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arXiv:2502.12818 · Physical Review A

Dynamics of open quantum systems with initial system-environment correlations via stochastic unravelings

Federico Settimo, Kimmo Luoma, Dariusz Chruściński, Andrea Smirne, Bassano Vacchini, Jyrki Piilo

Published Sep 11, 2025• 3 citations
arXivHTMLPDF

Abstract

In standard treatments of open quantum systems, the reduced dynamics is described starting from the assumption that the system and the environment are initially uncorrelated. This assumption, however, is not always guaranteed in realistic scenarios and several theoretical approaches to characterize initially correlated dynamics have been introduced. For the uncorrelated scenario, stochastic unravelings are a powerful tool to simulate the dynamics. So far they have not been used in the most general case in which correlations are initially present since they cannot be applied to nonpositive operators or noncompletely positive maps. In our work, we employ the bath positive $(\mathrm{B}+)$ or one-sided positive decomposition (OPD) formalism as a starting point to generalize stochastic unraveling in the presence of initial correlations. Noticeably, our approach does not depend on the particular unraveling technique, but holds for both piecewise deterministic and diffusive unravelings. This generalization allows not only for more powerful simulations for the reduced dynamics, but also for a deeper theoretical understanding of open system dynamics.

DOI
10.1103/q353-4232

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In standard treatments of open quantum systems, the reduced dynamics is described starting from the assumption that the system and the environment are initially uncorrelated. This assumption, however, is not always guaranteed in realistic scenarios and several theoretical approaches to characterize initially correlated dynamics have been introduced. For the uncorrelated scenario, stochastic unravelings are a powerful tool to simulate the dynamics. So far they have not been used in the most general case in which correlations are initially present since they cannot be applied to nonpositive operators or noncompletely positive maps. In our work, we employ the bath positive (B+)(\mathrm{B}+)(B+) or one-sided positive decomposition (OPD) formalism as a starting point to generalize stochastic unraveling in the presence of initial correlations. Noticeably, our approach does not depend on the particular unraveling technique, but holds for both piecewise deterministic and diffusive unravelings. This generalization allows not only for more powerful simulations for the reduced dynamics, but also for a deeper theoretical understanding of open system dynamics.
Stochastic unravelings represent a useful tool to describe the dynamics of open quantum systems, and standard methods, such as quantum state diffusion (QSD), call for the complete positivity of the open-system dynamics. Here, we present a generalization of QSD, which also applies to positive, but not completely positive evolutions. The rate and the action of the diffusive processes involved in the unraveling are obtained by applying a proper transformation to the operators which define the master equation. The unraveling is first defined for semigroup dynamics and then extended to a definite class of time-dependent generators. We test our approach on a prototypical model for the description of exciton transfer, keeping track of relevant phenomena, which are instead disregarded within the standard, completely positive framework.
We show that the dynamics of any open quantum system that is initially correlated with its environment can be described by a set of d2{d}^{2}d2 (or less) completely positive maps, where ddd is the dimension of the system. Only one such map is required for the special case of no initial correlations. The same maps describe the dynamics of any system-environment state obtained from the initial state by a local operation on the system. The reduction of the system dynamics to a set of completely positive maps allows known numerical and analytic tools for uncorrelated initial states to be applied to the general case of initially correlated states, which we exemplify by solving the qubit dephasing model for such states, and provides a natural approach to quantum Markovianity for this case. We show that this set of completely positive maps can be experimentally characterized using only local operations on the system, via a generalization of noise spectroscopy protocols. As further applications, we first consider the problem of retrodicting the dynamics of an open quantum system which is in an arbitrary state when it becomes accessible to the experimenter and explore the conditions under which retrodiction is possible. We also introduce a related one-sided or limited-access tomography protocol for determining an arbitrary bipartite state, evolving under a sufficiently rich Hamiltonian, via local operations and measurements on just one component. We simulate this protocol for a physical model of particular relevance to nitrogen-vacancy centers and in particular show how to reconstruct the density matrix of a set of three qubits, interacting via dipolar coupling and in the presence of local magnetic fields, by measuring and controlling only one of them.
Stochastic unravelings allow to efficiently simulate open system dynamics, yet their application has traditionally been restricted to master equations that preserve both Hermiticity and trace. In this work, we introduce a general framework that extends piecewise-deterministic unravelings to arbitrary trace-nonpreserving master equations, requiring only positivity and Hermiticity of the dynamics. Our approach includes, as special cases, unravelings of arbitrary dynamics in the Heisenberg picture, evolutions interpolating between fully Lindblad and non-Hermitian Hamiltonian generators, and equations employed in the derivation of full counting statistics, for which we show it can be used to obtain the moments of the associated probability distribution. The framework is suitable for both trace-decreasing and trace-increasing processes through stochastic disappearance and replication of the stochastic realizations, and it is compatible with different unraveling schemes and with reverse jumps in the non-Markovian regime. Thereby, our approach provides a powerful and versatile simulation method that significantly broadens the applicability of stochastic techniques for open system dynamics.
We consider open quantum systems with factorized initial states, providing the structure of the reduced system dynamics, in terms of environment cumulants. We show that such completely positive (CP) and trace-preserving (TP) maps can be unraveled by linear stochastic Schr\"odinger equations (SSEs) characterized by sets of colored stochastic processes (with nthn\mathrm{th}nth-order cumulants). We obtain both the conditions such that the SSEs provide CPTP dynamics and those for unraveling an open system dynamics. We then focus on Gaussian non-Markovian unravelings, whose known structure displays a functional derivative. We provide a description that replaces the functional derivative with a recursive operatorial structure. Moreover, for the family of quadratic bosonic Hamiltonians, we are able to provide an explicit operatorial dependence for the unraveling.
Stochastic unravelings provide a useful way to represent open quantum system dynamics in terms of pure state realizations, and have been widely studied both from a fundamental and from a computational point of view. They were initially formulated for Markovian dynamics described by the Gorini-Kossakowski-Sudarshan-Lindblad master equation. However, due to recent technological and experimental development, most physical relevant dynamics present temporal correlations beyond the Markov approximation. Such correlations cause decay rates to turn temporarily negative, thus requiring the generalization of stochastic unravelings from Markovian to non-Markovian scenarios. Indeed, many unraveling techniques have been introduced in this regime, and a comprehensive review of the different jump methods is currently missing. In this work, we provide an overview of widely used quantum jump unraveling techniques for non-Markovian systems and also discuss them in terms of their numerical efficiency, divisibility requirements, Hilbert space extension, and measurement interpretation.
Abstract We investigate the dynamics of open quantum systems which are initially correlated with their environment. The strategy of our approach is to analyze how given, fixed initial correlations modify the evolution of the open system with respect to the corresponding uncorrelated dynamical behavior with the same fixed initial environmental state, described by a completely positive dynamical map. We show that, for any predetermined initial correlations, one can introduce a linear dynamical map on the space of operators of the open system which acts like the proper dynamical map on the set of physical states and represents its unique linear extension. Furthermore, we demonstrate that this construction leads to a linear, time-local quantum master equation with generalized Lindblad structure involving time-dependent, possibly negative transition rates. Thus, the general non-Markovian dynamics of an open quantum system can be described by means of a time-local master equation even in the case of arbitrary, fixed initial system–environment correlations. We present some illustrative examples and explain the relation of our approach to several other approaches proposed in the literature.