atomic structure as a resource for ensemble control.
We demonstrate spin squeezing in a room temperature ensemble of approximately 10(12) cesium atoms using their internal structure, where the necessary entanglement is created between nuclear and electronic spins of each individual atom. This state provides improvement in measurement sensitivity beyond the standard quantum limit for quantum memory experiments and applications in quantum metrology and is thus a complementary alternative to spin squeezing obtained via interatom entanglement. Squeezing of the collective spin is verified by quantum state tomography.
Squeezed spin states and squeezed light are both key resources for quantum metrology and quantum information science, but have been separately investigated in experiments so far. Simultaneous generation of these two types of quantum states in one experiment setup is intriguing but remains a challenging goal. Here, we propose a novel protocol based on judiciously engineered symmetric atom-light interaction, and report proof-of-principle experimental results of concurrent spin squeezing of 0.61±0.09 dB and light squeezing of 0.65_{-0.10}^{+0.11} dB in a hot atomic ensemble. The squeezing process is deterministic, yielding fixed squeezing directions for both the light field and the collective atomic spin. Furthermore, the squeezed light modes lie in the multiple frequency sidebands of a single spatial mode. This new type of dual squeezed state is applicable for quantum enhanced metrology and quantum networks. Our method can be extended to other quantum platforms such as optomechanics, cold atoms, and trapped ions.
Unitary control of qudits can improve the collective spin squeezing of an atomic ensemble. Preparing the atoms in a state with large quantum fluctuations in magnetization strengthens the entangling Faraday interaction. The resulting increase in interatomic entanglement can be converted into metrologically useful spin squeezing. Further control can squeeze the internal atomic spin without compromising entanglement, providing an overall multiplicative factor in the collective squeezing. We model the effects of optical pumping and study the tradeoffs between enhanced entanglement and decoherence. For realistic parameters we see improvements of ~10 dB.
Squeezing of collective atomic spins has been shown to improve the sensitivity of atomic clocks and magnetometers to levels significantly below the standard quantum limit. In most cases the requisite atom-atom entanglement has been generated by dispersive interaction with a quantized probe field or by state-dependent collisions in a quantum gas. Such experiments typically use complex multilevel atoms like Rb or Cs, with the relevant interactions designed so that atoms behave like pseudospin-12\frac{1}{2}21​ particles. We demonstrate the viability of spin squeezing for collective spins composed of the physical angular momenta of 106{10}^{6}106 Cs atoms, each in an internal spin-4 hyperfine state. A peak metrological squeezing of at least 5dB is generated by quantum backaction from a dispersive quantum nondemolition (QND) measurement, implemented using a two-color optical probe that minimizes tensor light shifts without sacrificing measurement strength. Other significant developments include the successful application of composite pulse techniques for accurate dynamical control of the collective spin, enabled by broadband suppression of background magnetic fields inside a state-of-the-art magnetic shield. The absence of classical noise allows us to compare the observed quantum projection noise and squeezing to a theoretical model that properly accounts for both the relevant atomic physics and the spatial mode of the collective spin, finding good quantitative agreement and thereby validating its use in other contexts. Our work sets the stage for experiments on quantum feedback, deterministic squeezing, and closed-loop magnetometry. The implementation of real-time feedback may also create an opportunity for new types of quantum simulation, wherein the evolution of a quantum system is conditioned on the outcome of a time-continuous QND measurement. Such a scheme has the potential to access new regimes near the quantum-classical boundary, with opportunities to study long-standing issues related to quantum-classical correspondence in chaotic systems.