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arXiv:0802.2876 · Physical Review Letters

Spin Squeezing of Atomic Ensembles via Nuclear-Electronic Spin Entanglement

T. Fernholz, Hanna Krauter, Kasper Jensen, Jacob Friis Sherson, Anders Søndberg Sørensen, Eugene Simon Polzik

Published Aug 12, 2008• 170 citations
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Abstract

We demonstrate spin squeezing in a room temperature ensemble of approximately 10(12) cesium atoms using their internal structure, where the necessary entanglement is created between nuclear and electronic spins of each individual atom. This state provides improvement in measurement sensitivity beyond the standard quantum limit for quantum memory experiments and applications in quantum metrology and is thus a complementary alternative to spin squeezing obtained via interatom entanglement. Squeezing of the collective spin is verified by quantum state tomography.

DOI
10.1103/physrevlett.101.073601

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•Jan 1, 2014•3 citations
We demonstrate spin squeezing in a room temperature ensemble of approximately 10(12) cesium atoms using their internal structure, where the necessary entanglement is created between nuclear and electronic spins of each individual atom. This state provides improvement in measurement sensitivity beyond the standard quantum limit for quantum memory experiments and applications in quantum metrology and is thus a complementary alternative to spin squeezing obtained via interatom entanglement. Squeezing of the collective spin is verified by quantum state tomography.
Creating highly spin-squeezed states for quantum metrology surpassing the standard quantum limit is a topic of great interest. Spin squeezing has been achieved by either entangling different atoms in an ensemble, or by controlling the multilevel internal spin state of an atom. Here, we experimentally demonstrate combined internal and collective spin squeezing in a hot atomic ensemble with ∼10^{11} rubidium atoms. By synergistically combining these two types of squeezing and carefully aligning their squeezing quadratures, we have achieved a metrologically relevant spin squeezing of -6.21±0.84 dB, significantly outperforming the results obtained by utilizing either type of squeezing alone in our system. Our approach provides a new perspective on fully harnessing the degrees of freedom inherent in quantum states of an atomic ensemble.
Spin squeezing has been explored in atomic systems as a tool for quantum sensing, improving experimental sensitivity beyond the spin standard quantum limit for certain measurements. To optimize absolute metrological sensitivity, it is beneficial to consider macroscopic spin ensembles, such as nuclear spins in solids and liquids. Coupling a macroscopic spin ensemble to a parametrically-modulated resonant circuit can create collective spin squeezing by generating spin correlations mediated by the circuit. We analyze the squeezing dynamics in the presence of decoherence and finite spin polarization, showing that achieving 7 dB spin squeezing is feasible in several nuclear spin systems. The metrological benefit of squeezing a macroscopic spin ensemble lies in the suppression of technical noise sources in the spin detection system relative to the spin projection noise. This expands the experimental sensitivity bandwidth when searching for signals of unknown frequency and can improve the resonant signal-to-noise ratio. Squeezing macroscopic spin ensembles may prove to be a useful technique for fundamental physics experiments aimed at detecting spin interactions with oscillating background fields, such as ultralight dark matter.
Spin squeezing generated via inter-atom entanglement in multilevel atomic ensembles provides a powerful resource for quantum-enhanced metrology. Existing schemes that harness internal atomic degrees of freedom to boost squeezing typically encode the collective squeezing in complex superpositions of magnetic sublevels, which complicates state control and limits practical applications. Here, we propose a coherent control scheme that simultaneously enhances collective spin squeezing and maps the resulting atom-atom entanglement onto two well-defined magnetic sublevels suitable for subsequent metrology experiments. Our protocol sandwiches a quantum non-demolition measurement between two internal one-axis-twisting interactions arranged in an echo sequence. We show that this approach can optimally leverage internal states to boost the inter-atom entanglement and, at the same time, encode it in two magnetic sublevels, which is readily convertible into metrologically useful spin squeezing. Our results offer a straightforward and efficient strategy for generating highly entangled yet readily accessible quantum states in multilevel atomic systems.
Ultimate quantum fluctuations which limit the fundamental precision in metrology can be only reduced by entanglement of particles. In particular, squeezing of the fluctuations called the spin projection noise by means of generation of entanglement in an ensemble of atoms can improve the precision of spectroscopy and of atomic clocks. A powerful tool for generation of multiparticle entanglement is a quantum nondemolition measurement (QND). We will describe the fundamentals of QND measurement of atomic collective state with light and present a recent experiment [1] where this method has been used to reduce the projection noise on the clock transition in an ensemble of 105 cold and trapped Cesium atoms. Another method for generation of spin squeezing via electron-nucleus entanglement applicable only for atoms with angular momentum higher than ½ will be also discussed [2].
Unitary control of qudits can improve the collective spin squeezing of an atomic ensemble. Preparing the atoms in a state with large quantum fluctuations in magnetization strengthens the entangling Faraday interaction. The resulting increase in interatomic entanglement can be converted into metrologically useful spin squeezing. Further control can squeeze the internal atomic spin without compromising entanglement, providing an overall multiplicative factor in the collective squeezing. We model the effects of optical pumping and study the tradeoffs between enhanced entanglement and decoherence. For realistic parameters we see improvements of ~10 dB.
Abstract In this thesis, different experiments on spin squeezing and entanglement involving room temperature ensembles of Cesium atoms are described. The key method is the off-resonant Faraday interaction of spin-polarized atomic ensemble with a light field. And the key component is the micro-fabricated vapor cell coupled into an optical cavity. Quantum backaction evading measurement of one quadrature of collective spin components by stroboscopically modulating the intensity of probe beam at twice Larmor frequency is used to generate the spin-squeezed state. A projection noise limited optical magnetometer at room temperature is reported. Furthermore, using spin-squeezing of atomic ensemble, the sensitivity of magnetometer is improved. Deterministic continuous variable teleportation between two distant atomic ensembles is demonstrated. The fidelity of teleportating dynamically changing sequence of spin states surpasses a classical benchmark, demonstrating the true quantum teleportation.